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Enhanced large field-induced strain and energy storage properties of Sr0.6La0.2Ba0.1TiO3-modified Bi0.5Na0.5TiO3 relaxor ceramics

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Abstract

Dielectric materials especially relaxor ferroelectrics with giant strain and super-high energy density have received substantial attentions. Bi0.5Na0.5TiO3 (BNT)-based ceramics as one of the typical relaxor ferroelectric materials have been extensively explored for their distinctive performance. Here, lead-free (1−x)Na0.5Bi0.5TiO3–xSr0.6La0.2Ba0.1TiO3 (BNT–SLBT) ceramics were designed and prepared by the solid-state reaction method. A large strain response of 0.470% and huge piezoelectric strain coefficient of 600 pm/V were achieved in BNT–0.15SLBT relaxor, which were attributed to the relaxor-ferroelectric phase transition under stimulated electric field. The εr–T curve shows that with the increase of x content, the phase transition temperature moves to room temperature, which improves the energy storage performance. A super-high recoverable energy density Wrec of 3.18 J/cm3 and η of 82.8% under 250 kV/cm can be achieved in BNT–0.25SLBT ergodic relaxor. Moreover, the charge–discharge properties characterized by a high pulse discharge energy density (0.816 J/cm3), a rapid discharge duration (3 μs) and a power density (2.86 MW/cm3) are also observed in BNT–0.25SLBT ceramic. We provide a method for enhanced BNT-based ceramics with strain and energy storage in drive device or capacitor, facilitating the exploration of ceramic in the future.

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The data presented in this study are available upon request from the corresponding author.

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Acknowledgements

This work was supported by the Priority Academic Program Development (PAPD) of Jiangsu Higher Education Institutions.

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Authors and Affiliations

  1. The State Key Laboratory of Materials-Oriented Chemical Engineering, College of Materials Science and Engineering, Nanjing Tech University, Nanjing, 210009, China

    Tingting Ruan, Jie Yuan, Jing Xu, Yunfei Liu & Yinong Lyu

  2. Jiangsu National Synergetic Innovation Center for Advanced Materials (SICAM), Nanjing, China

    Tingting Ruan, Jie Yuan, Jing Xu, Yunfei Liu & Yinong Lyu

  3. Jiangsu Collaborative Innovation Center for Advanced Inorganic Function Composites, Nanjing, China

    Tingting Ruan, Jie Yuan, Jing Xu, Yunfei Liu & Yinong Lyu

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  1. Tingting Ruan
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Material preparation, data collection, and analysis were performed by JY and JX. The first draft of the manuscript was written by TR and all authors commented on previous versions of the manuscript. All authors read and approved the final manuscript.

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Correspondence to Yunfei Liu or Yinong Lyu.

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Ruan, T., Yuan, J., Xu, J. et al. Enhanced large field-induced strain and energy storage properties of Sr0.6La0.2Ba0.1TiO3-modified Bi0.5Na0.5TiO3 relaxor ceramics. J Mater Sci: Mater Electron 33, 15779–15790 (2022). https://doi.org/10.1007/s10854-022-08480-7

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