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A data set for validation of models of laser-induced incandescence from soot: temporal profiles of LII signal and particle temperature

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Abstract

We measured spectrally and temporally resolved laser-induced incandescence signals from flame-generated soot at laser fluences of 0.01–3.5 J/cm2 and laser wavelengths of 532 and 1,064 nm. We recorded LII temporal profiles at 681.8 nm using a fast-gated detector and a spatially homogeneous and temporally smooth laser profile. Time-resolved emission spectra were used to identify and avoid spectral interferences and to infer soot temperatures. Soot temperatures reach a maximum of 4,415 ± 65 K at fluences ≥0.2 J/cm2 at 532 nm and 4,424 ± 80 K at fluences ≥0.3 J/cm2 at 1,064 nm. These temperatures are consistent with the sublimation temperature of C2 of 4,456.59 K. At fluences above 0.5 J/cm2 at 532 nm, the measured spectra yield an apparent higher temperature after the soot has fully vaporized but well within the laser pulse. This apparent temperature elevation at high fluence is explained by fluorescence interferences from molecules present in the flame. We also measured 3-color LII temporal profiles at detection wavelengths of 451.5, 681.8, and 854.8 nm. The temperatures inferred from these measurements agree well with those measured using spectrally resolved LII. The data discussed in this manuscript are archived as electronic supplementary material.

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Acknowledgments

We thank László Nemes for his valuable comments on the manuscript. We also thank Daniel Strong for the rendition of the experimental setup shown in Fig. 1. This work was supported by the Division of Chemical Sciences, Geosciences, and Biosciences, the Office of Basic Energy Sciences, the US Department of Energy. Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration under contract DE-AC04-94-AL85000.

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  1. Fabien Goulay

    Present address: Department of Chemistry, West Virginia University, Morgantown, WV, 26506, USA

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  1. Combustion Research Facility , Sandia National Laboratories, MS 9055, P. O. Box 969, Livermore, CA, 94551, USA

    Fabien Goulay, Paul E. Schrader, Xerxes López-Yglesias & Hope A. Michelsen

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  1. Fabien Goulay
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Goulay, F., Schrader, P.E., López-Yglesias, X. et al. A data set for validation of models of laser-induced incandescence from soot: temporal profiles of LII signal and particle temperature. Appl. Phys. B 112, 287–306 (2013). https://doi.org/10.1007/s00340-013-5504-4

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