Abstract
Reaction between silver salt and conjugational N-hetrocyclic carboxylic acid with the presence of bipyridyl skeletons auxiliary ligand afforded a d10 metal polymer namely [(ddpp)Ag(bipy) (1)] (ddpp = 2, 5-di(2′,4′-dicarboxylphenyl)pyridine, bipy = 4,4′-bipyridine). It was characterized by elements analysis, infrared spectroscopy, single crystal X-ray diffraction and thermogravimetry studying. For the polymer 1, silver centers are three coordinated geometry with an ON2 donor set provided by ddpp and bipy. The polymer 1 is built from 1-D alternative/zig-zag chain, as the secondary building unit, and further stacks via hydrogen bonds which formed between two isophthalic moieties of ddpp ligands and weak interactions to generate a two-dimensional, 2D supramolecular layer. Moreover, the polymer 1 displays thermal stability in solid state and the luminescence behaviour is also investigated in a dimethyl sulphoxide solution at ambient temperature, and it also can be applied in design of sensors to detect of trace aluminum, zinc and calcium ion.
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Acknowledgments
This work was supported by the Ministry of Science and Technology of China (973 Project No. 2014CB660804), Natural Science Foundation of China (Nos. 21273101 and 21302082), Foundation for Science & Technology Innovation Talents in Henan province (Nos. 2014HASTIT014 and 164100510012), and Tackle Key Problem of Science and Technology Project of Henan Province (No. 142102310483).
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Bai, RF., Feng, X., Sun, YL. et al. A Silver–Organic Frameworks Based on Flexible-Aromatic Dicarboxylate and Bipyridinyl Skeletons Coligand: Crystal Structure and Luminescence Property. J Inorg Organomet Polym 26, 512–518 (2016). https://doi.org/10.1007/s10904-016-0358-y
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DOI: https://doi.org/10.1007/s10904-016-0358-y