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Interaction of radionuclides with natural and manmade materials using XAFS technique

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Abstract

The X-ray absorption fine structure (XAFS) technology has exhibited a very unique application in the study of sorption mechanism, chemical species and microstructures of radionuclides at the natural solid-water interfaces. In this review, the interaction mechanism of radionuclides with clay minerals and nanomaterials under different environmental conditions are summarized from the XAFS spectroscopy analysis. The coordination number and the bond distances of radionuclides, the oxidation-reduction reactions, the influence of humic substances and microorganisms on the species and structures of radionuclides at molecule level are reviewed and compared. This review is helpful to understand the interactions of radionuclides with oxides, natural clay minerals and nanomaterials, which is also crucial to evaluate the physicochemical behaviors of radionuclides in the natural environment.

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Acknowledgments

This work was supported from the National Natural Science Foundation of China (21225730, 91326202, 21577032), the Fundamental Research Funds for the Central Universities (JB2015001), and the Priority Academic Program Development of Jiangsu Higher Education Institutions, the Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions.

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Authors and Affiliations

  1. School of Environment and Chemical Engineering, North China Electric Power University, Beijing, 102206, China

    Shujun Yu, Xiangxue Wang, Shitong Yang, Guodong Sheng & Xiangke Wang

  2. Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions, Suzhou, 215123, China

    Shitong Yang & Xiangke Wang

  3. College of Chemistry and Chemical Engineering, Shaoxing University, Shaoxing, 312000, China

    Guodong Sheng

  4. Nonlinear Analysis and Applied Mathematics (NAAM) Research Group, Faculty of Science, King Abdulaziz University, Jeddah, 21589, Saudi Arabia

    Guodong Sheng, Ahmed Alsaedi, Tasawar Hayat & Xiangke Wang

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  1. Shujun Yu
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  6. Tasawar Hayat
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  7. Xiangke Wang
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Correspondence to Xiangke Wang.

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Yu, S., Wang, X., Yang, S. et al. Interaction of radionuclides with natural and manmade materials using XAFS technique. Sci. China Chem. 60, 170–187 (2017). https://doi.org/10.1007/s11426-016-0317-3

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  • DOI: https://doi.org/10.1007/s11426-016-0317-3

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