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Influencing factors and mechanism of CO2 adsorption capacity of FA-based carbon sequestration materials

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Abstract

Carbon dioxide mineral carbonisation is a means to achieve permanent carbon dioxide storage, this paper to solid waste materials as the main raw material to prepare fly ash-based carbon dioxide storage materials. Through the design of carbon dioxide adsorption experimental setup to study the main factors affecting the adsorption capacity of the fly ash-based storage materials, the experimental results show that, the fly ash mass fraction decreased from 90 to 10%, the water-cement ratio increased from 0.4 to 0.8 when the CO2 adsorption of fly ash-based materials increased by 82% and 30%, respectively. The effect of strong alkali on CO2 adsorption capacity was also investigated in this paper, and the results showed that the CO2 adsorption of the fly ash-based material sample with 10 ml NaOH added increased by 197% compared with that of the sample with 5 ml NaOH added, whereas the adsorption amount was reduced by 85% when 25 ml NaOH was added instead, which was attributed to the accelerated hydration process of the material due to the excessive alkalinity that consumed the calcium and magnesium ions in the material, and at the same time the production of hydration products hindered the transport of CO2 within the material, which led to a decrease in CO2 adsorption.

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Funding

This work was supported by the National Natural Science Foundation of China (grant numbers 52274212, 51934004, and 51704187); Shandong Natural Science Foundation, China (grant numbers ZR2022ME108 and ZR2019QEE029); Shandong Province Key Research and Development Plan, China (grant number 2019GSF109068); and the Science and technology support plan for Youth Innovation of colleges and universities in Shandong Province (grant number 2019KJH006).

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Authors and Affiliations

  1. College of Safety and Environment Engineering, Shandong University of Science and Technology, Qingdao, 266590, People’s Republic of China

    Lulu Sun, Shoulei Duan, Shuaihu Zhang, Weimin Cheng, Gang Wang & Xiaoqiang Cao

  2. State Key Laboratory of Mining Disaster Prevention and Control Co-founded by Shandong Province and the Ministry of Science and Technology, Shandong University of Science and Technology, Qingdao, 266590, People’s Republic of China

    Lulu Sun, Weimin Cheng & Gang Wang

  3. School of Safety Engineering, China University of Mining and Technology, Xuzhou, 221116, Jiangsu, People’s Republic of China

    Lulu Sun

Authors
  1. Lulu Sun
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  2. Shoulei Duan
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  3. Shuaihu Zhang
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  4. Weimin Cheng
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  5. Gang Wang
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  6. Xiaoqiang Cao
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Contributions

Writing—original draft preparation: Shoulei Duan; writing—review and editing: Lulu Sun; methodology: Lulu Sun; conceptualization: Shuaihu Zhang and Weimin Cheng; and supervision: Gang Wang and Xiaoqiang Cao.

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Correspondence to Lulu Sun.

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Sun, L., Duan, S., Zhang, S. et al. Influencing factors and mechanism of CO2 adsorption capacity of FA-based carbon sequestration materials. Environ Sci Pollut Res 30, 117225–117237 (2023). https://doi.org/10.1007/s11356-023-30350-w

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