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Synthesis of novel nanomaterials and their application in efficient removal of radionuclides

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Abstract

With the development of nuclear energy, large amounts of radionuclides are inevitably released into the natural environment. It is necessary to eliminate radionuclides from wastewater for the protection of environment. Nanomaterials have been considered as the potential candidates for the effective and selective removal of radionuclides from aqueous solutions under complicated conditions because of their high specific surface area, large amounts of binding sites, abundant functional groups, pore-size controllable and easily surface modification. This review mainly summarized the recent studies for the synthesis, fabrication and surface modification of novel nanomaterials and their applications in the efficient elimination and solidification of radionuclides, and discussed the interaction mechanisms from batch experiments, spectroscopy analysis and theoretical calculations. The sorption capacities with other materials, advantages and disadvantages of different nanomaterials are compared, and at last the perspective of the novel nanomaterials is summarized.

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Acknowledgements

This work was supported by the Science Challenge Project (TZ2016004), and the National Natural Science Foundation of China (21836001, 21876048).

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Authors and Affiliations

  1. Key Laboratory of Resources and Environmental Systems Optimization, Ministry of Education, College of Environmental Science and Engineering, North China Electric Power University, Beijing, 102206, China

    Xiangxue Wang, Shujun Yu & Xiangke Wang

  2. State Key Laboratory of Radiation Medicine and Protection, School of Radiation Medicine and Protection, Collaborative Innovation Center of Radiological Medicine of Jiangsu Higher Education Institutions, Soochow University, Suzhou, 215123, China

    Long Chen, Chengliang Xiao & Shuao Wang

  3. Laboratory of Nuclear Energy Chemistry and Key Laboratory for Biomedical Effects of Nanomaterials and Nanosafety, Institute of High Energy Physics, Chinese Academy of Sciences, Beijing, 100049, China

    Lin Wang & Weiqun Shi

  4. Key Laboratory of Petroleum Resources, Gansu Province, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou, 730000, China

    Qiaohui Fan

  5. Radiochemistry Laboratory, School of Nuclear Science and Technology, Lanzhou University, Lanzhou, 730000, China

    Duoqiang Pan & Wangsuo Wu

  6. CAS Key Laboratory of Photovoltaic and Energy Conservation Materials, Institute of Plasma Physics, Chinese Academy of Sciences, Hefei, 230031, China

    Jiaxing Li, Yi Xie & Changlun Chen

  7. Fundamental Science on Nuclear Wastes and Environmental Safety Laboratory, Southwest University of Science and Technology, Mianyang, 621010, China

    Fangting Chi

  8. State Key Laboratory of Nuclear Resources and Environment, School of Biology, Chemistry and Material Science, East China University of Technology, Fuzhou, 344000, China

    Feng Luo

  9. College of Materials Science and Chemical Engineering, Harbin Engineering University, Harbin, 150001, China

    Jun Wang

  10. China Academy of Engineering Physics, Mianyang, 621900, China

    Xiaolin Wang

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  1. Xiangxue Wang
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  2. Long Chen
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  3. Lin Wang
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  17. Shuao Wang
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  18. Xiangke Wang
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Corresponding authors

Correspondence to Feng Luo, Jun Wang, Xiaolin Wang, Changlun Chen, Wangsuo Wu, Weiqun Shi, Shuao Wang or Xiangke Wang.

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Wang, X., Chen, L., Wang, L. et al. Synthesis of novel nanomaterials and their application in efficient removal of radionuclides. Sci. China Chem. 62, 933–967 (2019). https://doi.org/10.1007/s11426-019-9492-4

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  • DOI: https://doi.org/10.1007/s11426-019-9492-4

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