Abstract
The purpose of this paper is to show that, by combining Feshbach resonances with external confining potentials, the energy scale factor of neighboring Efimov states can be tremendously reduced. The Efimov conditions can be reached for systems made of three different particles. For the case of two identical light particles and a heavy particle, the energy factor can be reduced by many orders of magnitude, and the Efimov states are in this way more easily reachable experimentally. The equivalence between external potentials and the formulation in terms of non-integer dimensions, d, is exploited. The technically simpler d-method is used to derive analytic expressions for two-component relative wave functions describing two short-range square-well interacting particles. The two components express one open and one closed channel. The scattering length is obtained after phase shift expansion, providing an analytic form for the Efimov condition. We illustrate the results by means of systems made of \(^7\)Li, \(^{39}\)K, and \(^{87}\)Rb, with realistic parameters. The related pairs of dimension and magnetic field are shown and discussed. The results are universal as they only rely on large-distance properties.
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1 Introduction
The ability to induce the population of a Feshbach resonance by means of a static magnetic field [1, 2] amounts in practice to the possibility of tuning the atom-atom interaction, and, for instance, control the scattering length of the corresponding two-body potential. This fact opened the door to the investigation of three-body systems where at least one of the internal two-body interactions, in particular, can be tuned to have an infinite scattering length. In this way conditions for the appearance of the Efimov effect [3] can be satisfied for systems containing three particles. The case of the Cesium trimers [4] or the Li-Cs-Cs system [5] are good examples of this.
More recently, in Ref. [6], it has been shown that the Efimov effect can also be induced by an external field that confines the system. This is based on the fact that, in three dimensions, an attractive potential might not bind a two-body system, but in two dimensions the two-body system will always be bound. As a consequence, if a two-body system is not bound in three dimensions, during the confinement process to two dimensions, there must necessarily be a moment where the two-body binding energy is equal to zero, or, in other words, the two-body scattering length is equal to infinity. Under these conditions, a three-body system made of two or three identical particles would as well fulfill the Efimov conditions.
An efficient way to describe the confinement by means of an external field is the d-method recently presented in Ref. [7]. The idea behind the method is to introduce a continuous dimension d, such that the d-dependent centrifugal barrier accounts for the effect of the external field, which does not enter explicitly in the calculation. The confinement induced Efimov effect was introduced in [8], although the continuous variation of the squeezing is not investigated.
An external potential along one axis constrains the particles to move only within a limited volume. The two extremes would be a spherical shape and a pancake corresponding respectively to dimensions \(d=3\) and \(d=2\). The equivalence to a dimension-dependent centrifugal barrier has been demonstrated in Refs. [9, 10], where the two limits, \(d=2,3\), are rigorously proved. The d-wave function is then interpreted in the ordinary three-dimensional space as a wave function deformed along the confinement axis. In particular, when the Efimov states are present, they must then be elongated following the deformed external field, i.e., perpendicularly to the squeezing direction.
The equivalence between a non-integer dimension d and the length, \(b_{ho}\), of an external harmonic oscillator squeezing potential can be found in [9] for two-body systems. For three-body systems with identical particles, assuming harmonic oscillator particle-particle interactions with harmonic oscillator length \(r_0\), the connection between d and \(b_{ho}\) was derived to be [10]
where \(r_\textrm{2D}\) is the rms radius of the three-body system in two dimensions with the realistic interactions.
The “d vs. \(b_{ho}/r_\textrm{2D}\)” curve in Eq. (1) is to a large extent universal, valid not only for particle-particle harmonic oscillator potentials in the three-body system. This is shown in Ref. [10], where the cases of Gaussian and Morse potentials are considered. When different species are involved, the intermediate d-values may correspond to different external fields. However, still correct in both limits, Eq. (1) must be semi-quantitatively, or at least qualitatively, correct for all d in the interval, \(2<d<3\). In any case fine tuning would probably be necessary for any specific experiment.
The confinement length, \(b_{ho}\), is related to the harmonic frequency, \(\omega \), by the relation \(\omega =\hbar /(m b_{ho}^2)\), where m is the mass of the atom. The currently available confinement frequencies move in the range of hundreds of Hz, which for a medium size atom implies that \(b_{ho}/r_0\) should even approach 1000. This value amounts to a very weak confinement, since, as we can see from Eq. (1), for \(b_{ho}/r_0\approx 1000\) we get \(d\approx 2.999999\), extremely close to 3. Note that, for instance, for \(d=2.9\) we have \(b_{ho}/r_0 \approx 3.1\). This leads to \(\omega \) in the range of tens of MHz, which in principle is nowadays out of experimental reach.
The critical dimension, \(d=d_E\), for which the two-body potential has infinite scattering length describes the confinement scenario at which the corresponding two-body state has zero energy. When this happens for two of the three subsystems a series of infinitely many three-body bound states appears, where ratios of energy and size of neighboring states are constant throughout the series. This is the hallmark of appearance of the Efimov effect. The properties and behavior of the Efimov states for arbitrary d, and how they appear and disappear in the vicinity of \(d=d_E\) are investigated in [6, 11]. Under these conditions the details of the short-distance two-body potentials play a very minor role, and the physics has therefore a universal character. For this reason, much of the physics can then be captured with simple potentials which could even provide analytic solutions. The universal connection between scattering length, magnetic field strength, and the measured molecular binding energy is derived analytically in Ref. [12] for \(d=3\). Here a two-channel model using finite-range square-well potentials avoids the zero-range singularity seen in Ref. [13]. These detailed relations are successfully tested in the experimentally known case of cesium molecules. The strong variations around the Feshbach resonance positions are very well reproduced.
The purpose of this work is to use a similar two-channel model with square-well potentials, but in d dimensions. The goal is to study, for a general, not necessarily integer, dimension d, the behavior of the scattering length under the presence of a static magnetic field. We are therefore using the d-method as theoretical framework. The model incorporates simultaneously the two different procedures to modify the effective two-body scattering length, the dimension d (or the confinement parameter) and the magnetic field. The presence of these two parameters will allow to tune simultaneously the scattering length for two different two-body systems. In this way it could then be possible to simultaneously tune the two interactions involved in a three-body system containing two identical particles, or even induce the Efimov effect in three-body systems with three different constituents. The connection to specific experiments is not in focus in the present paper. Although the results are overall applicable, direct experimental comparison needs detailed consideration.
The paper is organized as follows. We derive in Sect. 2 the analytical solution of the Schrödinger equation for the two-component problem (one open channel and one closed channel) in d dimensions and square-well potentials. Making use of the derived wave functions, we, in Sect. 3, provide expressions for the two-component scattering length and effective range. The behavior of the scattering length as a function of the dimension and external magnetic field is investigated in Sect. 4, where we focus on the condition such that the scattering length is infinite.
The possibility of tuning the two-body scattering length by means of both the dimension and the magnetic field is now exploited to investigate three-body systems and the simultaneous tuning of two of the internal two-body potentials. In Sect. 5 we discuss the most convenient systems to be investigated when two of the three constituents are identical and when all the three are different. The specific cases of the \(^{87}\)Rb-\(^7\)Li-\(^7\)Li and \(^7\)Li-\(^{39}\)K-\(^{87}\)Rb trimers are considered in Sects. 6 and 7, respectively. For each of them we determine the dimension d (related to the length of the squeezing harmonic oscillator potential through Eq. (1)) and the magnetic field that gives rise to the appearance of the Efimov effect on these systems, and such that the energy scale factor is relatively small. We finish in Sect. 8 with a summary and the conclusions. Finally, a number of mathematical derivations are collected in appendices.
2 Formulation
We consider a two-body system where only two channels, the ground state and one excited state, contribute to its wave function. We assume that the energy of the system, E, is below the excitation threshold, \(E^*\), and refer to the ground state and the excited state channels as open and closed channels, respectively.
The open and closed potentials are pictured in Fig. 1 for the case of square-well potentials with radius \(R_0\). The open and closed channels are coupled through a short-range coupling potential. The effect of the direct scattering process in the open channel, without coupling to any closed channel, gives rise to the background part of the two-body scattering length [14], usually denoted as \(a_{\textrm{bg}}\).
Below, we derive the analytic expressions for the wave functions and phase shifts of the scattering process assuming a relative s-wave state, square-well two-body interactions, and a general, not necessarily integer, dimension d.
2.1 Equations of motion
The reduced coupled radial Schrödinger equations describing the relative motion in a two-body system with relative energy E, and where only one open and one closed channels contribute, are given by:
where \(u_c\) and \(u_o\) are the two components describing the closed and open channels, respectively, related to the total wave function, \(\Psi \), by
In Eqs. (2) and (3) r is the relative coordinate, \(\mu \) is the reduced mass, \(V_c(r)\), \(V_o(r)\) and \(V_{oc}(r)= V_{co}(r)\) are the diagonal (closed and open) and coupling potentials, E is the energy of the system, and \(E^*\) is the excitation energy from the ground to the excited state. The generalized s-wave angular momentum, \(\ell \), for two particles depends on the dimension, d, and is given by [6, 7, 9, 10, 15]
such that the centrifugal barrier strength,
is zero for \(d=3\) and \(d=1\) and negative and equal to \(-1/4\) for \(d=2\).
In this work we shall assume that all the interactions, V(r), are spherical square-well potentials of the same radius, \(R_0\), that is of the form (see Fig. 1):
where \(V_0 (>0)\) represents the different strengths of \(V_c(r)\), \(V_o(r)\), and \(V_{oc}(r)= V_{co}(r)\), that we will denote, respectively, as \(V_c\), \(V_o\), and \(V_{co}\).
By introducing the dimensionless coordinate, \(x=r/R_0\), and multiplying Eqs. (2) and (3) by \(-2\mu R^2_0/\hbar ^2\), the equations of motion become
where primes denote derivative with respect to x, and the matrix A is defined as
where
and where we have used the abbreviations
all of them positive, and
Note that with these definitions, \(a_+\), \(a_-\), \(S_c\), \(S_o\), \(a_{co}\), \(\kappa _o\), \(k_o\), and \(\kappa _c\), all are dimensionless quantities.
2.2 Solutions
The square-well potentials require solutions in the two regions, that is inside and outside the box. The equations outside the box, \(r>R_0 \; (x>1)\), decouple, since then \(V_c(r)=V_o(r)=V_{co}(r)=0\), and the matrix A is diagonal and given by
With \(A=A^\mathrm {(out)}\) in Eq. (8), the two-component solutions are explicitly for positive energy, \(E>0\),
where \(h_\ell ^{(+)}\) is the outgoing Hankel function of first kind, \(j_\ell \) and \(\eta _\ell \) are, respectively the regular and irregular spherical Bessel functions, and \(B_c\) and \(B_o\) are normalization constants. The wave function describing the closed channel falls off exponentially, and the wave function for the open channel oscillates for large distances. For a negative energy, \(E<0\), also \(u_o^\mathrm {(out)}\) must fall off exponentially, which corresponds to an imaginary \(k_{o}\) in Eq. (16).
The equations inside the box, \(r<R_0 \; (x<1)\), are coupled in Eq. (8) through the potentials in the non-diagonal general matrix A in Eq. (9). The procedure to find the solutions is to diagonalize this matrix, A. The coordinate-dependent centrifugal barrier terms are identical in the diagonal. This fortunately implies that the transformation matrix, U, is a constant independent of the coordinate, x. We define the resulting diagonal matrix, D, as:
formed by the eigenvalues of A, and where:
if \(a_+>a_-\), or interchange of the two eigenvalues in the opposite case of \(a_+<a_-\), i.e.,
These definitions are chosen such that \(D_{\pm }^2 \rightarrow a_{\pm }\) when \(a_{co} \rightarrow 0\), independent of the relative size of \(a_+\) and \(a_-\). With these definitions we also have that
The eigenvectors associated to the above eigenvalues permit to construct the transformation matrix, \(U=U^{-1}\), with normalized column vectors, as:
where the normalization is given by
The difference and sum of \(a_+\) and \(a_-\), which enter in the definitions of \(D_{\pm }\) in Eqs. (18) and (19), are given by
The diagonal problem:
leads to the uncoupled equations for \(\phi _{\pm }\):
whose solutions, regular at the origin, are
where \(C_{\pm }\) are normalization constants and \(j_\ell \) is the regular spherical Bessel function.
Combining now Eqs. (8) and (17) it is simple to see that:
which, by comparison to Eq. (27), immediately leads to:
which, by combination of Eqs. (23) and (29), permit to obtain the solutions inside the box:
where we have omitted the unimportant normalization constant N.
3 Scattering length and effective range
The matching of the logarithmic derivatives of the solutions inside and outside the box, i.e., the matching of Eqs. (15) and (32), and Eqs. (16) and (33), at \(x=1\) is described in Appendix A. This leaves to the following expression for the phase shift, Eq.(A8):
where \(F_2\) is given by Eq. (A9).
The phase shift can be expanded in powers of energy, resulting in the effective range expansion defining the scattering length and the effective range. The lowest order term is then obtained by expanding in energy up to first order in E, or second order in \(k_{o}\), and inserting energy zero (\(E=0\)) in all resulting terms. The exception is the overall energy factor arising from \(\eta _\ell (k_{o})\) and \(j_\ell (k_{o})\), which however also must be expanded to include the two lowest orders in energy.
For the sake of clarity, we give the details of the derivations in Appendix B, and here we only quote and discuss the final results.
3.1 Expanding the phase shift
After the low-energy expansion of all the terms in Eq. (34) we get that, Eq. (B26):
where for non-integer values of \(\ell \) the factor \((2\ell +1)!!\) has to be replaced by \(\Gamma (2\ell +2)/(2^\ell \Gamma (\ell +1))\), \(F_2^{(0)}\) is given by Eq. (B21), \(F_2^{\prime (0)}=\partial F_2^{(0)}/\partial E\), and the superscript (0), wherever it appears, refers from now on to the function evaluated at \(E=0\).
The above expression can be compared to
where \(a_\textrm{tw}\) and \(R_\textrm{eff}\) are the two-component scattering length and the effective range, respectively.
From Eq. (36), after comparison with Eq. (35), and keeping in mind that \(E= \hbar ^2 k_0^2/(2\mu R^2_0)\), we can identify:
If \(a_{co}=0\), \(a_\textrm{tw}=a_{\textrm{bg}}\), and Eq. (37) reduces to:
which is the expression of the scattering length for the square-well potential and an arbitrary relative partial wave, \(\ell \).
From Eqs. (35) and (36) we can also extract the effective range as shown in Appendix C.
3.2 Connection to open and closed channels
Equation (37) gives the two-component scattering length for square-well potentials. To make it more general, it is convenient to write it in terms of the scattering lengths for the closed and open channels, \(a_\textrm{closed}\) and \(a_\textrm{open}\). With this in mind, we define:
and
such that in the limit of no coupling, \(a_{co}=0\), we recover the known \({\ell }\)-dependent square-well expression, Eq. (38), and therefore \(a_\textrm{open}=a_{\textrm{bg}}\).
In the same way we define \(\tilde{\kappa }_c\) as:
which, for any \(\ell \), in the presence of a very weakly bound state becomes \(\tilde{\kappa }_c \rightarrow R_0/a_\textrm{closed}\).
Using these definitions, it is not difficult to write \(F_2^{(0)}\) in Eq. (B21) as a function of \(a_\textrm{closed}\), \(a_\textrm{open}\), and \(\tilde{\kappa }_c\), and get that the scattering length in Eq. (37) becomes:
When \(a_{co}\rightarrow 0\), an expansion of Eq. (42) up to first order in \(a_{co}^2\) permits to reduce the equation to:
where the parameter \(\beta ^2\) is just the numerator in the last term of Eq. (42), which contains \(a_{co}^2\) multiplied by a series of, either finite or small, factors.
By identifying \(\beta \) in Eq. (43) and the coupling parameter \(\beta \) employed in Ref. [13], we can see that Eq. (43) reduces trivially for three dimensions (\(\ell =0\)) to Eq. (7) of Ref. [13], where the two-component problem is investigated in three dimensions with a contact interaction model.
4 Critical dimension
Equation (42) gives the scattering length for the two-component problem in d dimensions, from which we write:
It is obvious that the two-component scattering length, \(a_\textrm{tw}\), becomes infinite when the denominator of the fraction in the expression above is equal to zero. After some rewriting, this condition can be written as:
Note that the quantities \(\tilde{\kappa }_c\) in Eq. (41), \(a_\textrm{closed}\) in Eq. (39), and \(a_\textrm{open}\) in Eq. (40), are, through \(\ell \) in Eq. (5), functions of the dimension d. We define the critical dimension, \(d=d_E\), as the value of d such that the equality in Eq. (45) is fulfilled. For this dimension we have that \(a_\textrm{tw}=\infty \), or, equivalently, the two-body two-component system has zero binding energy.
The momentum, \(\tilde{\kappa }_c\) in Eq. (41), is a function of d and \(\kappa _c^{(0)}\), which is given in Eq. (B13). Also, \(a_+^{(0)}\) in Eq. (B14), and therefore \(D_\pm ^{(0)}\) in Eq. (B12), contain as well a dependence on \(\kappa _c^{(0)}\). If the system is under the influence of an external static magnetic field, B, the momentum \(\kappa _c^{(0)}\) then becomes:
where \(\delta _\mu \) is the difference between the magnetic moments of the system in the ground (open) and the excited (closed) states.
Therefore, the condition in Eq. (45) that determines when \(a_\textrm{tw}=\infty \), is now a function of d and B. In other words, one could get the curve “\(B_0\) vs. \(d_E\)” formed by the \((B_0,d_E)\) points satisfying Eq. (45).
5 Properties for three-body systems
Let us consider a three-body system formed by two identical particles and a different one. This system involves two different two-body interactions. If we plot the “\(B_0\) vs. \(d_E\)” curve for each of these two interactions, and they happen to cross, we then have the dimension \(d=d_E\) and magnetic field \(B=B_0\), that make \(a_\textrm{tw}=\infty \) simultaneously for both potentials. In this way it would be possible to get the Efimov condition fulfilled for all the two-body subsystems. Furthermore, following the same procedure, the Efimov conditions can also be fulfilled in a three-body system made of three different constituents, since with this method it is, in principle, possible to tune \(a_\textrm{tw}=\infty \) for two of the three two-body interactions involved.
Let us then focus on these two different three-body systems, one made of two identical particles and one different (ABB system), and a system made of three different particles (ABC system). Here we analyze the scaling between consecutive Efimov states, and how to construct the appropriate two-body potentials.
5.1 Mass dependence of the scale factor
Let us recall that for the ABB case, when only the AB scattering length is sufficiently large, the situation of two heavy particles and one light particle is particularly favorable for the appearance of Efimov states [16]. In this case, the energy scale factor between two consecutive states is significantly reduced. As a consequence, its experimental determination, or even its numerical calculation, is much easier than in the case of two light particles and one heavy particle.
The energy scale factor between two consecutive states is given by \(E_n/E_{n+1}=\exp {(2\pi /\vert \nu _\infty \vert )}\), where \(E_n\) is the binding energy of the \(n^\textrm{th}\) Efimov state and \(\vert E_n\vert > \vert E_{n+1}\vert \) (\(n=1,2,3,\cdots \)). The d-dependent \(\vert \nu _\infty \vert \) is independent of the interactions and independent of n. The value of \(\vert \nu _\infty \vert \) can be obtained through a transcendental equation as shown in Eqs. (26) and (27) of Ref. [17] for \(d=3\), and generalized for arbitrary dimension in subsection 5.2 of Ref. [15].
The results for the ABB system are shown in Fig. 2, where we show the logarithm of the energy ratios between two consecutive Efimov states as functions of the mass ratio \(m_B/m_A\). More precisely, the y-axis gives the exponent a when the energy ratio is written as \(10^a\).
We first focus on the results when the scattering length between the two identical particles, \(a_{BB}\), is equal to 0, and the one between the two different particles, \(a_{AB}\), is equal to infinity (thin curves). Three different dimensions, \(d=3.0\), 2.8, and 2.6, are considered. As we can see, when \(m_B \gg m_A\), which corresponds to two heavy particles and one light particle, the energy scale factor is many orders of magnitude smaller than for \(m_B \ll m_A\), which corresponds to two identical light particles and one heavy particle. We can also see that, the smaller the dimension, the sooner the divergence of the energy scale factor occurs with decreasing mass ratio, \(m_B/m_A\).
When the two scattering lengths, \(a_{AB}\) and \(a_{BB}\), are equal to infinity we obtain the results shown by the thick curves in Fig. 2. For two heavy particles and one light particle, we can see that the effect of making \(a_{BB}=\infty \) is very small. However, for two light particles and one heavy particle, the ratio between two consecutive Efimov states reduces significantly. For the three dimensions shown in the figure the scale factor ranges between 250 and 1000 when \(m_B/m_A \ll 1\). These ratios are comparable, or even smaller, than for three identical bosons in three dimensions, where the energy scale factor is 515.
In Fig. 3 we show the same as in Fig. 2 but for the ABC system. The scattering lengths between particles A and B, \(a_{AB}\), and between particles A and C, \(a_{AC}\), are equal to infinity, and the one between B and C, \(a_{BC}\), is equal to 0. The masses of particles B and C, \(m_B\) and \(m_C\), have been chosen such that \(m_C=2 m_B\). The curves are again shown as a function of \(m_B/m_A\). The behavior of these curves is very similar to the thin ones in Fig. 2. That is, when \(m_B \ll m_A\) the system behaves as the case of two identical light particles and a heavy particle in Fig. 2, and the energy scale factor between two consecutive Efimov levels is enormous. On the contrary, when \(m_A\) is much smaller than the other two masses, the system behaves as in the case of two identical heavy particles and a light particle, with an energy scale factor even smaller than 10 for \(m_B/m_A=100\) and for the three dimensions shown in the figure. The conclusion is then that, for an ABC system, if one of the particles is much lighter than the other two, and the scattering length between this light particle and the other two is sufficiently large, the energy scale factor can be reasonably small.
5.2 Constructing the two-body potentials
Equations (45) and (46) permit to obtain the pairs of values, magnetic field and dimension, that make the two-component scattering length, \(a_\textrm{tw}\), equal to infinity. The magnetic field and dimension values fulfilling this condition will be denoted as \((B_0,d_E)\).
The goal now is to obtain the \((B_0,d_E)\) points for specific two-body systems. To do so, it will be necessary to specify the potential used. In general, the parameters entering in the interaction will be determined making use of the experimental information available in three dimensions.
The two-component problem in three dimensions has been investigated in Ref. [13]. There, it has been shown that the two-component scattering length is given by:
where \(\beta ^2\) describes the coupling between the open and closed channels, and
In Ref. [13], \(a_\textrm{open}\) is taken equal to \(a_{\textrm{bg}}\), often known experimentally. The same equality, \(a_\textrm{open}=a_{\textrm{bg}}\), will be considered here.
From Eq. (47), and taking the value of the magnetic field, \(B=B_0\), such that \(a_\textrm{tw}=\infty \), we can easily see that:
In the same way, if we take \(B=B_0+\Delta B\) such that \(a_\textrm{tw}=0\), we obtain:
Feshbach resonances are therefore characterized by the experimental parameters \(a_{\textrm{bg}}\), \(B_0\), \(\Delta B\), and \(\delta _\mu \). With this experimental information we can, through Eq. (50), determine the coupling term \(\beta ^2\), and then, through Eq. (49), the scattering length for the closed channel, \(a_\textrm{closed}\).
The simple two-body square-well interactions used in this work require two parameters to be fully determined, the range and the strength. For the range we shall always use the van der Waals length, \(R_{\textrm{vdW}}\), often known experimentally. The strength of the open and closed channels, \(V_o\) and \(V_c\) in Eq. (11), are fixed in order to reproduce, respectively, the value of \(a_\textrm{open}\), known experimentally, and \(a_\textrm{closed}\) as given in Eq. (49) for \(d=3\). Finally, the coupling strength, \(V_{co}\) in Eq. (11), is obtained by imposing that, for \(B=B_0\) and \(d=3\), we must get \(a_\textrm{tw}=\infty \).
Even if these constraints permit to determine the range and the strength of the open, closed, and coupling potentials, there is still some freedom to fix these values. First, the value of \(E^*\), which enters through \(\kappa (B_0)\) in Eqs. (49) and (50), is completely arbitrary, although, as quoted in [13], its value does not affect the final observables significantly. And second, the values of \(V_o\) and \(V_c\) can be very different depending on the number of bound states hold by the potentials. About \(V_{co}\), after fixing \(V_o\) and \(V_c\), it is still possible to find a family of different values all of them giving rise to \(a_\textrm{tw}=\infty \).
In any case, in what follows, the goal is not to derive detailed two-body potentials for the systems under investigation, but specifically to show that, by a combination of the confinement and external magnetic field, it is in principle possible to simultaneously tune the two interactions involved in the ABB-systems, or two out of the three interactions involved in the ABC-systems. In this way, the energy separation between the Efimov states in ABB-systems can be drastically reduced, and even systems involving three different constituents could exhibit the Efimov effect with a reasonably small energy separation between the states.
6 The ABB-system
The energy scale factor for an ABB system was discussed in Fig. 2. In particular, we saw that, when particle A is much heavier than the other two, having the two scattering lengths, \(a_{AB}\) and \(a_{BB}\), simultaneously equal to infinity, enormously reduces the separation between consecutive Efimov states.
To illustrate this fact, we choose the \(^{87}\)Rb-\(^7\)Li-\(^7\)Li system, which in principle should not be a good candidate to exhibit the Efimov effect. In order to investigate this system it is necessary first to construct the required \(^7\)Li-\(^{87}\)Rb and \(^7\)Li-\(^7\)Li two-body potentials.
6.1 The \(^7\)Li-\(^{87}\)Rb dimer
The experimental information about this system can be found in Ref. [18]. In particular, they give a value for the \(C_6\) coefficient in the van der Waals potential of \(2550 E_h a_0^6\) (\(E_h\) is a Hartree and \(a_0\) the Bohr radius), from which one can get a van der Waals length of \(R_{\textrm{vdW}}=44.1 a_0\), which is taken as the potential range of our square-well potentials. The connection between the \(C_6\) coefficient and \(R_{\textrm{vdW}}\) is given by [2]:
where \(\mu \) is the reduced mass of the system.
In [18] they also found a broad Feshbach resonance centered at \(B_0=649\) G, with \(\Delta B=-70\) G, and \(a_{\textrm{bg}}=a_\textrm{open}=-36 a_0\). Although the value for \(\delta _\mu \) is not given, we shall use the typical value \(\delta _\mu = 2\mu _B\) (where \(\mu _B\) is the Bohr magneton).
With these values we have that \(\delta _\mu B_0=0.087\) K, which implies that \(E^*\) must be larger than this value (otherwise, see Eq. (48), we would get an imaginary value of \(\kappa (B_0)\)). In particular we have chosen \(E^*=5\) K, which is sufficiently larger than \(\delta _\mu B_0\) such that the final results are almost independent of the specific value of \(E^*\). Using the values of \(a_\textrm{open}\), \(E^*\), \(B_0\), \(\Delta B\), and \(\delta _\mu \) given above we get from Eq. (49) that \(a_\textrm{closed}=1.65 a_0\).
We therefore choose the strengths \(V_o\) and \(V_c\), such that the values of \(a_\textrm{open}=-36 a_0\) and \(a_\textrm{closed}=1.65 a_0\) are reproduced. To do so, one could in principle choose the minimum possible strength, which amounts to a two-body potential not even binding the two-body dimer in the case of negative scattering length. This is very unrealistic, since the number of bound \(^7\)Li-\(^{87}\)Rb states is probably quite high. For this reason we have chosen a strength for the open channel \(V_o=28.448\) K, which gives rise to about 20 bound dimer states. For the closed channel, among all the possible strengths reproducing the desired value of \(a_\textrm{closed}\), we have taken \(V_c= 28.441\) K as the value closest to the chosen \(V_o\) value.
For the coupling potential, \(V_{co}\), adjusted to obtain \(a_\textrm{tw}=\infty \) for \(B=B_0\), we have chosen a value clearly smaller than \(V_o\) and \(V_c\), but not small enough to be a perturbation. In particular we have taken \(V_{co}=4.733\) K.
The selected values of these potential parameters are collected in the first row of Table 1.
6.2 The \(^7\)Li-\(^{7}\)Li dimer
For the \(^7\)Li-\(^{7}\)Li interaction we proceed in the same way using the information provided in Ref. [2]. The van der Waals length is equal to 33.1 \(a_0\), which is taken as the range of the potentials.
In three dimensions, the Feshbach resonance for the \(^7\)Li-\(^{7}\)Li system is characterized by \(B_0=737\) G, \(\Delta B=-192.3\) G, \(a_\textrm{open}=-25 a_0\), and \(\delta _\mu =1.93 \mu _B\). These values correspond to \(\delta _\mu B_0=0.096\) K, and, as for the \(^7\)Li-\(^{87}\)Rb system, we choose \(E^*=5\) K.
With all this information, by means of Eq. (49), we now get \(a_\textrm{closed}=2.25 a_0\). The strengths of the open and closed channels have been chosen to be \(V_o=20.049\) K and \(V_c=20.026\) K, which reproduce, respectively, the desired values of \(a_\textrm{open}\) and \(a_\textrm{closed}\). With these strengths the dimer has 10 bound states. Finally, using the coupling potential strength, \(V_{co}=3.883\) K, we get that \(a_\textrm{tw}=\infty \) for \(d=3\).
We collect the details of this potential in the second row of Table 1,
6.3 Dimension dependence of the Feshbach resonances
Now that the parameters for the two-body interactions have been selected, we can investigate how the position of the Feshbach resonances change with dimension d.
In Fig. 4a we show, for \(d=3\), the denominator of Eq. (44), as a function of the magnetic field B, for the potentials parameters for the \(^{7}\)Li-\(^7\)Li and \(^{7}\)Li-\(^{87}\)Rb dimers. The crossings of the curves with the zero-axis correspond to the B-values giving rise to \(a_\textrm{tw}=\infty \), and therefore producing a Feshbach resonance. These values of the magnetic field reproduce of course the values given in Refs. [2] and [18], and quoted in Table 1, \(B_0=737\) G for \(^7\)Li-\(^7\)Li and \(B_0=649\) G for \(^7\)Li-\(^{87}\)Rb.
The same calculation as in Fig. 4a, but for different values of the dimension, would give rise to different \(B_0\)-values such that a Feshbach resonance appears on each of the two-body systems. In Fig. 4b we show the family \((B_0,d_E)\) values producing a Feshbach resonance for the \(^7\)Li-\(^7\)Li and the \(^7\)Li-\(^{87}\)Rb dimers, which are the ones entering in the \(^{87}\)Rb-\(^7\)Li-\(^7\)Li trimer. The arrows in the figure indicate the \(B_0\) values obtained for \(d_E=3\), \(B_0=737\) G (\(^7\)Li-\(^7\)Li) and 649 G (\(^7\)Li-\(^{87}\)Rb), which, as mentioned above, are the ones used to construct the potentials.
The relevant thing is that, as we can see in the figure, the solid and dashed curves cross at some particular \((B_0,d_E)\) point, \(d_E=2.93\) and \(B_0=149\) G. For these values of the dimension and the magnetic field, the scattering length, \(a_\textrm{tw}\), for both two-body potentials is, simultaneously, equal to infinity. This fact implies that, for this specific \((B_0,d_E)\) value, the three-body system \(^{87}\)Rb-\(^7\)Li-\(^7\)Li fulfills the Efimov conditions simultaneously in all the internal two-body subsystems. In particular, for \(d_E=2.93\) the energy scale factor for two consecutive Efimov states is only about 317, a value that can not even be compared to the scale factor obtained when only the \(^{87}\)Rb-\(^7\)Li has infinite scattering length, since in this case the scale factor is larger than \(10^{50}\).
The price to pay is that, as discussed below Eq. (1), a \(d_E\) value of 2.93, which leads to \(b_{ho}/r_0=3.71\), amounts to confinement frequencies in the range of the MHz, clearly higher than today’s available experimental values.
7 The ABC-system
As shown in Fig. 3, for the case of three different constituents, the most interesting situation is when one of them is clearly lighter than the other two. In this case, if the interaction between the light particle and the other two is tuned to produce \(a_\textrm{tw}=\infty \) in both cases, then the Efimov conditions are fulfilled, and, furthermore, the energy separation between the Efimov states is relatively small.
To illustrate this point we choose the \(^7\)Li-\(^{39}\)K-\(^{87}\)Rb system. The interaction used to describe the \(^7\)Li-\(^{87}\)Rb dimer was detailed in the previous section. The remaining interaction needed, the \(^7\)Li-\(^{39}\)K potential, is described below.
7.1 The \(^7\)Li-\(^{39}\)K dimer
The details of the Feshbach resonance in three dimensions, required to determine the \(^7\)Li-\(^{39}\)K potential, are taken from Ref. [19]. In particular the following information about the resonance is given: \(B_0=319\) G, \(\Delta B=30\) G, \(a_\textrm{open}=89 a_0\), and \(\delta _\mu =1.5 \mu _B\). Also, from the value provided for the \(C_6\) van der Waals coefficient we obtain the van der Waals length, \(R_{\textrm{vdW}}=42.1 a_0\), which is the value used for the radius of our square-well potentials.
With these numbers we get \(\delta _\mu B_0=0.032\) K, and, as in the previous cases, we choose \(E^*=5\) K. This value of \(E^*\), together with the values given above, by means of Eq. (49), results in \(a_\textrm{closed}=1.71 a_0\).
As for the other two potentials, we adjust \(V_o\) and \(V_c\) such that they reproduce the required values of \(a_\textrm{open}\) and \(a_\textrm{closed}\). We take then \(V_o=17.072\) K and \(V_c=17.040\) K. These two strengths give rise to a \(^7\)Li-\(^{39}\)K dimer holding about 15 bound states. When combined with a coupling strength \(V_{co}=2.505\) K, we obtain a two-component scattering length \(a_\textrm{tw}=\infty \) for \(d=3\).
As for the other two potentials, we collect in the last row of Table 1 the details of this interaction.
7.2 Dimension dependence of the Feshbach resonance positions
We proceed now as for the ABB-case, and show in Fig. 5a the denominator of Eq. (44), as a function of the magnetic field, B, for the potential described above for the \(^7\)Li-\(^{39}\)K dimer and \(d=3\). We also show this denominator for the \(^7\)Li-\(^{87}\)Rb case, already plotted in Fig. 4a. Again, the crossing of each curve with the zero-axis corresponds to the different B-values giving rise to \(a_\textrm{tw}=\infty \), and therefore producing a Feshbach resonance. This crossings can be easily seen in the zoom of the figure shown in the inset. Again, as expected, the crossings correspond to the values \(B_0=319\) G (\(^7\)Li-\(^{39}\)K) and \(B_0=649\) G (\(^7\)Li-\(^{87}\)Rb) used to construct the potentials (see Table 1).
We can now investigate how the position of the Feshbach resonances change with the dimension d, and get the different \((B_0,d_E)\) values that produce a Feshbach resonance in both, the \(^7\)Li-\(^{39}\)K and the \(^{7}\)Li-\(^{87}\)Rb dimers, and in particular, check if it is possible to find a \((B_0,d_E)\) value that produces a resonance simultaneously in both systems.
This is shown in Fig. 5b, which is the same as in Fig. 4b, but for the \(^7\)Li-\(^{39}\)K and \(^{7}\)Li-\(^{87}\)Rb dimers. We can see that, again, both curves cross, determining therefore a dimension, \(d_E=2.81\), and a magnetic field, \(B_0=-673\) G, such that \(a_\textrm{tw}=\infty \) in the two systems at the same time. The negative value of \(B_0\) means a projection of the magnetic field opposite to the direction of the magnetic moment difference of the open and closed two-body channels. The Efimov conditions are therefore fulfilled, and with these mass ratios for \(d=2.81\), and assuming that the scattering length between the \(^{39}\)K and \(^{87}\)Rb is small, the energy scale factor between two consecutive Efimov states is then about 330. From Eq. (1) we obtain that this dimension corresponds to \(b_{ho}/r_0=2.17\), which again represents a pretty tight confinement, with frequencies in the range of the MHz.
8 Summary and conclusions
The d-method, where the dimension d can take non-integer values, is an efficient way of describing systems squeezed by an external field. During the squeezing process, the effective interaction between two particles is modified, in such a way that, if the two-body system is unbound in three dimensions, there must necessarily be a moment where the two-body binding energy is equal to zero (infinite scattering length). The equivalent dimension describing this squeezing situation is what we call the critical dimension, \(d_E\).
A different procedure that permits as well the modification of the effective two-body interaction consists on putting the system under the effect of a static magnetic field. The coupling of the field with the magnetic moments of the particles allows in particular the population of the so called Feshbach resonances, which appear for some particular value, \(B_0\), of the magnetic field, and which corresponds as well to an infinite two-body scattering length.
In this work we have considered the combination of these two different procedures in order to investigate the possibility of simultaneous tuning of two of the different interactions involved in an asymmetric three-body system. This would permit to construct ABB three-body systems where the AB and BB two-body potentials have both infinite scattering length. In this way, for systems consisting of two identical light particles and a heavy one, the energy scale factor between consecutive Efimov states is reduced by many orders of magnitude. Even for systems made of three different particles, ABC systems, it would be possible to tune the AB and AC potentials, and construct in this way a series of Efimov states whose energy separation is reasonably small when the mass of particle A is much smaller than the mass of the other two.
The analysis of the Feshbach resonances as a function of the dimension has been done analytically assuming a two-component problem for the two-body systems, where only one open and one closed channel contribute, and assuming square-well two-body potentials. In this way we have derived analytic expressions for the open-channel and closed-channel wave functions, and from them we have obtained an analytic expression for the phase shifts. By expansion of the phase shift in powers of energy we have obtained analytic expressions for the scattering length and the effective range. A detailed analysis of the two-component scattering length allowed us to extract the curve made by all the \((B_0,d_E)\) points such that for that value, \(B_0\), of the magnetic field, and that dimension, \(d_E\), the two-body scattering length is equal to infinity.
All these analytical expressions have been used to investigate the two-body potentials involved in two different three-body systems, \(^{87}\)Rb-\(^7\)Li-\(^7\)Li, as an example of an ABB system containing two light particles and a heavy one, and \(^7\)Li-\(^{39}\)K-\(^{87}\)Rb, as an example of an ABC system where one particle is much lighter than the other two. Making use of the available experimental information we have constructed the \(^{87}\)Rb-\(^7\)Li, \(^7\)Li-\(^7\)Li, and \(^7\)Li-\(^{39}\)K potentials in three dimensions. With the obtained potential parameters we have then made use of the derived analytical expression for the scattering length and, for each of the interactions, we have constructed the \((B_0,d_E)\)-curve providing all the \((B_0,d_E)\) pair values corresponding to infinite two-body scattering length. We have then observed that the curves arising from the \(^{87}\)Rb-\(^7\)Li and \(^7\)Li-\(^7\)Li potential cross at some particular \((B_0,d_E)\)-point. For these values of the magnetic field and the dimension, both the \(^{87}\)Rb-\(^7\)Li and the \(^7\)Li-\(^7\)Li, scattering lengths are equal to infinity, and the energy scale factor between two consecutive Efimov states reduce by many orders of magnitude down to a value of about 317. The same happens for the \(^7\)Li-\(^{39}\)K-\(^{87}\)Rb system. The \((B_0,d_E)\)-curves corresponding to the \(^{87}\)Rb-\(^7\)Li and the \(^7\)Li-\(^{39}\)K potentials cross as well at some particular \((B_0,d_E)\)-point, in such a way that for this magnetic field and dimension the Efimov conditions are fulfilled, and the separation between the Efimov states reduces to a factor of about 330.
The trimers chosen in this work and the rough estimate of the atom-atom potentials, have led to confinement frequencies that are too high compared to the current available experimental values. However, this fact does not invalidate the main conclusion, which is that simultaneous tuning of two different two-body potentials after combination of squeezing of the system and the population of Feshbach resonances by means of a static magnetic field is in principle possible. This could be today limited to systems where this happens for a very modest confinement strength, but there is always the possibility that, eventually, much higher frequencies could be reached.
Our results open the door to the construction of Efimov states in three-body systems which in principle are not good candidates to exhibit this phenomenon, like systems made of two identical particles and a heavy one, or even systems made of three different particles.
In summary, the numerical discussions are based on short-range particle-particle square-well potentials. However, the Efimov physics is a long-distance phenomenon, and appearance and properties are independent of the employed short-range potentials. We emphasize therefore that our conclusions are universal as described in terms of the long-range gross properties, scattering length and effective range. The results are also universal in the sense that they apply to all two and three-body systems in any subfield of physics or chemistry.
A number of perspectives are immediate for future few-body investigations involving external deformed squeezing potentials, which can be studied using the equivalent d-method for non-integer dimensions. More precise calculations on specific experimental selected systems could be necessary. Also extended computations would be of interest, for example shapes of Feshbach resonances and three-body recombination rates related to Efimov physics.
Data Availability Statement
This manuscript has no associated data or the data will not be deposited. [Authors’ comment: Since this is a theoretical work, there are no external data associated with this manuscript.]
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Acknowledgements
This work has been partially supported by grant No. PGC2018-093636-B-I00, funded by MCIN/AEI/10.13039/501100011033 and by “ERDF A way of making Europe”. We acknowledge Jan Arlt for providing experimental information.
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Both authors have equally contributed to the discussion and the analytic calculations. EG has performed the numerical calculations.
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Appendices
Appendix A: Matching at box radius, \(x=1\).
The logarithmic derivatives of the solutions in Eqs. (15) and (32), and in Eqs. (16) and (33), outside and inside the box, must be equal at the box radius, \(x=1\). This condition leads to the following two equations:
where the prime denotes derivative with respect to the full coordinate of the corresponding Hankel or Bessel function. Both equations contain the ratio between the normalization constants, \(C_+\) and \(C_-\) in Eq. (29). Equation (A1) can be used to determine
which by use of Eq. (D29) reduces to
where we have defined
and where the relation in Eq. (D31) has been used.
From Eq. (A2) we can now extract the phase shift and find
where
Using Eq. (A4) and, again Eq. (D29), we reformulate Eqs. (A6) and (A7), and finally write:
where, after inserting the expression for \(C_+/C_-\) from Eq. (A4), and using Eqs. (21) and (D29), we have redefined \(F_2\) as:
which, together with Eq. (A5), provides the final analytical formula for the phase shift.
Note that in case of no coupling, \(a_{co}=0\), we have that \(F_2=\sqrt{a_-} j_{\ell +1}(\sqrt{a_-})/j_{\ell }(\sqrt{a_-})\), and Eq. (A8) reduces to Eq. (20) of Ref. [20].
Appendix B: Low-energy expansion of the phase shift
The quantities entering in the expression for the phase shift, Eq. (A8), are \(D_{\pm }\) and \(a_{\pm }\) in various combinations. The relevant expressions are Eqs. (9), (18), (19), (25), and (26). The following abbreviations in terms of the basic interaction quantities are useful
The expressions in Eq. (A8) can be reduced for low energy as [21]
and
The remaining functions to expand around finite values are then \(F_1\), \(F_2\), and the ratios of various Bessel functions. With obvious notation we can write
where we explicitly have for both Eqs. (A5) and (A9)
and
The derivatives, \(F_1^{\prime (0)}\) and \(F_2^{\prime (0)}\) both involve combinations of derivatives of ratios of spherical Bessel or Hankel functions of the form \(f_a(z) = z \frac{j_{a+1}(z)}{j_{a}(z)}\), where z is \(D_{\pm }\), and \(g_a(z) = z \frac{h_{a+1}^{(+)}(z)}{h_{a}^{(+)}(z)}\) with \(z=i \kappa _c\). The derivatives, \(f^\prime _a(z)\) and \(g^\prime _a(z)\), of these pieces are evaluated by use of Eq. (D32), where the derivatives of z must also be inserted, that is
Noting also that \((D^2_--a_+)\) is E-independent, the derivatives are then easily obtained to be
and
The phase shift expanded to second order in energy is now
which can be rewritten as
where for non-integer values of \(\ell \) the factor \((2\ell +1)!!\) should be replaced by \(\Gamma (2\ell +2)/(2^\ell \Gamma (\ell +1))\).
Appendix: C The two-component effective range
As done for the scattering length, after comparison of Eqs. (35) and Eq. (36), we obtain:
If we assume relative s-waves (\(\ell =0\)), making use of Eqs. (B23) and (D29), and after some tedious algebra, we can see that Eq. (C27) reduces to the known analytic form of the effective range for the square-well potential [22]:
Making use of Eqs. (B21), (39), (40), and (41), we can obtain the effective range, Eq. (C27), in terms of \(a_\textrm{open}\) and \(a_\textrm{closed}\), although the expression obtained is certainly more complicated than the one given in Eq. (42) for the scattering length.
Appendix: D Some useful Bessel function properties
Here, we collect relations between the Bessel functions used to derive the expressions obtained in this work. They have been taken from [21].
Below, \(B_\ell \) represents either the regular, \(j_\ell \), the irregular, \(\eta _\ell \), spherical Bessel functions, or the Hankel, \(h^{(\pm )}_{\ell }= j_\ell \pm i \eta _\ell \), functions. The derivative of \(B_\ell (z)\) is given by:
The Hankel function \(h_\ell ^{(+)}(i\kappa _c)\) is related to the modified Bessel function of third kind, \(K_{\ell +\frac{1}{2}}(\kappa _c)\), by:
which permits to write:
The derivative of \(f_a(z) = z \frac{B_{a+1}}{B_{a}}\) is given by:
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Garrido, E., Jensen, A.S. Tuning of Efimov states in non-integer dimensions. Eur. Phys. J. D 77, 46 (2023). https://doi.org/10.1140/epjd/s10053-023-00628-2
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DOI: https://doi.org/10.1140/epjd/s10053-023-00628-2