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Rational design of metal selenides nanomaterials for alkali metal ion (Li+/Na+/K+) batteries: current status and perspectives

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Abstract

Recently, metal selenides have obtained widespread attention as electrode materials for alkali (Li+/Na+/K+) batteries due to their promising theoretical capacity and mechanism. Nevertheless, metal selenides, similar to metal oxides and sulfides, also suffer from severe volume explosion during repeated charge/discharge processes, which results in the structure collapse and the following pulverization of electrode materials. Hence, it leads to poor cycle stability and influencing their further application. In order to solve these issues, some special strategies, including elemental doping, coupling with carbon materials, synthesis of the bimetal selenides with heterostructure, etc., have been gradually applied to design novel electrode materials with outstanding electrochemical performance. Herein, the recent research progress on metal selenides as anodes for alkali ion batteries is summarized, including the regulation of crystal structure, synthesis strategies, modification methods, and electrochemical mechanisms and kinetics. Besides, the challenges of metal selenides and the perspective for future electrode material design are proposed. It is hoped to pave a way for the development of metal selenide electrode materials for the potential applications for alkali metal ion (Li+/Na+/K+) batteries.

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概要

近年来, 金属硒化物作为碱性电池(锂/钠/钾离子电池)电极材料, 因其具有良好的理论容量和作用机理而受到广泛关注.然而, 与金属氧化物和硫化物类似, 金属硒化物在反复充放电过程中也会发生严重的体积膨胀, 导致结构崩塌和粉碎.因 此,导致循环稳定性差, 影响其进一步应用.为了解决这些问题, 一些特殊的策略, 包括元素掺杂, 与碳材料偶联, 合成异质结构双金属硒化物等, 逐渐被应用于设计具有优异电化学性能的新型电极材料. 本文综述了近年来金属硒化物作为碱离子电池负极的研究进展,包括晶体结构调控, 合成策略, 改性方法, 电化学机理和动力学等.此外, 还提出了金属硒化物面临的挑战和未来电极材料设计的展望.希望为开发碱金属离子(Li+/Na+/K+)电池中潜在应用的金属硒化电极材料提供建议.

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Scheme 1
Fig. 1
Fig. 2

Reproduced with permission from Ref. [34]. Copyright 2018, American Chemical Society. h Synthesis process and rate-mediated crack reassembly formation mechanism. Reproduced with permission from Ref. [36]. Copyright 2019, Royal Society of Chemistry. i Synthetic procedure of FexSey@CN composites. Reproduced with permission from Ref. [41]. Copyright 2022, Royal Society of Chemistry

Fig. 3
Fig. 4
Fig. 5

Reproduced with permission from Ref. [64]. Copyright 2018, American Chemical Society. DOS plots of e CoSe2@C and f CoSe2@NC heterostructures; g adsorption energy of CoSe2@C and CoSe2@NC for Na+. Reproduced with permission from Ref. [69]. Copyright 2022, Royal Society of Chemistry

Fig. 6

Reproduced with permission from Ref. [75]. Copyright 2020, Elsevier B.V. h, i TEM images of NiCoSe/NC; j ex situ XRD patterns of NiCoSe@NC electrode during the first charge/discharge process. Reproduced with permission from Ref. [92]. Copyright 2022, Elsevier B.V. k Synthesis; l cycling stability of NSG composite at 1 A·g−1. Reproduced with permission from Ref. [93]. Copyright 2020, Elsevier B.V

Fig. 7
Fig. 8
Fig. 9

Reproduced with permission from Ref. [130]. Copyright 2018. Royal Society of Chemistry. d In-situ XRD patterns; e sodium storage mechanism for NiN-Sb2Se3@C electrode. Reproduced with permission from Ref. [142]. Copyright 2022. Wiley–VCH GmbH

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Acknowledgements

This work was financially supported by the National Natural Science Foundation of China (Nos. 51563002 and 52101243), the “100-level” Innovative Talents Project of Guizhou Province, China (No. [2016] 5653), the Natural Science Foundation of Guangdong Province (No. 2020A1515010886), and the Science and Technology Planning Project of Guangzhou (No. 202102010373).

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  1. College of Materials Science and Metallurgy Engineering, Guizhou University, Guiyang, 550025, China

    Rui Sun, Feng Xu, Cai-Hong Wang, Sheng-Jun Lu, Yu-Fei Zhang & Hao-Sen Fan

  2. School of Chemistry and Chemical Engineering, Guangzhou University, Guangzhou, 510006, China

    Hao-Sen Fan

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Sun, R., Xu, F., Wang, CH. et al. Rational design of metal selenides nanomaterials for alkali metal ion (Li+/Na+/K+) batteries: current status and perspectives. Rare Met. 43, 1906–1931 (2024). https://doi.org/10.1007/s12598-023-02563-y

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