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Metal oxide ion-gated transistors: A perspective on in operando characterizations and emerging Li-ion-based applications

  • MRS 50th Anniversary Prospective
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Abstract

In this Prospective, we discuss how ionic media interfaced to metal oxide (MO) semiconducting thin films can modulate their electronic conductivity. From in situ diagnosis tools to monitor the state-of-health of Li-ion batteries, to synaptic transistors where ion diffusive dynamics governs short-term and long-term plasticity, technologies based on ionic medium/MO interfaces are emerging, strongly benefitting from advanced nanoscale resolved scanning probe techniques and computational chemistry.

Graphical abstract

Schematic representations of ion-gated transistors (IGT) making use of a metal oxide as semiconductor channel

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Acknowledgments

We acknowledge the financial support from Institut Trottier de l’Energie (‘‘In situ diagnosis tools for lithium ion batteries’’, appel à projets 2020). Luan P. Camargo and Lariel C. S. Neres would like to thank the Emerging Leaders of Americas Program (ELAP) Scholarship provided with the support of Global Affairs Canada and Coordenação de Aperfeiçoamento de Pessoal de Nível Superior (CAPES—Brazil) for the Doctorate Scholarship (Edital 44/2022-PROPG). José R. Herrera Garza thanks the National Council for the Humanities, Sciences and Technologies (CONAHCYT), Grant 739478. Francesca Soavi thanks the Italian MUR (Fondi PNRR-CNMS-Spoke 13-MOST Code: CN00000023) for financial support. Also, we thankfully acknowledge Professor Ph.D. Luiz Henrique Dall’Antonia (State University of Londrina, Londrina—Brazil) for the discussion regarding the metal oxide synthesis procedure.

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Authors and Affiliations

  1. Institute of Chemistry, State University of São Paulo (UNESP), Araraquara, SP, 14801-970, Brazil

    Lariel Chagas da Silva Neres

  2. Engineering Physics Department, Polytechnique Montreal, Montreal, QC, H3C 3A7, Canada

    Lariel Chagas da Silva Neres, Luan Pereira Camargo, Ramin Karimi Azari, José Ramón Herrera Garza & Clara Santato

  3. Chemistry Department, CCE, State University of Londrina (UEL), Londrina, PR, 86057-970, Brazil

    Luan Pereira Camargo

  4. Department of Chemistry “Giacomo Ciamician”, Alma Mater Studiorum Universitá di Bologna, Via Selmi 2, 40126, Bologna, Italy

    Francesca Soavi

  5. Institute of Chemistry, Federal University of Goias (UFG), Av. Esperança, s/n—Chácaras de Recreio Samambaia, Goiânia, GO, 74690-900, Brazil

    Martin Schwellberger Barbosa

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  1. Lariel Chagas da Silva Neres
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da Silva Neres, L.C., Camargo, L.P., Azari, R.K. et al. Metal oxide ion-gated transistors: A perspective on in operando characterizations and emerging Li-ion-based applications. MRS Communications 13, 695–703 (2023). https://doi.org/10.1557/s43579-023-00437-z

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