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Structure, thermal stability and dielectric properties of aluminoborosilicate glasses doped with Pr2O3

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Abstract

The structure, thermal stability and dielectric properties of aluminoborosilicate glasses with different contents of Pr2O3 were researched by XRD, FT-IR, DSC and electronic impedance analyzer. FT-IR results showed that the addition of Pr2O3 enhanced the degree of polymerization of glass network. The molar volume decreased at first and then increased, which reached the minimum value with the content of Pr2O3 up to 1.5 mol%. With the addition of Pr2O3 the glass transition temperature (Tg) showed an upward trend, while Dietzel's thermal stability (ΔT) and the Saad parameter (S) both increased initially to be followed by a decrease, which indicated that the thermal stability of glass can be improved by doping proper content of Pr2O3. The dielectric constant (εr) and dielectric loss (tanα) both decreased at first then started to go up as the content of Pr2O3 increased. When Pr2O3 content moved up to 0.5 mol% and 1.5 mol%, the εr and tanα reached the minimum values 4.68 and 3.13 × 10–4, respectively.

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Acknowledgements

This paper was funded by National Natural Science Foundation of China (Nos. 51872117, 51804131, 52072148 and 51672105), Natural Science Foundation of Shandong Province (No. ZR2019BEM002), and Opening Project of State Key Laboratory of Advanced Technology for Float Glass (No. 2020KF01)

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Author notes

  1. Jingang Zhao and Xiaokun Tian contributed equally to this work and should be considered as cofirst authors

Authors and Affiliations

  1. School of Materials Science and Engineering, University of Jinan, Jinan, 250000, China

    Jingang Zhao, Xiaokun Tian, Lulu Zhang, Ya Qu, Chao Wu, Yunlong Yue & Junfeng Kang

  2. State Key Laboratory for New Technology of Float Glass, 751 Donghai Dadao, Bengbu, 233000, China

    Fengyang Zhao

  3. Shandong Product Quality Inspection Research Institute, 31000 Jingshi East Road, Jinan, 250102, China

    Xianjing Chen

  4. Shandong Road New Materials Co., Ltd, Taian, 271000, China

    Xunmei Liang

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  1. Jingang Zhao
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Correspondence to Yunlong Yue or Junfeng Kang.

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Zhao, J., Tian, X., Zhang, L. et al. Structure, thermal stability and dielectric properties of aluminoborosilicate glasses doped with Pr2O3. J Mater Sci: Mater Electron 32, 24964–24970 (2021). https://doi.org/10.1007/s10854-021-06954-8

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