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Influence of order–disorder effects on the optical parameters of Ag7(Si1−xGex)S5I-mixed crystals

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Abstract

The temperature behavior of fundamental absorption edge for Ag7(Si1−xGex)S5I (x = 0, 0.2, 0.4, 0.6, 0.8, 1) mixed crystals was studied in the temperature range 77–300 K. The temperature dependences of the optical pseudogap Eg* and the Urbach energy EU were analyzed in the framework of Einstein model. Monotonous non-linear decrease of Eg* and EU values in the process of Si+ 4→Ge+ 4 cationic substitution was established. The parameters of electron–phonon interaction σ, which results in the Urbach behavior of the fundamental absorption edge, were determined. The increase in temperature leads to the electron–phonon interaction weakening, which agrees well with the Dow–Redfield model. The monotonous Urbach energy increase and a similar optical pseudogap decrease indicate the absence of phase transitions within the studied temperature range. The temperature and structural disordering influence on the optical absorption in Ag7(Si1−xGex)S5I-mixed crystals were discussed. The Urbach energy in Ag7(Si1−xGex)S5I-mixed crystals is shown to be determined by the effect of the temperature related, structural, and compositional disordering.

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Acknowledgements

The authors would also thank the Armed Forces of Ukraine for providing security to perform this work. This work has become possible only because resilience and courage of the Ukrainian Army.

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Authors and Affiliations

  1. Uzhhorod National University, Pidhirna Str. 46, 88000, Uzhhorod, Ukraine

    A. I. Pogodin, M. M. Pop, I. A. Shender, I. P. Studenyak, M. J. Filep, T. O. Malakhovska, O. P. Kokhan, T. Y. Babuka & L. M. Suslikov

  2. Institute of Information Registration, National Academy of Sciences of Ukraine, Zamkovi Shody Street, 88000, Uzhhorod, Ukraine

    M. M. Pop & V. M. Rubish

  3. Ferenc Rákóczi II Transcarpathian Hungarian College of Higher Education, Kossuth Sq. 6, 90200, Beregovo, Ukraine

    M. J. Filep

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  1. A. I. Pogodin
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Contributions

All authors contributed to the study conception and design. Material preparation, data collection, and analysis were performed by AP, MP, IS, IS, MF, TM, OK, TB, LS, and VR. The first draft of the manuscript was written by MP and all authors commented on previous versions of the manuscript. All authors read and approved the final manuscript.

Credit author statement: Supervision, Visualization, Investigation, and Writing of the original draft: AP; Visualization, Investigation, and Writing of the original draft: MP; Visualization and Investigation: IS; Supervision: IS; Data curation, Visualization, and Writing of the original draft: MF; Software and Validation: TM; Conceptualization and Methodology: OK; Investigation, Software, and Validation: TB; Writing, reviewing, & editing of the manuscript: LS; Validation and Data Curation: VR.

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Correspondence to A. I. Pogodin.

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Pogodin, A.I., Pop, M.M., Shender, I.A. et al. Influence of order–disorder effects on the optical parameters of Ag7(Si1−xGex)S5I-mixed crystals. J Mater Sci: Mater Electron 33, 15054–15066 (2022). https://doi.org/10.1007/s10854-022-08422-3

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  • DOI: https://doi.org/10.1007/s10854-022-08422-3

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