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Highly efficient 1D p-Te/2D n-Bi2Te3 heterojunction self-driven broadband photodetector

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Abstract

Broadband photodetectors with self-driven functions have attracted intensive scientific interest due to their low energy consumption and high optical gain. However, high-performance broadband self-driven photodetectors are still a significant challenge due to the complex fabrication processes, environmental toxicity, high production costs of traditional 3D semiconductor materials and sharply raised contact resistance, severe interfacial recombination of 2D materials and 2D/3D mixed dimension heterojunction. Here, 1D p-Te/2D n-Bi2Te3 heterojunctions are constructed by the simple and low-cost hydrothermal method. 1D p-Te/2D n-Bi2Te3 devices are applied in photoelectrochemical (PEC) photodetectors, with their high performance attributed to the good interfacial contacts reducing interface recombination. The device demonstrated a broad wavelength range (365–850 nm) with an/ph//dark as high as 377.45. The RiD*, and external quantum efficiency (EQE) values of the device were as high as 12.07 mA/W, 5.87 × 1010 Jones, and 41.05%, respectively, which were significantly better than the performance of the prepared Bi2Te3 and Te devices. A comparison of the freshly fabricated device and the device after 30 days showed that 1D p-Te/2D n-Bi2Te3 had excellent stability with only 18.08% decay of photocurrent. It is anticipated that this work will provide new emerging material for future design and preparation of a high-performance self-driven broadband photodetector.

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Acknowledgements

This work was supported by the National Key Research and Development Program of China (No. 2019YFA0705201), and the National Natural Science Foundation of China (No. U2032129).

Author information

Authors and Affiliations

  1. School of Materials Science and Engineering, Harbin Institute of Technology, Harbin, 150001, China

    Chenchen Zhao, Dongbo Wang, Zhi Zeng, Bingke Zhang, Jingwen Pan, Donghao Liu, Sihang Liu, Shujie Jiao, Tianyuan Chen, Liancheng Zhao & Jinzhong Wang

  2. School of Astronautics, Harbin Institute of Technology, Harbin, 150001, China

    Jiamu Cao

  3. Center for High Pressure Science and Technology Advanced Research, Shanghai, 201203, China

    Gang Liu

  4. State Key Laboratory of High Power Semiconductor Lasers, Changchun University of Science and Technology, Changchun, 130022, China

    Xuan Fang

Authors
  1. Chenchen Zhao
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  2. Dongbo Wang
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  3. Jiamu Cao
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  4. Zhi Zeng
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  5. Bingke Zhang
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  6. Jingwen Pan
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  7. Donghao Liu
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  8. Sihang Liu
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  9. Shujie Jiao
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  10. Tianyuan Chen
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  11. Gang Liu
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  12. Xuan Fang
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  13. Liancheng Zhao
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  14. Jinzhong Wang
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Corresponding authors

Correspondence to Dongbo Wang, Jiamu Cao, Gang Liu, Xuan Fang or Jinzhong Wang.

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Zhao, C., Wang, D., Cao, J. et al. Highly efficient 1D p-Te/2D n-Bi2Te3 heterojunction self-driven broadband photodetector. Nano Res. 17, 1864–1874 (2024). https://doi.org/10.1007/s12274-023-5905-6

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  • DOI: https://doi.org/10.1007/s12274-023-5905-6

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