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New insights on (V10O28)6−-based electrode materials for energy storage: a brief review

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Abstract

Progress in humanity has intensified the demand for efficient and renewable energy storage, which warrants the development of advanced rechargeable batteries such as lithium-ion batteries (LIBs), sodium-ion batteries (SIBs), zinc-ion batteries (ZIBs), and lithium-sulfur batteries (Li–S batteries). Nevertheless, these batteries still suffer from certain limitations, such as the insufficient capacity and inferior stability in their electrode materials. Therefore, developing a feasible electrode material for Li/Na/Zn ion storage represents a critical challenge. Recently, polyoxovanadates (POVs) materials, particularly decavanadate anion (V10O28)6− clusters, have attracted considerate attention as promising battery electrodes, due to their rich multi-electron redox process, high structural stability, simple preparation process, and abundant ligand environment. In this review, we provide an overview of the research progress of (V10O28)6−-based materials in various metal-ion battery systems, including LIBs, SIBs, ZIBs, and Li–S batteries. We also discuss the underlying challenges associated with this type of materials, and we provide alternative strategies to overcome these issues. This review aims to facilitate the research and development of the next-generation (V10O28)6−-based battery materials.

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摘要

人类的进步加大了对高效和可再生存储能源的需求，这促使了我们需大量开发先进的可充电电池，如锂离子电池（LIBs）、钠离子电池（SIBs）、锌离子电池（ZIBs）和锂硫电池（Li-S电池）。然而，这些电池仍然存在一定的限制，例如电极材料的容量偏低以及稳定性较差的问题。因此，亟需开发性能优异的存储锂/钠/锌离子的电极材料。最近，基于十钒酸阴离子(V10O28)6−团簇的多金属钒氧酸盐(POVs)材料因具有多电子氧化还原过程、良好的结构稳定性、简单的制备过程以及丰富的配位环境等优点，被视为有前途的电池电极材料，引起了人们的广泛关注。在这篇综述中，我们系统地概述了(V10O28)6−基材料在各种金属离子电池系统中的研究进展，包括LIBs、SIBs、ZIBs和Li-S电池。我们还讨论了与这类材料相关的挑战，并提供了克服这些问题的策略。本综述旨在促进下一代(V10O28)6−基电池材料的研究和开发。

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Fig. 1
Fig. 2

Reproduced with permission from Ref. [43]. Copyright 2006, Elsevier. g 51 V NMR spectrum of Na6[V10O28]; h normalized in situ V K-edge XANES spectra for redox process of Na6[V10O28] cathodes; i examples of transient currents with fitting curves at 25 °C. Reproduced with permission from Ref. [45]. Copyright 2017, The Royal Society of Chemistry

Fig. 3

Reproduced with permission from Ref. [46]. Copyright 2017, The Royal Society of Chemistry

Fig. 4

Reproduced with permission from Ref. [49]. Copyright 2015, Elsevier

Fig. 5

Reproduced with permission from Ref. [38]. Copyright 2022, Wiley–VCH GmbH. g Synthesis scheme of Na6V10O28·18H2O. Reproduced with permission from Ref. [59]. Copyright 2022, Elsevier

Fig. 6

Reproduced with permission from Ref. [60]. Copyright 2022, Wiley–VCH GmbH

Fig. 7

Reproduced with permission from Ref. [62]. Copyright 2020, Elsevier

Fig. 8

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Acknowledgements

This work was financially supported by the National Natural Science Foundation of China (Nos. 52071132, U21A20284 and U1904216), Zhongyuan Thousand People Plan-The Zhongyuan Youth Talent Support Program (in Science and Technology), China (No. ZYQR201810139), the Innovative Funds Plan of Henan University of Technology, China (No. 2020ZKCJ04), and the Natural Science Foundation of Henan, China (No. 222300420138). Additionally, Dr. Xianyong Wu acknowledges the support from the NSF Center for the Advancement of Wearable Technologies (No. 1849243).

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Authors and Affiliations

  1. School of Chemistry and Chemical Engineering, Henan University of Technology, Zhengzhou, 450001, China

    Tao Zhou, Yu Niu, Hao-Ran Xiao, Yu-Jie Li, Qing Han, Xin-Li Yang, Li-Min Zhu & Xiao-Yu Cao

  2. School of Environmental Engineering, Henan University of Technology, Zhengzhou, 450001, China

    Ling-Ling Xie & Xue-Jing Qiu

  3. Key Laboratory of High Specific Energy Materials for Electrochemical Power Sources of Zhengzhou City, Zhengzhou, 450001, China

    Tao Zhou, Ling-Ling Xie, Yu Niu, Hao-Ran Xiao, Yu-Jie Li, Qing Han, Xue-Jing Qiu, Xin-Li Yang & Xiao-Yu Cao

  4. Department of Chemistry, University of Puerto Rico-Rio Piedras Campus, San Juan, PR, 00925, USA

    Xian-Yong Wu

  5. School of Chemistry and Chemical Engineering, Yangzhou University, Yangzhou, 225009, China

    Li-Min Zhu & Huan Pang

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  1. Tao Zhou
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Zhou, T., Xie, LL., Niu, Y. et al. New insights on (V10O28)6−-based electrode materials for energy storage: a brief review. Rare Met. 42, 1431–1445 (2023). https://doi.org/10.1007/s12598-022-02207-7

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