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Green and Facile Fabrication of Thermal Superamphiphobic Nanofibrillated-cellulose/Chitosan/OTS Composites Through Mechano-Chemical Method

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Abstract

Superamphiphobic nanofibrillated-cellulose/chitosan/OTS composite was successfully prepared through mechano-chemical method pretreatment, freeze-thaw treatment, regeneration and freeze drying. The morphology, structure, chemical components, element variation and thermally stable property of the prepared nanofibrillated-cellulose/chitosan/OTS composite was characterized by scanning electron microscopy (SEM), Fourier transform infrared spectroscopy (FT-IR) and X-ray photoelectron spectroscopy (XPS) thermogravimetric/differential thermogravimetric (TG-DTG). Results indicate that micro/nano-biomimetic structures of the prepared nanofibrillated-cellulose/chitosan/OTS composite were alike to the micromorphology of a lotus leaf. As-prepared nanofibrillated-cellulose/chitosan/OTS composite not only exhibited superhydrophobic performance with a water contact angle (WCA) of 154 ° and the surface exhibits self-cleaning ability with sliding angle of 6 °, but also had excellent superoleophobic behavior. What’s more, the nanofibrillated-cellulose/chitosan/OTS composite is resistant to high-temperature-humidity-resistant, outperforming original wood fiber.

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Acknowledgements

This study became financially supported by the National Natural Science Foundation of China (No. 31971586 and No. 31570555).

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Authors and Affiliations

  1. Key Laboratory of Wood Adhesives and Glued Products, Southwest Forestry University, Kunming, Yunnan, 650224, China

    Yushan Yang, Huajie Shen & Jian Qiu

  2. Korea Blockchain Institute, Seoul, 06651, Korea

    Liang Shan

  3. School of Material Science and Engineering, Southwest Forestry University, Kunming, Yunnan, 650224, China

    Yushan Yang, Huajie Shen & Jian Qiu

  4. Key Laboratory of Forest Resources Conservation and Utilization in the Southwest Mountains of China, Southwest Forestry University, Kunming, Yunnan, 650224, China

    Yushan Yang, Huajie Shen & Jian Qiu

Authors
  1. Yushan Yang
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  2. Liang Shan
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  3. Huajie Shen
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  4. Jian Qiu
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Correspondence to Jian Qiu.

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Yang, Y., Shan, L., Shen, H. et al. Green and Facile Fabrication of Thermal Superamphiphobic Nanofibrillated-cellulose/Chitosan/OTS Composites Through Mechano-Chemical Method. Fibers Polym 22, 1407–1415 (2021). https://doi.org/10.1007/s12221-021-0221-9

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  • DOI: https://doi.org/10.1007/s12221-021-0221-9

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