Abstract
A process combining ceramic ultrafiltration, catalytic ozonation, and adsorption by activated carbon was applied and evaluated for the advanced treatment of domestic effluent from a biological aerated filter in a pilot scale. The main operating parameters such as operating pressure and ozone dose were optimized, and a stable operation was conducted for 30 days. The results showed that the chemical oxygen demand was decreased from 30 ± 10 mg L−1 to less than 15 mg L−1, ammonium nitrogen was reduced from 2.5 ± 0.5 mg L−1 to less than 1.0 mg L−1, chroma became colorless from the dilution times of 32, and suspended solids as well as Escherichia coli were completely removed from the initial concentration of 20 ± 5 mg L−1 and at least 2.4 × 106 MPN L−1, respectively. The removal of chemical oxygen demand and chroma was mainly attributed to the synergetic effect of the ultrafiltration and catalytic ozonation, the removal of suspended solids and Escherichia coli was associated with the ultrafiltration, and the removal of ammonium nitrogen mainly resulted from the activated carbon adsorption. The quality of the effluent would be close to the water quality standard III of surface water, and the electricity cost calculated in the optimal conditions was 0.79 kW h t−1.
Similar content being viewed by others
References
Abdullayev A, Bekheet MF, Hanaor DA, Gurlo A (2019) Materials and applications for low-cost ceramic membranes. Membranes 9(9):105. https://doi.org/10.3390/membranes9090105
Bergamasco R, Konradt-Moraes L, Vieira M, Fagundes-Klen M, Vieira A (2011) Performance of a coagulation–ultrafiltration hybrid process for water supply treatment. Chem Eng J 166:483–489. https://doi.org/10.1016/j.cej.2010.10.076
Cao L, Sun R, Dong W, Wang H, Dai Z, Wang X, Xie J, Li H (2022) A novel multistage anoxic/aerobic process with sludge regeneration zone (R-MAO) for advanced nitrogen removal from domestic sewage. J Environ Sci. https://doi.org/10.1016/j.jes.2022.02.008
Chen R, Zhang K, Wang H, Wang X-m, Zhang X-h (2022a) Incorporating catalytic ceramic membrane into the integrated process of in situ ozonation, membrane filtration and biological degradation: enhanced performance and underlying mechanisms. J Membr Sci 652:120509. https://doi.org/10.1016/j.memsci.2022.120509
Chen R, Zhang K, Wang H, Wang X-m, Zhang X-h, Huang X (2022b) Incorporating catalytic ceramic membrane into the integrated process of in situ ozonation, membrane filtration and biological degradation: enhanced performance and underlying mechanisms. J Membr Sci 652:120509. https://doi.org/10.1016/j.memsci.2022.120509
Chen T, Wei X, Chen Z, Morin D, Alvarez SV, Yoon Y, Huang Y (2022c) Designing energy-efficient separation membranes: knowledge from nature for a sustainable future. Adv Membr 2:100031. https://doi.org/10.1016/j.advmem.2022.100031
Deng F, Qiu S, Chen C, Ding X, Ma F (2015) Heterogeneous catalytic ozonation of refinery wastewater over alumina-supported Mn and Cu oxides catalyst. Ozone-Sci Eng 37:150724175904004. https://doi.org/10.1080/01919512.2015.1065173
Dong Y, Wu H, Yang F, Gray S (2022) Cost and efficiency perspectives of ceramic membranes for water treatment. Water Res 220:118629. https://doi.org/10.1016/j.watres.2022.118629
Fan Y, Guo Z, Wang J, Zhang B, Shen Y, Gao X (2022) Online learning-empowered smart management for A2O process in sewage treatment processes. Environ Res 210:113015. https://doi.org/10.1016/j.envres.2022.113015
Farabegoli G, Chiavola A, Rolle E (2009) The biological aerated filter (BAF) as alternative treatment for domestic sewage. Optimization of plant performance. J Hazard Mater 171(1):1126–1132. https://doi.org/10.1016/j.jhazmat.2009.06.128
Guerra K, Pellegrino J (2012) Development of a techno-economic model to compare ceramic and polymeric membranes. Separ Sci Technol. https://doi.org/10.1080/01496395.2012.690808
Guillossou R, Roux JL, Brosillon S, Mailler R, Gaspéri J (2019) Benefits of ozonation before activated carbon adsorption for the removal of organic micropollutants from wastewater effluents. Chemosphere 245:125530. https://doi.org/10.1016/j.chemosphere.2019.125530
Hernandez-Sancho F, Molinos-Senante M, Sala-Garrido R (2011) Cost modelling for wastewater treatment processes. Desalination 268(1–3):1–5. https://doi.org/10.1016/j.desal.2010.09.042
Hoek E, Elimelech M (2004) Cake-enhanced concentration polarization: a new fouling mechanism for salt-rejecting membranes. Environ Sci Technol 37:5581–5588. https://doi.org/10.1021/es0262636
Huang L, Han J, Wang G, Hou Y, Li Z, Yi F (2023) Optimization of A2O–MBR–BAF–O3 combination process for domestic wastewater. Int J Environ Sci Technol. https://doi.org/10.1007/s13762-023-04785-0
Jiang T, Tian T, Guan Y-F, Yu H-Q (2022) Contrasting behaviors of preozonation on ceramic membrane biofouling: early stage vs late stage. Water Res 220:118702. https://doi.org/10.1016/j.watres.2022.118702
Karnik B, Davies S, Chen K-C, Jaglowski D, Baumann M, Masten S (2005) Effects of ozonation on the permeate flux of nanocrystalline ceramic membranes. Water Res 39:728–734. https://doi.org/10.1016/j.watres.2004.11.017
Kim J, Davies S, Baumann M, Tarabara V, Masten S (2008) Effect of ozone dosage and hydrodynamic conditions on the permeate flux in a hybrid ozonation–ceramic ultrafiltration system treating natural waters. J Membrane Sci 311:165–172. https://doi.org/10.1016/j.memsci.2007.12.010
Li K, Huang T, Qu F, Du X, Ding A, Li G, Liang H (2016) Performance of adsorption pretreatment in mitigating humic acid fouling of ultrafiltration membrane under environmentally relevant ionic conditions. Desalination 377:91–98. https://doi.org/10.1016/j.desal.2015.09.016
Li P, Miao R, Wang P, Sun F, Li X-y (2021) Bi-metal oxide-modified flat-sheet ceramic membranes for catalytic ozonation of organic pollutants in wastewater treatment. Chem Eng J 426:131263. https://doi.org/10.1016/j.cej.2021.131263
Manica M, Battistelli A, Belli T, Souza J, Lapolli F, Vidal C (2021) Effects of electrocoagulation on membrane fouling and treatment performance of a membrane bioreactor operated without sludge discharge. Int J Environ Sci Technol 18:1695–1708. https://doi.org/10.1007/s13762-020-02953-0
Mestre S, Gozalbo A, Lorente-Ayza M, Sánchez E (2019) Low-cost ceramic membranes: a research opportunity for industrial application. J Eur Ceram Soc 39(12):3392–3407. https://doi.org/10.1016/j.jeurceramsoc.2019.03.054
Mišík M, Ferk F, Schaar H, Yamada M, Jaeger W, Knasmueller S, Kreuzinger N (2020) Genotoxic activities of wastewater after ozonation and activated carbon filtration: different effects in liver-derived cells and bacterial indicators. Water Res 186:116328. https://doi.org/10.1016/j.watres.2020.116328
Özgün H, Sakar H, Ağtaş M, Koyuncu İ (2023) Investigation of pre-treatment techniques to improve membrane performance in real textile wastewater treatment. Int J Environ Sci Technol 20(2):1539. https://doi.org/10.1007/s13762-022-04034-w
Qi M, Yang Y, Zhang X, Zhang X, Wang M, Zhang W, Lu X, Tong Y (2020) Pollution reduction and operating cost analysis of municipal wastewater treatment in China and implication for future wastewater management. J Cleaner Prod 253:120003. https://doi.org/10.1016/j.jclepro.2020.120003
Qu F, Du X, Liu B, He J, Ren N-Q, Li G, Liang H (2015) Control of ultrafiltration membrane fouling caused by Microcystis cells with permanganate preoxidation: significance of in situ formed manganese dioxide. Chem Eng J. https://doi.org/10.1016/j.cej.2015.05.009
Rasouli Y, Abbasi M, Hashemifard SA (2019) A new combination of microfiltration, powdered activated carbon and coagulation for treatment of oily wastewater. Int J Environ Sci Technol 16(10):5595. https://doi.org/10.1007/s13762-018-1906-5
Ren Z, Jia B, Zhang G, Fu X, Wang Z, Wang P, Lv L (2021) Study on adsorption of ammonia nitrogen by iron-loaded activated carbon from low temperature wastewater. Chemosphere 262:127895. https://doi.org/10.1016/j.chemosphere.2020.127895
Rifi S, Fels L, Driouich A, Hafidi M, Ettaloui Z, Souabi S (2022) Sequencing batch reactor efficiency to reduce pollutant in olive oil mill wastewater mixed with urban wastewater. Int J Environ Sci Technol 19(11):11361–11374. https://doi.org/10.1007/s13762-021-03866-2
Rodríguez-Chueca J, Ormad M, Mosteo R, Ovelleiro JL (2015) Kinetic modeling of Escherichia coli and Enterococcus sp. inactivation in wastewater treatment by photo-Fenton and H2O2/UV-vis processes. Chem Eng Sci. https://doi.org/10.1016/j.ces.2015.08.051
Su J, Ji D, Lin M, Chen Y, Sun Y, Huo S, Zhu J, Xi B (2017) Developing surface water quality standards in China. Resour Conserv Recycl 117:294–303. https://doi.org/10.1016/j.resconrec.2016.08.003
Uddin Z, Ahmad F, Ullan T, Nawab Y, Ahmad S, Azam F, Rasheed A, Zafar MS (2022) Recent trends in water purification using electrospun nanofibrous membranes. Int J Environ Sci Technol 19(9):9149. https://doi.org/10.1007/s13762-021-03603-9
Wang X, Chen S, Dong W, Wang Z, Yang L, Xi X, Zhang Q, Shi L (2012) Contribution of main pollutants in oilfield polymer-flooding wastewater to the total membrane fouling resistance. Separ Sci Technol. https://doi.org/10.1080/01496395.2012.656873
Wang X, Liu Y, Zhang Y, Shi W, Yang Y, Kong L (2023) Study on the application and optimization of domestic sewage treatment demonstration based on a novel biofilter-constructed wetland coupling system. Int J Environ Sci Technol 20(1):909. https://doi.org/10.1007/s13762-022-03939-w
Wu S, Yuanfeng Q, He S, Fan C, Dai B, Zhou W, Gao L, Huang J (2015) Preparation and application of novel catalytic-ceramic-filler in a coupled system for TNT manufacturing wastewater treatment. Chem Eng J 280:417–425. https://doi.org/10.1016/j.cej.2015.06.017
Zawadzki P (2022) Evaluation of TiO2/UV; O3/UV, and PDS/Vis for improving chlorfenvinphos removal from real municipal treated wastewater effluent. Int J Environ Sci Technol. https://doi.org/10.1007/s13762-022-04370-x
Zhang Q, Xu R, Xu P, Chen R, He Q, Zhong J, Gu X (2014) Performance study of ZrO2 ceramic micro-filtration membranes used in pretreatment of DMF wastewater. Desalination 346:1–8. https://doi.org/10.1016/j.desal.2014.05.006
Zhang J, Yu H, Quan X, Chen S, Zhang Y (2016) Ceramic membrane separation coupled with catalytic ozonation for tertiary treatment of dyestuff wastewater in a pilot-scale study. Chem Eng J 301:19–26. https://doi.org/10.1016/j.cej.2016.04.148
Zhou Z, Liu J, Zhou N, Zhang T, Zeng H (2021) Does the “10-point water plan” reduce the intensity of industrial water pollution? Quasi-experimental evidence from China. J Environ Manag 295:113048. https://doi.org/10.1016/j.jenvman.2021.113048
Acknowledgements
The authors would like to acknowledge the support for this work by the Beijing Key Laboratory of Aqueous Typical Pollutant Control and Water Quality Safeguard.
Funding
Beijing Key Laboratory of Aqueous Typical Pollutant Control and Water Quality Safeguard, 09210102050133, Jianlin Zhang.
Author information
Authors and Affiliations
Contributions
JLZ involved in methodology, software, investigation, and writing—original draft. JGZ involved in writing—review and editing, supervision, and data curation. JXZ involved in investigation and writing—review and editing. SS involved in software and writing—review and editing. HS involved in writing—review and editing. XZ involved in writing—review and editing. RTL involved in resources and writing—review and editing.
Corresponding author
Ethics declarations
Conflict of interest
There is no relationship with any person or organization that affected the results and conclusions of this work. The authors declare no conflict of interest.
Ethical approval
This article does not contain any studies with human participants or animals performed by any of the authors.
Additional information
Editorial responsibility: Samareh Mirkia.
Rights and permissions
Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.
About this article
Cite this article
Zhang, J.L., Zhang, J.G., Zhang, J.X. et al. Advanced treatment of domestic sewage through ceramic ultrafiltration, catalytic ozonation and activated carbon adsorption in pilot-scale study. Int. J. Environ. Sci. Technol. 21, 2913–2922 (2024). https://doi.org/10.1007/s13762-023-05101-6
Received:
Revised:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s13762-023-05101-6