Abstract
Better soft magnetic properties of magnetic thin films are needed as micro-electromechanical systems electromagnetic devices become high-frequency, miniaturized, and integrated. Multilayer magnetic composites outperform single-layer materials in performance and flexibility, attracting interest. However, lamination’s effect on the soft magnetic properties of magnetic composites remains unclear. This study created a Comsol finite-element simulation model of the magnetic film to evaluate how lamination affects the eddy current suppression rate (SR) and magnetostriction performance reduction rate (RR). In addition, incorporating the experimental findings related to the soft magnetic properties, the magnetic composite material had been effectively developed: after inserting ten layers of 5 nm alumina film, the eddy current SR reached 92.8%, while the magnetostriction RR and coercive force were found to be merely 7.1% and 2 × 79.6 A/m, respectively. Furthermore, an investigation of the microscopic mechanism behind the impact of lamination on the properties of the magnetic film is also being addressed. It is found that the substrate and thickness effect simultaneously determine the properties of the single-layer magnetic film. In addition, the complex interlayer coupling effect between the isolated magnetic films is another critical factor affecting the soft magnetic properties of the magnetic composites. This study provides an optimal design approach for magnetic composite materials and clarifies the internal effect mechanism to improve the soft magnetic properties of those materials. The findings offer guidance for the application of high-frequency magnetic devices.
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References
Q. Pan, X.Y. Zhang, B.J. Xia, B.J. Chu, Magnetoelectric response in laminated BaFe12O19/Pb (Zr, Ti) O3 composites. J. Appl. Phys. (2023). https://doi.org/10.1063/5.0150380
S. Sadhukhan, A. Mahapatra, A. Mitra, N. Bhakta, S. Das, A. Mallick, A. Banerjee, S. Chatterjee, J. Greneche, P.K. Chakrabarti, Strong modulation effects on magnetoelectric behavior of Co-ferrite nanoparticles incorporated in ZnO medium in nano-regime synthesized in chemical routes. Appl. Phys. A (2023). https://doi.org/10.1007/s00339-022-06345-8
M. Sufyan, Z.Y. Lu, Z.W. Chen, X. Wang, M.W. Hanif, Magnetoelectric response of 3-phase (1–x)[0.7BiFeO3-0.3CoFe2O4]-xPbTiO3 multiferroic ceramic composites. Appl. Phys. A. (2023). https://doi.org/10.1007/s00339-022-06286-2
F.S. Bruckmann, F.B. Nunes, T.R. Salles, C. Franco, F.C. Cadona, C.R.B. Rhoden, Biological applications of silica-based nanoparticles. Magnetochemistry 8, 10 (2022)
F.B. Nunes, F.S. Bruckmann, T.R. Salles, C.R.B. Rhoden, Study of phenobarbital removal from the aqueous solutions employing magnetite-functionalized chitosan. Environ. Sci. Pollut. R. 30(5), 12658–12671 (2023)
T.R. Salles, F.S. Bruckmann, A.R. Viana, L.M.F. Krause, S.R. Mortari, C.R.B. Rhoden, Magnetic nanocrystalline cellulose: azithromycin adsorption and in vitro biological activity against melanoma cells. J. Polym. Environ. 30(7), 2695–2713 (2022)
Z.F. Yao, S. Tiwari, J.D. Schneider, R. Candler, G. Carman, Y. Wang, Enhanced planar antenna efficiency through magnetic thin-films. IEEE J. Multiscale Multiphys. Comput. Tech. 6, 249–258 (2021)
K. Yadagiri, Y. Wang, P. Wu, T. Wu, Ferromagnetic resonance properties of multilayer FeGaB/Ta/FeGaB structure. J. Mater. Sci. 33(7), 3870–3879 (2022)
K. Yadagiri, J.W. Long, Y.X. Wang, Z. Zhu, T. Wu, Magnetodynamic properties on square patterned of FeGaB and Al2O3/FeGaB thin films. J. Mater. Sci. 33(19), 15927–15935 (2022)
X. Xing, M. Liu, S.D. Li, O. Obi, J. Lou, Z.Y. Zhou, B. Chen, N.X. Sun, RF magnetic properties of FeCoB/Al2O3/FeCoB structure with varied Al2O3 thickness. IEEE Trans. Magn. 47, 3104–3107 (2011)
I. Shahid, G. Yin, J. Yuan, Y.G. Ma, S.L. He, FeGaB(25 nm)/Al2O3/FeGaB(25 nm) multilayer structures: effects of variation of Al2O3 thickness on static and dynamic magnetic properties. Rare Metal Mat. Eng. 47, 1951–1957 (2018)
Y. Karampuri, Y.X. Wang, T. Wu, Ferromagnetic resonance and spin-wave exchange stiffness of FeGaB/Al2O3 multilayer thin film stack for microwave applications. Mater. Chem. Phys. 279, 125776 (2022)
T. Nan, H. Lin, Y. Gao, A.D. Matyushov, G.L. Yu, H.H. Chen, N. Sun, S.J. Wei, Z.G. Wang, M.H. Li, X.J. Wang, A.M. Belkessam, R. Guo, B. Chen, J. Zhou, Z. Qian, Y. Hui, M. Rinaldi, M. Mcconney, B. Howe, Z.Q. Hu, J.G. Brown, N. Sun, Acoustically actuated ultra-compact NEMS magnetoelectric antennas. Nat. Commun. (2017). https://doi.org/10.1038/s41467-017-00343-8
Y.F. He, Y. Gao, H.H. Chen, H. Lin, Y.Y. Wei, X. Yang, N. Sun, Integrated tunable bandstop filter using self-biased FeGaB/Al2O3 multilayer thin film. IEEE T. Magn. 54(9), 1–4 (2018)
W.C. Ren, J.T. Li, G. Liu, J.R. Chen, S. Chen, Z.J. Gu, J.B. Li, J.R. Li, Y. Gao, Design and optimization of a BAW magnetic sensor based on magnetoelectric coupling. Micromachines 13(2), 206 (2022)
W.C. Ren, J.T. Li, S. Chen, G.F. Wang, P.C. Zhu, J.C. Chen, Eddy current suppression and soft magnetism enhancement in FeGaB-based magnetic composites with alumina lamination. J. Magn. Magn. Mater. 574, 170714 (2023)
Z.M. Cai, C.Q. Zhu, L.W. Wu, B.C. Luo, P. Feng, X.H. Wand, Vortex domain configuration for energy-storage ferroelectric ceramics design: a phase-field simulation. Appl. Phys. Lett. (2021). https://doi.org/10.1063/5.0051853
P.C. Xiong, W.B. Ma, S. Yuan, Y. Liu, B. Wand, Control of the chirality of a vortex in a ferroelectric nanodot by uniform electric fields mediated by inhomogeneous surface screening. AIP Adv. (2022). https://doi.org/10.1063/5.0076281
W. Xiong, W.J. Chen, Y. Zheng, Path-dependent vortex switching in ferroelectric nanoplate junctions toward a memory device concept. Front. Phys. (2022). https://doi.org/10.3389/fphy.2021.791019
J. Lindner, K. Baberschke, Ferromagnetic resonance in coupled ultrathin films. J. Phys. Condens. Mat. 15(5), S465–S478 (2003)
M. Endo, S. Kanai, F. Matsukura, H. Ohno, Electric-field effects on thickness dependent magnetic anisotropy of sputtered MgO/Co40Fe40B20/Ta structures. Appl. Phys. Let. (2010). https://doi.org/10.1063/1.3429592
F.D. Broeder, W. Hoving, P. Bloemen, Magnetic anisotropy of multilayers. J. Magn. Magn. Mater. 93, 562–570 (1991)
P. Gowtham, G. Stiehi, D. Ralph, R. Buhrman, Thickness-dependent magnetoelasticity and its effects on perpendicular magnetic anisotropy in Ta/CoFeB/MgO thin films. Phys. Rev. B (2016). https://doi.org/10.1103/PhysRevB.93.024404
Y.L. Bai, J.Y. Chen, S.F. Zhao, Q.S. Lu, Magneto-dielectric and magnetoelectric anisotropies of CoFe 2O4/Bi5Ti3FeO15 bilayer composite heterostructural films. RSC Adv. 6(57), 52353–52359 (2016)
Funding
This work was supported by the Science and Technology on Electronic Information Control Laboratory (Grant number: 6142105200203).
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WR: conceptualization, methodology, writing, analysis. JL: deposition, characteristics, analysis. TW: deposition, characteristics. BL: conceptualization, methodology. GW: simulation, data collection. ZW: deposition, data processing. CL: investigation, formal analysis. TL: modeling. HG: software.
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Ren, W., Li, J., Wei, T. et al. Soft magnetic properties enhancement of FeGaB composites through alumina lamination and its mechanism. Appl. Phys. A 129, 696 (2023). https://doi.org/10.1007/s00339-023-06989-0
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DOI: https://doi.org/10.1007/s00339-023-06989-0