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Temperature- and frequency-dependent dielectric and impedance spectroscopy of double perovskite oxide BiBa0.5Ag0.5Ni2O6 electronic material

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Abstract

The objective of this research is to develop perovskite compounds with electrical and dielectric properties that can be used in technological applications including magnetism, health, and electronic devices. Polycrystalline of double perovskite BiBa0.5Ag0.5Ni2O6 was successfully synthesized by sol–gel method. Preliminary X-ray investigation established at room temperature the formation of compound with rhombohedral structure of the R\(\overline{3 }\)C space group. The uniform grain distribution and chemical composition are predicted from the scanning electron microscope and energy-dispersive X-ray technique, which has an average grain size of 563 nm. Electrical properties electrical depends on temperature and frequency. Impedance spectroscopy and electrical modulus of the compound were analyzed by impedance analyzer in the range of frequency (1 kHz–1 MHz) and temperature (200–400 K) that confirmi non-Debye type of relaxation. In addition, the frequency dependence of the electrical conductivity of material prepared at different temperatures was studied using Jonscher’s law. The conduction and relaxation mechanisms remain same in the entire temperature range. From these results, it may be concluded that this compound may have extreme potential applications at different temperatures, for example in the electrical field, in capacitors.

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Authors and Affiliations

  1. Laboratoire de Physique des Matériaux, Faculté des Sciences de Sfax, Université de Sfax, B.P. 1171, 3000, Sfax, Tunisia

    K. Iben Nassar, F. Tayari, M. Slimi, N. Rammeh & A. Njeh

  2. Faculté des Sciences de Monastir, Université de Monastir, 5019, Monastir, Tunisia

    M. Slimi

  3. I3N-Aveiro, Department of Physics, University of Aveiro, 3810-193, Aveiro, Portugal

    S. Soreto Teixeira & M. P. F. Graça

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All authors take public responsibility for the content of the work submitted for review. The contributions of all authors must be described in the following manner: The authors confirm contribution to the paper as follows: study conception and design: KIN and FT; data collection: MS; analysis and interpretation of results: NR and AN; draft manuscript preparation: SST and MPFG. All authors reviewed the results and approved the final version of the manuscript. The author confirms sole responsibility for the following: study conception and design, data collection, analysis and interpretation of results, and manuscript preparation.

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Iben Nassar, K., Tayari, F., Slimi, M. et al. Temperature- and frequency-dependent dielectric and impedance spectroscopy of double perovskite oxide BiBa0.5Ag0.5Ni2O6 electronic material. J Mater Sci: Mater Electron 34, 216 (2023). https://doi.org/10.1007/s10854-022-09746-w

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