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Visualize the Spatial Organization of Charge and Spin Stripes by Resonant Micro X-ray Diffraction (RμXRD)

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Abstract

The interplay between the charge-density wave (CDW), the spin-density wave (SDW), and the defect ordering in complex materials is under an intense discussion. There is a strong interest in how the competition between these striped orders plays a role in the promotion of the material’s functionality at the macroscopic scale. Up to now, only few works point the attention to the direct visualization of how SDW, CDW, and defects are organized in the materials. Here, we propose the use of an innovative technique that combines the sensitivity of resonant X-ray scattering (SXR) with the spatial resolution of scanning micro X-ray diffraction (μXRD), allowing the investigation of the spatial organization of the resonant magnetic and charge order. Recent results on nickelates, cobaltites, and cuprates demonstrate the presence of a nanoscale phase separation scenario where these multiple striped orders get self-organized and form competing granular networks of nanodomains.

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References

  1. Ghiringhelli, G., et al.: Long-range incommensurate charge fluctuations in (Y,Nd)Ba2Cu3O6 + x. Science 337, 821–825 (2012)

    Article  ADS  Google Scholar 

  2. Chang, J., et al.: Direct observation of competition between superconductivity and charge density wave order in YBa2cu3o6.67. Nat. Phys. 8, 871–876 (2012)

    Article  Google Scholar 

  3. Wu, H.H., et al.: Charge stripe order near the surface of 12-percent doped La2 -xSrxCuO4. Nat. Commun. 3, 1023 + (2012)

    Article  ADS  Google Scholar 

  4. Bianconi, A.: Quantum materials: Shape resonances in superstripes. Nat. Phys. 9, 536–537 (2013)

    Article  MathSciNet  Google Scholar 

  5. Komarek, A.C., et al.: Dimerization and charge order in hollandite K2V8O16. Phys. Rev. Lett. 107 (2011)

  6. Komarek, A.C., et al.: Magnetic order, transport and infrared optical properties in the ACro3 system (A = Ca, Sr, and Pb). Phys. Rev. B 84 (2011)

  7. Shuvaev, A., et al.: Electric field control of terahertz polarization in a multiferroic manganite with electromagnons. Phys. Rev. Lett. 111 (2013)

  8. Komarek, A.C., et al.: Strong magnetoelastic coupling in VOCl: Neutron and synchrotron powder x-ray diffraction study. Phys. Rev. B 79 (2009)

  9. Kuo, C.Y., et al.: k =0 magnetic structure and absence of ferroelectricity in SmFeO3, magnetic structure and absence of ferroelectricity in SmFeO3. Phys. Rev. Lett. 113 (2014)

  10. Imada, M., Fujimori, A., Tokura, Y.: Metal-insulator transitions. Rev. Mod. Phys. 70, 1039–1263 (1998)

    Article  ADS  Google Scholar 

  11. Dagotto, E.: Complexity in strongly correlated electronic systems. Science 309, 257–262 (2005)

    Article  ADS  Google Scholar 

  12. Drees, Y., Lamago, D., Piovano, A., Komarek, A.C.: Hour-glass magnetic spectrum in a stripeless insulating transition metal oxide. Nat. Commun. 4 (2013)

  13. Drees, Y., et al.: Hour-glass magnetic excitations induced by nanoscopic phase separation in cobalt oxides. Nat. Commun. 5, 5731 + (2014)

    Article  ADS  Google Scholar 

  14. Guo, H., et al.: Charge correlations in cobaltates La2-xSrxCoO4. Phys. Status Solidi RRL (2015)

  15. Becker, T., et al.: Intrinsic inhomogeneities in manganite thin films investigated with scanning tunneling spectroscopy. Phys. Rev. Lett. 89 (2002)

  16. Bianconi, A., et al.: The measurement of the polaron size in the metallic phase of cuprate superconductors. Europhys. Lett. (EPL) 31, 411–415 (1995)

    Article  ADS  Google Scholar 

  17. Lanzara, A., et al.: Evidence for onset of charge density wave in the La-based perovskite superconductors. J. Supercond. Nov. Magn. 10, 319–321 (1997)

    Article  ADS  Google Scholar 

  18. Ricci, A.: Nanoscale dynamics in complex materials by resonant X-ray photon correlation spectroscopy (rXPCS). J. Supercond. Nov. Magn. 28, 1295–1298 (2015)

    Google Scholar 

  19. Fratini, M., et al.: Scale-free structural organization of oxygen interstitials in La2CuO4 + y. Nature 466, 841–844 (2010)

    Article  ADS  Google Scholar 

  20. Campi, G., et al.: Inhomogeneity of charge-density-wave order and quenched disorder in a high-Tc superconductor. Nature 525, 359–362 (2015)

    Article  ADS  Google Scholar 

  21. Poccia, N., et al.: Evolution and control of oxygen order in a cuprate superconductor. Nat. Mater. 10, 733–736 (2011)

    Article  ADS  Google Scholar 

  22. Poccia, N., et al.: Percolative superconductivity in La2CuO4.06 by lattice granularity patterns with scanning micro x-ray absorption near edge structure. Appl. Phys. Lett. 104, 221903 + (2014)

    Article  ADS  Google Scholar 

  23. Poccia, N.A., et al.: Size evolution of the oxygen interstitial nanowires in La2CuO4 + y by thermal treatments and x-ray continuous illumination. Supercond. Sci. Technol. 25, 124004 + (2012)

    Article  ADS  Google Scholar 

  24. Poccia, N., et al.: Spatial inhomogeneity and planar symmetry breaking of the lattice incommensurate supermodulation in the high-temperature superconductor Bi2Sr2CaCu2O8 + y. Phys. Rev. B 84, 100504 + (2011)

    Article  ADS  Google Scholar 

  25. Ricci, A., et al.: Nanoscale phase separation in the iron chalcogenide superconductor K0.8Fe1.6Se2 as seen via scanning nanofocused x-ray diffraction. Phys. Rev. B 84, 060511 + (2011)

    Article  ADS  Google Scholar 

  26. Ricci, A., et al.: Direct observation of nanoscale interface phase in the superconducting chalcogenide KxFe2-ySe2 with intrinsic phase separation. Phys. Rev. B 91 (2015)

  27. Ricci, A.: Supercond. Sci. Technol. 24, 082002 + (2011)

    Article  ADS  Google Scholar 

  28. Innocenti, D., et al.: J. Supercond. Nov. Magn. 22, 529 (2009). ISSN 1557-1939

    Article  Google Scholar 

  29. Campi, G., et al.: Scanning micro-x-ray diffraction unveils the distribution of oxygen chain nanoscale puddles in YBa2Cu3O6.33. Phys. Rev. B 87, 014517 + (2013)

    Article  ADS  Google Scholar 

  30. Ricci, A., et al.: Multiscale distribution of oxygen puddles in 1/8 doped YBa2Cu3O6.67. Sci. Rep. 3, 2383 + (2013)

    Article  ADS  Google Scholar 

  31. Ricci, A., et al.: Networks of superconducting nano-puddles in 1/8 doped YBa2Cu3O6.5+y controlled by thermal manipulation. New J. Phys. 16, 053030 + (2014)

    Article  ADS  Google Scholar 

  32. Poccia, N., et al.: Optimum inhomogeneity of local lattice distortions in La2CuO4 + y. Proc. Natl. Acad. Sci. 109, 15685–15690 (2012)

    Article  ADS  Google Scholar 

  33. Poccia, N., Ricci, A., Bianconi, A.: Misfit strain in superlattices controlling the electron-lattice interaction via microstrain in active layers. Adv. Condens. Matter Phys. 2010, 1–7 (2010)

    Article  Google Scholar 

  34. Ricci, A., Fratini, M., Bianconi, A.: The tetragonal to orthorhombic structural phase transition in multiband FeAs-based superconductors. J. Supercond. Nov. Magn. 22, 305–308 (2009)

    Article  Google Scholar 

  35. Ricci, A., Poccia, N., Ciasca, G., Fratini, M., Bianconi, A.: The microstrain-doping phase diagram of the iron pnictides: heterostructures at atomic limit. J. Supercond. Nov. Magn. 22, 589–593 (2009)

    Article  Google Scholar 

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Ricci, A. Visualize the Spatial Organization of Charge and Spin Stripes by Resonant Micro X-ray Diffraction (RμXRD). J Supercond Nov Magn 29, 633–636 (2016). https://doi.org/10.1007/s10948-016-3425-2

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  • DOI: https://doi.org/10.1007/s10948-016-3425-2

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