Skip to main content
Log in

Enhancement of optical and mechanical properties of sodium silicate glasses using zirconia

  • Published:
Optical and Quantum Electronics Aims and scope Submit manuscript

Abstract

Ternary glass system with the composition of 50Na2O–(50–x) SiO2x ZrO2, (0 ≤ x ≤ 20 mol %) has been prepared by melt quenching method. The structure changes of these glasses are studied by FT-IR spectra. The mechanical properties have been related to the results of FT-IR spectra. X-ray diffractograms showing the amorphous nature of these glasses. The mechanical properties of these glasses are studied and their elastic-moduli have been estimated. It was noted that the elastic-moduli, density and some physical properties of these samples are increased. Optical feature spectra are recorded at room temperature. The dispersion parameters as refractive index (n) and extinction coefficient (k) are determined in the wavelength range of 300–2500 nm. Energy band gap and Urbach energy with indirect allowed transitions are estimated using Tauc model. The dielectric constant in term of real and imaginary parts are investigated. Other physical parameters like skin depth, cut-off wavelength, dissipation factor, optical and electrical conductivities are calculated as well.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6
Fig. 7
Fig. 8
Fig. 9
Fig. 10
Fig. 11
Fig. 12
Fig. 13
Fig. 14
Fig.15
Fig. 16
Fig. 17
Fig. 18
Fig. 19
Fig. 20
Fig. 21
Fig. 22

Similar content being viewed by others

References

  • Abdel Wahab, E.A., Shaaban, K.S., Elsaman, R., Yousef, E.S.: Radiation shielding and physical properties of lead borate glass-doped ZrO2 nanoparticles. Appl. Phys. A 125(12), 869 (2019). https://doi.org/10.1007/s00339-019-3166-8

    Article  ADS  Google Scholar 

  • Abdelghany, A.M., El Batal, F.H., El Batal, H.A., Ezz El Din, F.M.: Optical and FTIR structural studies of CoO-doped sodium borate, sodium silicate and sodium phosphate glasses and effects of gamma irradiation-a comparative study. J. Mol. Struct. 1074, 503–510 (2014)

    ADS  Google Scholar 

  • Abdullah, A.Q.: Surface and volume energy loss, optical conductivity of Rhodamine 6G dye (R6G). Chem. Mater. Res 56, 63 (2013). https://doi.org/10.1007/s00339-019-3264-7

  • Abouhaswa, A.S., Al-Buriahi, M.S., Chalermpon, M., Rammah, Y.S.: Influence of ZrO2 on gamma shielding properties of lead borate glasses. Appl. Phys. A 126(1), 78 (2020)

    ADS  Google Scholar 

  • Alharbi, T., Mohamed, H.F.M., Saddeek, Y.B., El-Haseib, A.Y., Shaaban, K.S.: Study of the TiO2 effect on the heavy metals oxides borosilicate glasses structure using gamma-ray spectroscopy and positron annihilation technique. Rad. Phys. Chem. 164, 108345 (2019)

    Google Scholar 

  • Azooz, M.A., Saddeek, Y.B., Aly, K.A., Shaaban, K.S., Mokhtar, H.M.: Optical, infrared spectral and mechanical investigations of CeO2-doped borosilicate glasses containing Bi2O3 and TeO2. J. Inor. Organometal. Polym. Mater. 29, 1680–1687 (2019). https://doi.org/10.1007/s10904-019-01130-2

    Article  Google Scholar 

  • Bishay, A., Maghrabi, C.: Properties of bismuth glasses in relation to structure. Phys. Chem. Glasses 10, 1–11 (1969)

    Google Scholar 

  • Bollot, J.P., Colomban, P., Blanchard, N.: Formation of superionic gels and glasses by low temperature chemical polytenization. Solid State Ion 9–10, 639–644 (1983)

    Google Scholar 

  • Bollot, J.P., Colomban, P., Blanchard, N.: Naslcon amorphous to crystalline compounds. Solid State Ion 18–19, 974–980 (1986)

    Google Scholar 

  • Chandrakala, C., Reddy, A.S.S., Jedryka, J., et al.: Third-order nonlinear optical features of zirconia-added lead silicate glass ceramics embedded with Pb2Fe2O5 perovskite crystal phases and role of Fe ions. Appl. Phys. A 126, 413 (2020). https://doi.org/10.1007/s00339-020-03570-x

    Article  ADS  Google Scholar 

  • Efimov, A.M.: Vibrational spectra, related properties, and structure of inorganic glasses. J. Non-Cryst. Solids 253(1–3), 95–118 (1999)

    ADS  Google Scholar 

  • El Radaf, I., et al.: Influence of spray time on the optical and electrical properties of CoNi2S4 thin films. Mater. Res. Express 5(4), 046406 (2018). https://doi.org/10.1088/2053-1591/aaba0a

    ADS  Google Scholar 

  • ElBatal, F.H., Abdelghany, A.M., ElBatal, H.A.: Characterization by combined optical and FT infrared spectra of 3d-transition metal ions doped-bismuth silicate glasses and effects of gamma irradiation. Spectrochim. Acta Part A Mol. Biomol. Spectrosc. 122, 461–468 (2014)

    ADS  Google Scholar 

  • El-Nagar, H., Abd El-sadek, M.S., Ezzeldien, M.: Structural analysis, optical and mechanical properties of TixZr1−xO2 nanoparticles synthesized by modified co-precipitation route. Appl. Phys. A 126, 126 (2020). https://doi.org/10.1007/s00339-019-3272-7

    Article  ADS  Google Scholar 

  • Eloy, J.F.: Power laser national Sch. Phy. Wiley, France (1984)

    Google Scholar 

  • Fisher, J.G., James, P.F., Parker, J.M.: Soda lime zirconia silicate glasses as prospective hosts for zirconia-containing radioactive wastes. J. Non-Cryst. Solids 351, 623–631 (2005)

    ADS  Google Scholar 

  • Fouad, S., et al.: Multifunctional CZTS thin films: structural, optoelectrical, electrical and photovoltaic properties. J Alloys Compd 757, 124–133 (2018)

    Google Scholar 

  • Girisun, T.S., Dhanuskodi, S.: Linear and nonlinear optical properties of tris thiourea zinc sulphate single crystals. Cryst. Res. Technol. J. Exp. Ind. Crystallogr. 44(12), 1297–1302 (2009)

    Google Scholar 

  • Hoj, J.W., Engell, J.: Superconducting glass in the system Na2O–ZrO2–SiO2–P2O5. Mater. Sci. Eng. B14, 231–234 (1992)

    Google Scholar 

  • Hrma, P.: High temperature viscosity of commercial glasses. Ceram.-Silikáty 50, 57–66 (2006)

    Google Scholar 

  • Karell, R., Kraxner, J., Chromčíková, M.: Properties of selected zirconia containing silicate glasses. Ceram. Silik. 50, 78–82 (2006)

    Google Scholar 

  • Kennedy, E., Sachin, B.S., Ramachandra, M., Niranjan, C.A., Sriraman, N., Kumar, V., Jain, S., Sathya Narayanan, N.: Effect of ZrO2 nano-particles on mechanical and corrosion behaviour of Al2024 alloy. J. Mat. Pr. 1, 1 (2020). https://doi.org/10.1016/j.matpr.2020.06.194

    Article  Google Scholar 

  • Khalil, E.M.A., Elbatal, F.H., Hamdy, Y.M., Zidan, H.M., Aziz, M.S., Abdelghany, A.M.: Infrared absorption spectra of transition metals-doped soda lime silica glasses. Phys. B Condens. Matte 405(5), 1294–1300 (2010)

    ADS  Google Scholar 

  • Khalil, E.M.A., El-Batal, F.H., Hamdy, Y.M., Zidan, H.M., Aziz, M.S., Abdelghany, A.M.: UV-visible and IR spectroscopic studies of gamma irradiated transition metal doped lead silicate glasses. Silicon 2(1), 49–60 (2010)

    Google Scholar 

  • Khan, B.S., Kaur, G., Singh, K.: Effect of ZrO2 on dielectric, optical and structural properties of yttrium calcium borosilicate glasses. Ceram. Int. 43, 722–727 (2017)

    Google Scholar 

  • Lu, X., Deng, L., Kerisit, S., Du, J.: Structural role of ZrO2 and its impact on properties of boroaluminosilicate nuclear waste glasses. Npj Mater. Degrad. 2(1), 1–10 (2018a)

    Google Scholar 

  • Lu, X., Deng, L., Du, J.: Efect of ZrO2 on the structure and properties of soda-lime silicate glasses from molecular dynamics simulations. J. Non-Cryst. Solids 491, 41–150 (2018)

    Google Scholar 

  • Lu, X., Deng, L., Kerisit, S., Du, J.: Structural role of ZrO2 and its impact on properties of boroaluminosilicate nuclear waste glasses. Npj Mater. Degrad. (2018b). https://doi.org/10.1038/s41529-018-0041-6

    Article  Google Scholar 

  • Makishima, A., Mackenzie, J.D.: Direct calculation of Young's moidulus of glass. J. Non-Cryst. Solids 12(1), 35–45 (1973)

    ADS  Google Scholar 

  • Makishima, A., Mackenzie, J.D.: Calculation of bulk modulus, shear modulus and Poisson's ratio of glass. J. Non-cryst. Solids 17(2), 147–157 (1975)

    ADS  Google Scholar 

  • Ming-Wei, Lu, Kun-Lin, Lin, Chien-Cheng, Lin: Investigation of the interactions between titanium and calcium zirconium oxide (CaZrO3) ceramics modified with alumina. Process. Appl. Ceram. 13(1), 79–88 (2019). https://doi.org/10.2298/PAC1901079L

    Article  Google Scholar 

  • Moustafa, M.G., Hassaan, M.Y.: Optical and dielectric properties of transparent ZrO2–TiO2–Li2B4O7 glass system. J. Alloys Compd. (2017). https://doi.org/10.1016/j.jallcom.2017.03.192

    Article  Google Scholar 

  • Rahmani, K., Majzoobi, G.H., Sadooghi, A., Kashfi, M.: Mechanical and physical characterization of Mg-TiO2 and Mg-ZrO2 nanocomposites produced by hot-pressing. Mater. Chem. Phys. 246, 122844 (2020). https://doi.org/10.1016/j.matchemphys.2020.122844

    Article  Google Scholar 

  • Reddy, A.S.S., Kityk, I.V., Kumar, V.R., Jedryka, J., Ozga, K., Venkatramaiah, N., Veeraiah, N.: Third order nonlinear optical effects of ZnO–ZrO2–B2O3 glass ceramics embedded with ZnZrO3 perovskite crystal phases. J. Mater. Sci. Mater. Electron. 28(21), 16403–16414 (2017). https://doi.org/10.1007/s10854-017-7551-9

    Google Scholar 

  • Salah, M., Azizi, S., Boukhachem, A.W., Khaldi, C., Amlouk, M., Lamloumi, J.: Structural, morphological, optical and photodetector properties of sprayed Li-doped ZnO thin films. J. Mater. Sci. 52, 10439–10454 (2017). https://doi.org/10.1007/s10853-017-1218-z

    Article  ADS  Google Scholar 

  • Shaaban, K.S., Saddeek, Y.B.: Effect of MoO3 content on structural, thermal, mechanical and optical properties of (B2O3–SiO2–Bi2O3–Na2O–Fe2O3) glass system. Silicon 9(5), 785–793 (2017). https://doi.org/10.1007/s12633-017-9558-5

    Google Scholar 

  • Shaaban, K.H.S., Saddeek, Y., Aly, K.: Physical properties of pseudo quaternary Na2B4O7–SiO2–MoO3–Dy2O3 glasses. Ceram. Int. 44, 3862–3867 (2018)

    Google Scholar 

  • Shaaban, K.S., El-Maaref, A.A., Abdelawwad, M., Saddeek, Y.B., Wilke, H., Hillmer, H.: Spectroscopic properties and Judd-Ofelt analysis of Dy3+ ions in molybdenum borosilicate glasses. J. Lumines. 196, 477–484 (2018). https://doi.org/10.1016/j.jlumin.2017.12.041

    Article  ADS  Google Scholar 

  • Shaaban, K.S., Wahab, E.A.A., Shaaban, E.R., Yousef, E.S., Mahmoud, S.A.: Electronic polarizability, optical basicity, thermal, mechanical and optical investigations of (65B2O3–30Li2O–5Al2O3) glasses doped with titanate. J. Electron. Mater. 49, 2040–2049 (2019). https://doi.org/10.1007/s11664-019-07889-x

    Article  ADS  Google Scholar 

  • Shaaban, K.S., Abd-Allah, W.M., Saddeek, Y.B.: Gamma rays interactions with CdO-doped lead silicate glasses. Opt. Quantum Electron. (2020a). https://doi.org/10.1007/s11082-019-2094-3

    Article  Google Scholar 

  • Shaaban, K.S., Abd-Allah, W.M., Saddeek, Y.B.: Gamma rays interactions with CdO-doped lead silicate glasses. Opt. Quant. Electron. 52, 3 (2020b). https://doi.org/10.1007/s11082-019-2094-3

    Article  Google Scholar 

  • Shakra, A., Atyia, H., Fadel, M.: Single oscillator parameters and optical properties for ZnSnSb2 chalcopyrite in thin film form. J. Alloys Compd. 763, 983–989 (2018)

    Google Scholar 

  • Susman, S., Delbeq, C.J., McMlllan, J.A., Roche, M.F.: Nasiglas a new Vitreous electrolyte. Solid State Ion 9–10, 667–674 (1983)

    Google Scholar 

  • Tsurita, Y., Wada, K.: Preparation of the porous supports with SiO2–ZrO2–Na2O composition. Mater. Res. Soc. 180, 361–364 (1990)

    Google Scholar 

  • Veit, U., Rüssel, C.: Elastic properties of quaternary glasses in the MgO–CaO–Al2O3–SiO2 system: modelling versus measurement. J. Mater. Sci. 52, 8159–8175 (2017). https://doi.org/10.1007/s11082-019-2094-3

    Article  ADS  Google Scholar 

  • Vogel, W.: Glass chemistry. Springer, Berlin (1994)

    Google Scholar 

  • Wahab, E.A.A., Shaaban, K.S.: Effects of SnO2 on spectroscopic properties of borosilicate glasses before and after plasma treatment and its mechanical properties. Mater. Res. Express 5(2), 025207 (2018)

    ADS  Google Scholar 

  • Wang, M.T., Cheng, J.Z., Li, M., He, F.: Structure and properties of soda lime silicate glass doped with rare earth. Phys. B Condens. Matter 406, 187–191 (2011)

    ADS  Google Scholar 

  • Zaka, H., Parditka, B., Erdelyi, Z., Atyia, H.E., Sharma, P., Fouad, S.S.: Investigation of dispersion parameters, dielectric properties and opto–electrical parameters Of ZnO thin film grown by ALD. Optik 203, 163933 (2019). https://doi.org/10.1016/j.ijleo.2019.163933

    Article  ADS  Google Scholar 

Download references

Acknowledgements

This work was support of King Khalid University, the Ministry of Education, and Kingdom of Saudi Arabia for this research through a Grant (RCAMS/KKU/013/20) under research center for advanced material science.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to E. A. Abdel Wahab.

Additional information

Publisher's Note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Abdel Wahab, E.A., Shaaban, K.S. & Yousef, E.S. Enhancement of optical and mechanical properties of sodium silicate glasses using zirconia. Opt Quant Electron 52, 458 (2020). https://doi.org/10.1007/s11082-020-02575-3

Download citation

  • Received:

  • Accepted:

  • Published:

  • DOI: https://doi.org/10.1007/s11082-020-02575-3

Keywords

Navigation