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Application of UiO-66 and its composites for remediation and resource recovery of typical environmental contaminants: a review

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Abstract

UiO-66 series metal–organic framework materials (MOFs) are typical porous materials assembled by Zr4+ with a large mass-to-nucleus ratio and terephthalic acid ligands, which form tetrahedral and octahedral cages arranged in a periodic triangular window pattern. Due to the strong interaction between Zr and O, UiO-66 series MOFs exhibit high thermal stability, structural stability, and chemical stability. This article mainly reviews the applications of UiO-66 and its composites in adsorption, photocatalysis, and resource utilization, while exploring the harm of pollutants to human health and the environment. In the first part, the differences in adsorption and removal mechanisms of liquid organic pollutants, heavy metals, and volatile organic compounds (VOCs) are investigated. The results show that organic pollutants are mainly removed by physical adsorption, electrostatic interactions, hydrogen bonding, and π-π interactions, while heavy metals are mainly removed by chemical adsorption, electrostatic interactions, reduction, and chelation. VOCs are mainly removed by the pore volume and pore size structure of the material. Heterojunction catalysis can achieve non-toxic treatment of pollutants, and this study mainly focuses on UiO-based composite materials constructed by strategies such as semiconductor composites, ion doping, and metal/dye encapsulation. In the second part, the synergistic effect between the components of UiO-based composite materials promotes the oriented and rapid separation and transfer of carriers at the material interface, thereby promoting the generation of active species such as h+, ·O2− and ·OH, and achieving rapid degradation of pollutants and detoxification of heavy metals. In the third part, heterojunctions can realize the resource utilization of pollutants in water and air, producing energy-type substances such as hydrogen and methanol while solving environmental problems. In addition, this article also summarizes the harm of common typical pollutants to the environment and human health. Finally, the development prospects and unresolved problems of UiO-66-based materials in water remediation, gas purification, and environmental resource utilization are reviewed.

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摘要

UiO-66系列MOFs是具有较大质核比的Zr4+离子与同为硬酸的对苯二甲酸配体自组装得到的具有由四面体笼和八面体笼通过三角窗口周期排列典型微孔材料。由于金属节点中的Zr与配体中的O具有较强的相互作用，进而UiO-66系列MOFs具有较高的热稳定性、结构稳定性和化学稳定性。本文主要综述了UiO-66及其复合材料在污染物吸附、光催化及资源化利用方面的应用，同时探究了污染物对人体和环境的危害。第一部分主要探究了液相有机污染物、重金属和气相污染物吸附去除机制的差异，结果表明，液相污染物主要依赖物理吸附、静电、氢键、π-π相互作用吸附去除，重金属主要依赖于化学吸附、静电、还原和螯合作用去除，然而气相污染物主要依赖于材料的孔容和孔径结构去除。异质结催化可实现污染物的无毒害处理，本研究主要关注半导体复合、离子掺杂、金属/染料封装等策略构筑的UiO基复合材料。第二部分，由于UiO基复合材料组分间的协同效应，促使载流子在材料界面定向快速分离和转移，促进h+、·O2-和·OH等活性物种的生成，进而实现污染物的快速降解及重金属的削毒。第三部分，异质结可将水体和大气中的污染物实现资源化，在解决环境问题的同时，产生氢气、甲醇等能源型物质。此外，本文也综述了常见典型污染物对环境和人体的危害。最后，本文综述了UiO-66基材料在水体修复、气体净化及环境资源化方面发展的前景及未解决的问题。

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Acknowledgements

This work was financially supported by the National Natural Science Foundation of China (No. 22206080), Zhongyuan Yingcai Jihua (No. ZYYCYU202012183), Henan Key Scientific Research Projects (No. 23B610004), Henan Postdoctoral Foundation (No. 202003027), the Natural Science Youth Fund of Henan Province (Nos. 202300410034 and 232300420336), the Natural Science Foundation of Jiangsu (No. SBK2022041070), the Science and Technology Project of Henan Province (No. 232102321050), the International Science and Technology Cooperation Projects of Henan Province (No. 232102521009), the Young Teacher Foundation of Henan University of Urban Construction (No. YCJQNGGJS202306), China Postdoctoral Science Foundation (No. 2021M701099), the Academic Leader of Henan Institute of Urban Construction (No. YCJXSJSDTR202204), the Science and Technology Major Special of Pingdingshan (No. 2021ZD03), the Key University Scientific Research Project of Henan Province (No. 22A610007) and the Doctoral Research Start-up Project of Henan University of Urban Construction (No. 990/K-Q2022016).

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  1. School Infirmary, Henan University of Urban Construction, Pingdingshan, 467036, China

    Hui-Min Zhang

  2. Faculty of Environmental and Municipal Engineering, Henan Key Laboratory of Water Pollution Control and Rehabilitation Technology, Key Laboratory of Carbon Emission Reduction and Combined Air Pollution Control Technology, Henan University of Urban Construction, Pingdingshan, 467036, China

    Yun-Long Wang, Xin-Feng Zhu, Zhen-Zhen Huang, Dan-Dan Pang, Kai Wang, Chao-Hai Wang, Zhong-Xian Song, Shi-Qiang Yin, Lin-Lin Chang & Jin-Hui Zhang

  3. The Key Lab of Pollution Control and Ecosystem Restoration in Industry Clusters, Ministry of Education, Guangzhou Higher Education Mega Centre, South China University of Technology, Guangzhou, 510006, China

    Jin-Hui Zhang

  4. School of Resources & Environment, Collaborative Innovation Center of Coalbed Methane and Shale Gas for Central Plains Economic Region, Henan Polytechnic University, Jiaozuo, 454003, China

    Kai Wang

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Zhang, HM., Wang, YL., Zhu, XF. et al. Application of UiO-66 and its composites for remediation and resource recovery of typical environmental contaminants: a review. Rare Met. 43, 2498–2526 (2024). https://doi.org/10.1007/s12598-023-02591-8

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  • DOI: https://doi.org/10.1007/s12598-023-02591-8

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