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Metal organic framework (MOF)–derived iron oxide@nitrogen–doped carbon nanocomposites as anode materials for lithium-ion batteries

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Abstract

Iron oxide (Fe2O3) has shown great potential to substitute carbon-based anode materials for lithium-ion batteries because of its high theoretical specific capacity. However, its huge volume change during the lithiation and de-lithiation processes has restricted its extensive application. Herein, we design a nitrogen-doped carbon-coated iron oxide (Fe2O3@NC) from Material of Institute Lavoisier (MIL)-53 (Fe) by a solvothermal method. Nitrogen-doped carbon can release the expansion stress of Fe2O3 to ensure the structural integrity and ameliorate electronic conductivity. Therefore, Fe2O3@NC displays a specific capacity of 875.4 mAh g−1 at 100 mA g−1 after 100 cycles and a good cycling stability of 342 mAh g−1 at a high rate of 500 mA g−1 in the best case.

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Funding

This work was financially supported by National Natural Science Foundation of China (No. 21701083) and Postgraduate Research & Practice Innovation Program of Jiangsu Province (Grant No. KYCX20_3137).

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Authors and Affiliations

  1. School of Energy and Power, Jiangsu University of Science and Technology, Zhenjiang, 212003, China

    Tao Wei, Yilie Zhao, Rentian Chen, Sijia Wang, Yanyan Zhou, Cheng Sun & Zidong Yu

  2. Institute of Mechanics and Energy, National Research Ogarev Mordovia State University, Saransk, 430000, Russia

    Yilie Zhao & Sergey Maltsev

  3. Power & Energy Storage System Research Center, College of Mechanical and Electrical Engineering, Qingdao University, Qingdao, 266071, China

    Xiangyun Qiu

  4. College of Chemical Engineering and Technology, Taiyuan University of Technology, Taiyuan, 030024, Shanxi Province, China

    Shoudong Xu

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  1. Tao Wei
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Wei, T., Zhao, Y., Chen, R. et al. Metal organic framework (MOF)–derived iron oxide@nitrogen–doped carbon nanocomposites as anode materials for lithium-ion batteries. Ionics 28, 4185–4194 (2022). https://doi.org/10.1007/s11581-022-04655-8

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