Abstract
A new low temperature cofired ceramic (LTCC) tape based on 40 wt% Al2O3–60 wt% LABS glass (40Li2CO3:10Al2O3:30B2O3:20SiO2) has been developed. The dielectric properties of the LABS glass are studied. The structural, dielectric, thermal as well as the chemical compatibility with Ag electrode of the bulk Al2O3–LABS sintered at 800 °C are investigated .The room temperature thermal conductivity and CTE of the bulk are 3.80 Wm−1 K−1 and 5.1 ppm/°C respectively. The Al2O3–LABS slurry which has a pseudoplastic nature is made into thin sheets using tape casting technique. The green tape has a surface roughness of 293 nm and tensile strength 0.2 MPa. The Al2O3–LABS based LTCC tapes are sintered at 775 °C has εr of 4.70 with tanδ 0.005 and τε of +412 ppm/°C at 5 GHz. The results suggest that the Al2O3–LABS based LTCC tapes is a possible candidate for LTCC device applications.
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K. Malecha, T. Maeder, C. Jacq, J. Eur. Ceram. Soc. 32, 3277 (2012)
S. Duan, E. Li, H. Chen, B. Tang, Y. Yuan, X. Zho, J. Mater. Sci. 26, 8819 (2016)
U. Ullah, M.F. Ain, N.M. Mahyuddin, M. Othman, Z.A. Ahmad, M.Z. Abdullah, A. Marzuki, IEEE Antennas Propag. Mag. 57, 241 (2015).
J.J. Bian, J.Y. Wu, J. Am. Ceram. Soc. 95, 318 (2012)
M.T. Sebastian, H. Jantunen, Int. Mater. Rev. 53, 57 (2008)
D. Chen, Y. Liu, Y. Li, W. Zhong, H. Zhang, J. Magn. Magn. Mater. 324, 449 (2012)
V. Vinothini, P. Singh, M. Balasubramanian, in Proceedings of International Symposium of Research Students on Material Science and Engineering, Chennai, 20–22 2004
P. Vozdecky, A. Roosen, C. Knieke, W. Peukert, J. Am. Ceram. Soc. 93, 1313 (2010)
N.P. Prasanth, J.M. Varghese, K. Prasad, B. Krishnan, A. Seema, K.R. Dayas, J. Mater. Sci. 19, 1100 (2008)
J.H. Feng, F. Dogan, J. Am. Ceram. Soc. 83, 1681 (2000)
K. Kumari, G.V. Sasidharan, K.M. Sapna, R. Natarajan, Bull. Mater. Sci. 28,103 (2005)
R.E. Mistler, E.R. Twiname, Tape Casting Theory and Practice (The American Ceramic Society, Westerville, 2000)
R. Moreno, Am. Ceram. Soc. Bull. 71, 1647 (1992)
L. Ren, Y.P. Zeng, D. Jiang, Int. J. Appl. Ceram. Technol. 5, 505 (2008)
Z. Jingxian, J. Dongliang, L. Weisensel, P. Greil, J. Eur. Ceram. Soc. 24, 147 (2004)
S.A. Uhland, R.K. Holman, S. Morissette, M.J. Cima, E.M. Sachs, J. Am. Ceram. Soc. 84, 2809 (2001)
C. Berry, D. Parlow, T. Vasilow, S. Gurkovich, A. Bailey, in Proceedings on International Symposium on Microelectronics, IMAPS, Boston, 150 2000
M. Liu, H. Zhou, X. Xu, Z. Yue, M. Liu, H. Zhu, J. Mater. Sci. 24, 3985 (2013)
Y.H. Jo, M.S. Kang, K.W. Chung, Y.S. Cho, Mater. Res. Bull. 43, 361 (2008)
S. Rajesh, H. Jantunen, M. Letz, S. Willhelm, Int. J Appl. Ceram. Technol. 9, 52 (2011)
M.T. Sebastian, in Dielectric materials for wireless communication (Elsevier, Oxford, 2008)
D. Zeng, J. Xu, Y. Chen, W. Chen, Y. Yu, H. Wang, R. Zeng, Int. J. Appl. Ceram. Technol. 12, 112 (2015)
B. Li, Y. Xu, S. Zhang, Glass Phys. Chem. 41, 503 (2015).
E. Li, Y. Shi, C. Sun, Y. Zhao, S. Zhang, J. Mater. Sci. 27, 6592 (2016)
N. Monmaturapoj, P. Lawita, W. Thepsuwan, Adv. Mater. Sci. Eng. 2013, 1 (2013)
A. Arvind, R. Kumar, M.N. Deo, V.K. Shrikhande, G.P. Kothiyal, Ceram. Int. 35, 1661 (2009)
Y.J. Choi, J.H. Park, W.J. Ko, J.H. Park, S. Nahm, J.G. Park, J. Electroceram. 14, 157 (2005)
S. Hyeok, D.H. Kim, Y. La, H. Kim, N.J. Hwang, J. Cha, B.K. Ryu, Electron. Mater. Lett. 6, 71 (2010)
V.O. Soares, O. Peitl, E.D. Zanotto, J. Am. Ceram. Soc. 96, 1143 (2013)
B. Li, Z. Qing, Y. Li, H. Li, S. Zhang, J. Electroceram. 37, 145 (2016)
A. Prasad, A. Basu, J. Mater. Sci. 24, 1855 (2013)
R. Brown, in RF/Microwave hybrids (Kluwer Academic Publishers, Dordrecht, 2004)
J.M. Wu, H.L. Huang, J. Non-Cryst. Solids 260, 116 (1999)
L. He, G. Xia, D. Yang, J. Alloys Compd. 556, 12 (2013)
C. Xiaoge, T. An, Z. Hongsong, L. Yanxu, Z. Haoming, Z. Yongde, Ceram. Int. 42, 13491 (2016)
M. Dubey, N. Suri, P.K. Khanna, Int. J. Res. Eng. Tech. 2, 441 (2013)
W.K. Jones, Y. Liu, B. Larsen, P. Wang, M. Zampino, Int. J. Microcircuits Electron Package 23, 469 (2000)
R. Riedel, I. Chen, in Ceramics Science and Technology (Wiley VCH, Weinheim, Germany, 2013)
J.C. Whitaker, in The electronics handbook (Technical Press, Oregon, 1996)
N. Chantaramee, S. Tanaka, Z. Kato, N. Uchida, K. Uematsu, J. Eur. Ceram. Soc. 29, 943 (2009)
I.J. Induja, P. Abhilash, S. Arun, K.P. Surendran, M.T. Sebastian, Ceram. Int. 41, 13572 (2015)
Acknowledgements
Induja. I. J is grateful to the Kerala State Council for Science, Technology and Environment (KSCSTE) Kerala, India for the award of Research Fellowship. The authors are grateful to Dr. K. P. Surendran for the constant support. Dr. P. Prabhakar Rao, Mrs. Soumya for extending the SEM facility, A. Peer Mohammed for rheology and surface area measurements, Dr. Yoosaf and Mr. Aswin Maheswar for AFM and Mr. M. Brahmakumar for tensile measurements.
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Induja, I.J., Varma, M.R. & Sebastian, M.T. Preparation, characterization and properties of alumina-lithium aluminium borosilicate glass based LTCC tapes. J Mater Sci: Mater Electron 28, 14655–14663 (2017). https://doi.org/10.1007/s10854-017-7330-7
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DOI: https://doi.org/10.1007/s10854-017-7330-7