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Regulating electrochemical performances of lithium battery by external physical field

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Abstract

Lithium batteries have always played a key role in the field of new energy sources. However, non-controllable lithium dendrites and volume dilatation of metallic lithium in batteries with lithium metal as anodes have limited their development. Recently, a large number of studies have shown that the electrochemical performances of lithium batteries can be enhanced through the regulation of external physical fields. Especially, it significantly hinders the growth of lithium dendrites and promoting the reaction kinetics. This review summarizes recent innovations in the investigation of various physical fields of lithium batteries. The application of magnetic field in the synthesis of lithium battery electrode materials is introduced. The influence factors and regulation mechanism of various physical fields on the electrochemical performance of lithium batteries are reviewed emphatically. In addition, the current research status and existing challenges, along with future directions for the evolution of lithium batteries, are minutely discussed and prospected. New strategies for the further evolution of lithium batteries have also been provided.

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摘要

锂电池在新能源领域一直发挥着关键的作用, 但是目前以锂金属为负极的电池中无法控制的锂枝晶和金属锂体积膨胀等问题一直限制其发展. 最近, 有大量的研究表明, 通过外加物理场的调控可以改善锂电池的电化学性能, 特别是在抑制锂枝晶的生长和促进反应动力学上发挥着巨大的作用. 本综述总结了多种物理场在锂电池中应用的最新进展. 介绍了磁场在锂电池电极材料制备中的应用, 着重综述了多种物理场对锂电池的性能影响因素和调控机理. 并且对目前的研究现状和存在的问题以及未来的锂电池发展方向进行了讨论与展望. 这篇综述将为锂电池的发展提供新的策略.

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Scheme 1
Fig. 1

Reproduced with permission from Ref. [38]. Copyright 2022, Elsevier; g cyclic stability at 0.5C of 1D-Fe3O4@C/S, Fe3O4@C/S and Super P/S electrodes. Reproduced with permission from ref. [49]. Copyright 2021, American Chemical Society

Fig. 2

Reproduced with permission from Ref. [55]. Copyright 2019, American Chemical Society. c Cross-sectional SEM images of reference and d aligned Gt electrodes; e Nyquist plots of Gt-G and Gt-N containing cells after 70 cycles-charged state (lithiated) and f discharged state (delithiated) along with simulated EIS data. Reproduced with permission from Ref. [39]. Copyright 2022, American Chemical Society. g Schematic diagram of producing Ti3C2Tx electrodes. Reproduced with permission from Ref. [56]. Copyright 2021, American Chemical Society

Fig. 3

Reproduced with permission from Ref. [40]. Copyright 2021, The Electrochemical Society

Fig. 4

Reproduced with permission from Ref. [35]. Copyright 2019, Wiley–VCH GmbH

Fig. 5

Reproduced with permission from Ref. [80]. Copyright 2020, Elsevier. c Schematic diagram of electronic transition of Co from a low spin state to a high spin state; d Gibbs free energy profiles and adsorption conformation of LiPS species on CoS2; e galvanostatic charging and discharging plots. Reproduced with permission from Ref. [36]. Copyright 2022, Wiley–VCH GmbH

Fig. 6

Reproduced with permission from Ref. [23]. Copyright 2022, Wiley–VCH GmbH. b Schematic illustration of interaction between magnetic field and NiO/FNi under illumination. Reproduced with permission from Ref. [95]. Copyright 2021, Wiley–VCH GmbH. c Design diagram of ICS. Reproduced with permission from Ref. [98]. Copyright 2020, Wiley–VCH GmbH. d Energy-level diagram. Reproduced with permission from Ref. [97]. Copyright 2023, American Chemical Society. e Cyclic performance of photoinduced Li–CO2 batteries with different bending angles of 0°, 8° and 180°. Reproduced with permission from Ref. [98]. Copyright 2020, Wiley–VCH GmbH. f TiO2 and Au@TiO2 LSV curves with and without illumination. Reproduced with permission from Ref. [22]. Copyright 2022, American Chemical Society

Fig. 7

Reproduced with permission from Ref. [41]. Copyright 2021, Nature Publishing Group

Fig. 8

Reproduced with permission from Ref. [126]. Copyright 2022, The Electrochemical Society; d AG+SBR, e NG+SBR and f NG+PAA (SBR: styrene butadiene rubber; PAA: polyacrylic acid) electrode cells under different preload force. Reproduced with permission from Ref. [127]. Copyright 2021, Elsevier; g–i SEM cross sections with magnifications of 1000 × . Reproduced with permission from Ref. [128]. Copyright 2022, Elsevier

Fig. 9

Reproduced with permission from Ref. [136]. Copyright 2022, Elsevier. SEM images of cross-sectional morphology of Li anode: g bare Li, h normal charging, and i 1:1 pulsed charging. Reproduced with permission from Ref. [139]. Copyright 2022, American Chemical Society

Fig. 10

Reproduced with permission from Ref. [143]. Copyright 2022, Elsevier

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Acknowledgements

This work was financially supported by the National Natural Science Fund of China (Nos. 12172118 and 12172205), the Research Program of Local Science Research Development under the Guidance of Central (No. 216Z4402G) and Science Research Project of Hebei Education Department (No. JZX2023004). We also acknowledge support from ‘‘Yuanguang” Scholar Program of Hebei University of Technology.

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  1. School of Mechanical Engineering, School of Materials Science and Engineering, Hebei University of Technology, Tianjin, 300401, China

    Shi-Kang Wang, Shuai Wu, Hassanien Gomaa, Cui-Hua An, Qi-Bo Deng & Ning Hu

  2. Shanghai Key Laboratory of Mechanics in Energy Engineering, Shanghai, 200444, China

    Yi-Cheng Song & Qi-Bo Deng

  3. State Key Laboratory of Reliability and Intelligence Electrical Equipment, Key Laboratory of Advanced Intelligent Protective Equipment Technology, Ministry of Education, Hebei University of Technology, Tianjin, 300130, China

    Ning Hu

  4. Tianjin Key Laboratory of Power Transmission and Safety Technology for New Energy Vehicles, Tianjin, 300401, China

    Qi-Bo Deng

  5. Department of Chemistry, Faculty of Science, Al-Azhar University, Assiut, 71524, Egypt

    Hassanien Gomaa

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Wang, SK., Wu, S., Song, YC. et al. Regulating electrochemical performances of lithium battery by external physical field. Rare Met. 43, 2391–2417 (2024). https://doi.org/10.1007/s12598-024-02645-5

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