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Study the impact of sintering temperature on electromagnetic properties of (1 − y) [Ba0.9Ca0.1Zr0.1Ti0.9O3] + (y) [Ni0.25Cu0.13Zn0.62Fe2O4] composites

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Abstract

In this study, polycrystalline (1 − y) [Ba0.9Ca0.1Zr0.1Ti0.9O3] (BCZTO) + (y) [Ni0.25Cu0.13Zn0.62Fe2O4] (NCZFO) (where y = 0.0–1.0) composites via the solid-state reaction approach. The evolution of the cubic structure for NCZFO and tetragonal structure for BCZTO was confirmed by XRD and FTIR studies. The dielectric constant was decreased with increasing NCZFO content due to the dilution effect. The dielectric properties were improved with increasing sintering temperature. A close resemblance between the porosity corrected and measured dielectric constant was noticed. The small polaron hopping model was responsible for the electrical conduction. Complex impedance analysis revealed that the grain boundaries have a greater impact on overall electric properties. The permeability was increased with increasing NCZFO content. The dielectric constant and permeability were calculated theoretically using the different models and compared with experimental values. The disparity between the experimental and calculated values of dielectric constant and permeability might be attributed to the diffusion of ions and interaction between two phases.

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Acknowledgements

The authors are sincerely thankful to the Department of Physics, University of Dhaka, Bangladesh for providing the necessary materials to perform this study. The authors also sincerely acknowledge the authority of the Center for Advanced Research in Sciences (CARS), University of Dhaka and Solid-State Physics Laboratory, Department of Physics, Bangladesh University of Engineering and Technology (BUET), Dhaka, Bangladesh for providing characterization facilities. Sharifa Nasrin is grateful to the University Grants Commission, Bangladesh for providing a Basic Science Research fellowship for the present research work. Sharifa Nasrin, also grateful to the Directorate of Secondary and Higher Education (DSHE), Ministry of Education, Government of the People’s Republic of Bangladesh for providing study leave to pursue Ph.D. research at the Department of Physics, University of Dhaka, Bangladesh.

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Authors and Affiliations

  1. Department of Physics, University of Dhaka, Dhaka, 1000, Bangladesh

    Sharifa Nasrin, Most. Sharmin & Md. D. Rahaman

  2. Directorate of Secondary and Higher Education (DSHE), Ministry of Education, Government of the People’s Republic of Bangladesh, Dhaka, 1000, Bangladesh

    Sharifa Nasrin

  3. Department of Glass and Ceramic Engineering, Bangladesh University Engineering and Technology (BUET), Dhaka, 1000, Bangladesh

    M. A. Matin

  4. Department of Physics, Bangladesh University Engineering and Technology (BUET), Dhaka, 1000, Bangladesh

    A. K. M. Akther Hossain

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  1. Sharifa Nasrin
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  2. Most. Sharmin
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  3. M. A. Matin
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  4. A. K. M. Akther Hossain
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  5. Md. D. Rahaman
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Correspondence to Md. D. Rahaman.

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Nasrin, S., Sharmin, M., Matin, M.A. et al. Study the impact of sintering temperature on electromagnetic properties of (1 − y) [Ba0.9Ca0.1Zr0.1Ti0.9O3] + (y) [Ni0.25Cu0.13Zn0.62Fe2O4] composites. Appl. Phys. A 127, 59 (2021). https://doi.org/10.1007/s00339-020-04172-3

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  • DOI: https://doi.org/10.1007/s00339-020-04172-3

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