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Free-energy landscapes of granular clusters grown by magnetic interaction

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Abstract.

We experimentally study the aggregation of small clusters made of non-Brownian dipolar beads in a vibro-fluidized system. The particles are paramagnetic spheres that add around a fixed magnetic seed inside a granular gas of glass beads. We observe that under appropriate physical conditions symmetric and asymmetric cluster configurations are created and, as the number of particles increases, the aggregation time obeys a power law. We use an ensemble statistics to evaluate the free-energies and entropies landscapes of the granular clusters. The correspondence between such landscapes shows that, even if the system is of macroscopic scale and not in strict equilibrium, our approach to understand the relationship between the cluster structures and the interactions that create them is reliable.

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References

  1. M. Volmer, A. Weber, Z. Phys. Chem. 119, 277 (1926)

    Google Scholar 

  2. R. Becker, W. Doring, Ann. Phys. 24, 719 (1935)

    Article  MATH  Google Scholar 

  3. T.A. Witten Jr., L.M. Sander, Phys. Rev. Lett. 47, 1400-3 (1981)

    Article  ADS  Google Scholar 

  4. D. Turnbull, J.C. Fisher, J. Chem. Phys. 17, 71 (1949)

    Article  ADS  Google Scholar 

  5. A.S. Myerson, The structure of supersaturated solutions (North-Holland, Amsterdam, 1993)

  6. J.M. Garcia-Ruiz, J. Struct. Biol. 42, 22 (2003)

    Article  Google Scholar 

  7. R. Patel, B. Chudasama, Phys. Rev. E 80, 012401 (2009)

    Article  ADS  Google Scholar 

  8. C. Bustamante, J. Liphardt, F. Ritort, arXiv 0511629 (2005)

  9. D.J. Evans, D.J. Searles, Phys. Rev. E 50, 1645 (1994)

    Article  ADS  Google Scholar 

  10. S.F. Edwards, R.B.S. Oakeshott, Physica A 157, 1080 (1988)

    Article  MathSciNet  ADS  Google Scholar 

  11. R. Blumenfeld, S.F. Edwards, Phys. Rev. Lett. 90, 114303 (2003)

    Article  ADS  Google Scholar 

  12. G. Meng, N. Arkus, M.P. Brenner, V.N. Manoharan, Science 327, 560 (2010)

    Article  ADS  Google Scholar 

  13. P.G. de Gennes, P.A. Pincus, Phys. Kondens. Materie 11, 189 (1970)

    ADS  Google Scholar 

  14. M.G. Clerc, P. Cordero, J. Dunstan, K. Huff, N. Mujica, D. Risso, G. Varas, Nat. Phys. 4, 249 (2008)

    Article  Google Scholar 

  15. H.M. Jaeger, S.R. Nagel, R.P. Behringer, Rev. Mod. Phys. 68, 1259 (1996)

    Article  ADS  Google Scholar 

  16. W. Losert, D.G.W. Cooper, J.P. Gollub, Phys. Rev. E 59, 5855 (1999)

    Article  ADS  Google Scholar 

  17. M.V. Sapozhnikov, I.S. Aranson, J.S. Olafsen, Phys. Rev. E 67, 010302(R) (2003)

    Article  ADS  Google Scholar 

  18. A. Prevost, P. Melby, D.A. Egolf, J.S. Urbach, Phys. Rev. E 70, 050301(R) (2004)

    Article  ADS  Google Scholar 

  19. A. Götzendorfer, J. Kreft, C.A. Kruelle, I. Rehberg, Phys. Rev. Lett. 95, 135704 (2005)

    Article  ADS  Google Scholar 

  20. D.A. Egolf, Science 287, 101 (2000)

    Article  ADS  Google Scholar 

  21. I.S. Aranson, L.S. Tsimring, Rev. Mod. Phys. 78, 641 (2006)

    Article  ADS  Google Scholar 

  22. H.S. Leff, Am. J. Phys. 67, 1114 (1999)

    Article  MATH  MathSciNet  ADS  Google Scholar 

  23. A. Ben-Naim, Entropy Demystified, the Second Law Reduced to Plain Common Sense (World Scientific, Singapore, 2007)

  24. C. Shannon, Bell System Tech. J. 27, 379 (1948)

    Article  MATH  MathSciNet  Google Scholar 

  25. S. Ogawa, A. Umemura, N. Oshima, J. Appl. Math. Phys. 31, 483 (1980)

    Article  MATH  Google Scholar 

  26. D.L. Blair, A. Kudrolli, Phys. Rev. E 67, 021302 (2003)

    Article  ADS  Google Scholar 

  27. A. Ben-Naim, A farewell to entropy: statistical thermodynamics based on information (World Scientific, Singapore, 2008)

  28. O. Carvente, G.G. Peraza-Mues, J.M. Salazar, J.C. Ruiz-Suárez, Granular Matter 14, 303 (2012)

    Article  Google Scholar 

  29. G.J. Gao, J. Blawzdziewicz, C.S. O'Hern, Phys. Rev. E 74, 061304 (2006)

    Article  ADS  Google Scholar 

  30. C. Briscoe, C. Song, P. Wang, H.A. Makse, Phys. Rev. Lett. 101, 1881001 (2008)

    Article  Google Scholar 

  31. G.J. Gao, J. Blawzdziewicz, C.S. O'Hern, M. Shattuck, Phy. Rev. E 80, 061304 (2009)

    Article  ADS  Google Scholar 

  32. K. Wang, C. Song, P. Wang, H.A. Makse, EPL 91, 68001 (2010)

    Article  ADS  Google Scholar 

  33. J.E. Martin, R.A. Anderson, R.L. Williamson, J. Chem. Phys. 118, 1557 (2003)

    Article  ADS  Google Scholar 

  34. C.L. Klix, K.-i. Murata, H. Tanaka, S.R. Williams, A. Malins, C.P. Royall, Sci. Rep. 3, 2072 (2013)

    Article  ADS  Google Scholar 

  35. I.G. Main, F.H. Al-Kindy, Geophys. Res. Lett. 29, 1121 (2002)

    Article  ADS  Google Scholar 

  36. D. Aleksandar, F.H. Stillinger, S. Torquato, J. Chem. Phys. 127, 124 (2007)

    Google Scholar 

  37. A.J. Doig, M.J.E. Sternberg, Protein Sci. 4, 2247 (1995)

    Article  Google Scholar 

  38. O. Carvente, J.C. Ruiz-Suárez, Phys. Rev. E 78, 011302 (2008)

    Article  ADS  Google Scholar 

  39. G. Lumay, N. Vandewalle, New J. Phys. 9, 406 (2007)

    Article  ADS  Google Scholar 

Download references

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Correspondence to J. C. Ruiz-Suárez.

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González-Gutiérrez, J., Carrillo-Estrada, J.L., Carvente, O. et al. Free-energy landscapes of granular clusters grown by magnetic interaction. Eur. Phys. J. E 37, 37 (2014). https://doi.org/10.1140/epje/i2014-14037-x

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  • DOI: https://doi.org/10.1140/epje/i2014-14037-x

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