Abstract
This paper presents a depth study of structural, magnetic, magnetocaloric effects, and critical behavior of the La0.67Ba0.22Sr0.11Mn0.95Ni0.05O3 manganite compound. This material was synthesized using the solid–solid method. The crystallographic study shows that our compound crystallizes in a Pnma orthorhombic structure. The magnetic measurements M (T) show that our material has a transition from the ferromagnetic (FM) state to the paramagnetic (PM) state with increasing the temperature. Arrott plots (\(\mu_{0} \frac{H}{M}\) vs. M2) show that our compound presents a second-order transition. The magnetic entropy change (−∆SM) was determined by Relying on the Maxwell relation. The obtained results prove that our compound is a promising material which can be used in magnetic refrigeration application, operating over a wide range of temperatures. In addition, the magnetocaloric properties have been investigated using a phenomenological model. Finally, the estimated critical exponents values β, γ, and δ using through various techniques are comparable to those predicted by the mean-field model. The magnetic interaction nature in our samples is described by the calculation of exchange distance J(r).
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RC: Synthesis of materials, preparing original draft preparation, data analysis, graphics, formal analysis, investigation. ME: Mentor, Conceptualization, Data curation, Investigation, Writing, modification & Editing, language editing, manuscript submission. EKH: Data curation and analysis, Draft modification, Investigation, final analysis. RM: Data analysis, graph modification, writing, and editing draft. RJ: Investigation, Draft modification, writing review, and editing.
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Chaabouni, R., Ellouze, M., Hlil, E.K. et al. Role of nickel substitution in the structural, magnetic properties, and magnetocaloric effect in La0.67Ba0.22Sr0.11Mn0.95Ni0.05O3 sample. J Mater Sci: Mater Electron 33, 23524–23541 (2022). https://doi.org/10.1007/s10854-022-09113-9
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DOI: https://doi.org/10.1007/s10854-022-09113-9