Abstract
We derive a macroscopic limit for a sharp interface version of a model proposed in Komura et al. (Langmuir 22:6771–6774, 2006) to investigate pattern formation due to competition of chemical and mechanical forces in biomembranes. We identify sub- and supercritical parameter regimes and show with the introduction of the autocorrelation function that the ground state energy leads to the isoperimetric problem in the subcritical regime, which is interpreted to not form fine scale patterns.
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1 Introduction
We consider the family of nonlocal isoperimetric problems
where \(u \in BV(\mathbb {T}^n, \{0,1\})\) and where \(\mathbb {T}^n\), \(n \ge 2\), is the n–dimensional unit flat torus. Here, \(\gamma > 0\) is a fixed parameter and \({\mathcal K}\) is a radially symmetric kernel with certain integrability conditions. For details, see Sect. 2. This class of problems appears in mathematical models of complex materials (such as biomembranes, see below), diblock copolymers (see [10, 25]) and cell motility (see [15]). We derive the limit \(\epsilon \rightarrow 0\) of the family of models \(E_{\gamma ,\epsilon }\) in the framework of \(\Gamma \)–convergence.
The family of functionals (1) is a more general sharp interface version of a model proposed in [28] for the investigation of structures which arise due to competing diffusive and mechanical forces. In particular, it is relevant for the modelling of formation of so called lipid rafts in cell membranes. These are complex nanostructures made up of lipids, proteins and cholesterol and are believed to be responsible for many biological phenomena such as transmembrane signaling and cellular homeostasis (see e.g. [29, 41, 45, 46]). A diffuse interface version of (1) was considered in [18] and can be formulated in terms of the order parameter (i.e. concentration of the chemical) u alone. The resulting energy is given by
where \(\Omega \) is a reference domain, W is a double well potential, \(\epsilon > 0\) and \(q < 1\). The solution operator \(({\textbf{1}} - \epsilon ^2\Delta )^{-1}\) is subject to Neumann boundary conditions. In [18] it was shown that for sufficiently small \(q > 0\), the family \({\mathcal F}_{q,\epsilon }\) \(\Gamma \)–converges to a constant multiple of the perimeter functional as \(\epsilon \rightarrow 0\) in the \(L^2\)–topology for a standard family of double well potentials (quadratic roots and quadratic growth). We comment on the relation between the diffuse and sharp interface model in Sect. 2 below.
In this article, we compute explicitely the \(\Gamma \)–limit of the family \(E_{\gamma ,\epsilon }\) under suitable assumptions on \({\mathcal K}\). We identify two parameter regimes (sub– and supercritical) with respect to \(\gamma \) and show that the limit problem is the isoperimetric problem (with modified prefactor) in the subcritical regime. In the supercritical regime, we show that minimising sequences of \(E_{\gamma ,\epsilon }\) always have unbounded perimeter.
Our main observation is that both the perimeter and the non-local term in (1) can be represented in terms of the (symmetrised) autocorrelation function
The formulation of the energy in terms of the autocorrelation function (Lemma 4.2) reveals that although the energy \(E_{\gamma ,\epsilon }\) is not linear in u, it is linear in terms of the autocorrelation function. For the proofs of the upper and lower bound we then can use properties of the autocorrelation function, which allows us to treat a large class of kernels.
Related literature The \(\Gamma \)–convergence of (1) has been considered in different setups. In [40], the author studied the stability of large mass minimisers of (1) in the whole space setting (see also [23, 34]) and established the \(\Gamma \)–convergence in the subcritical regime under more restrictive assumptions on the kernel \({\mathcal K}\), namely that \({\mathcal K}\ge 0\). The ideas involve sharp estimates of the non–local term by the classical perimeter for the lower bound and the pointwise convergence of the non–local term proved in [16] (see also [6]) for the upper bound. Apart from the different underlying geometry, we will relax the assumption of non–negativity of the kernel and recover their \(\Gamma \)–convergence result. We note that because of the aformentioned relaxation, two main challenges arise. First, we cannot directly use the results obtained in [16] for the upper bound (which implies that constant sequences can be used as recovery sequences) and instead utilise an approximation by polytopes. Second, the lower bound is more delicate since the control by the perimeter is achieved by estimating the integral of the difference quotient pointwise within the non-local term. If the kernel is allowed to have negative values, this estimate no longer holds. We deal with this issue by reformulating the energy in terms of the derivative of the autocorrelation function and shifting the control in terms of the perimeter to that derivative. This reformulation results in working with the integrated kernel (rather than the kernel itself) and allows us to relax the non-negativity.
The \(\Gamma \)–convergence of (1) in the special case where \({\mathcal K}\) is the solution to the Helmholtz equation on domains with different boundary conditions was considered in [33]. Their techniques are based on PDE arguments and they require the family of kernels to be solutions of the Helmholtz equation, wheras our techniques work for a larger class of kernels and are based on decay estimates. In particular, we recover the \(\Gamma \)–convergence result and are able to extend it to kernels which are given by \({\mathcal K}+ (-\Delta )^{\frac{s}{2}} {\mathcal K}= \delta _0\) for any \(1 < s \le 2\) (see the appendix).
Different classes of kernels in isoperimetric problems, where the non–local term has the same scaling as the local one, were considered e.g. in [8, 33, 38, 42]. Representing the energy in terms of the autocorrelation function and exploiting its fine properties has been proposed for a similar family of energies in [27]. There, the autocorrelation function was used to derive a second order expansion for the perimeter functional. However, the family of kernels is subject to different conditions and converge monotonically to a measurable function with certain integrability properties, wheras our family of kernels is assumed to form an approximation of the identity. Due to the highly singular nature of the considered kernels near the origin, our techniques require more information about the regularity of the autocorrelation function. This is not needed in [27] by the assumption of monotone convergence of the kernels. For this purpose, we show regularity properties of the autocorrelation function for polytopes, which are able to approximate any shape of finite perimeter (see (9)).
Lastly, non–local isoperimetric problems of the form (1) have also been considered in the mathematical literature in many different models, e.g. sharp interface variants of the Ohta-Kawasaki model where the non–local term is a Coulomb or Riesz type interaction (see [1, 2, 10, 12, 14, 21, 22, 25, 37]). We note that, contrary to our energy, in these models the non–local term does not have the same scaling as the perimeter functional.
Structure of the paper In Sect. 2 we present and discuss our main results. We also outline the proofs. In Sect. 3 we introduce the autocorrelation function and give some of its properties. In Sect. 4 we reformulate the energy in terms of the autocorrelation function and present the proofs of our main results, namely the compactness and \(\Gamma \)–convergence of \(E_{\gamma ,\epsilon }\) (see Theorem 2.1 and Theorem 2.3). In the Appendix we collect some further calculations.
Notation Throughout this paper, we write \(\mathbb {T}^n := \mathbb {R}^n/\mathbb {Z}^n\) for the n dimensional flat torus. Without distinction in notation, we identify \((0,1)^n\)–periodic functions in \(\mathbb {R}^n\) with functions on \(\mathbb {T}^n\). We denote \(|\Omega |\) for the Lebesgue measure of \(\Omega \). For \(r > 0\) and \(x \in \mathbb {R}^n\) we denote \(B_r(x) := \{y \in \mathbb {R}^n: |x - y| < r\}\) for the ball around x of radius r and the unit sphere by \({\mathbb {S}}^{n - 1} := \partial B_1(0)\). We denote \(\omega _n\) for the volume of the unit ball in \(\mathbb {R}^n\) and \(\sigma _n := n \omega _n\) for its surface area. We write \(A \lesssim B\) if there exists a universal constant \(C > 0\), such that \(A \le C B\). A function \(u \in L^1(\mathbb {T}^n)\) is said to be a function of bounded variation if
In this case, we write \(u \in BV(\mathbb {T}^n)\). We denote the perimeter functional \(P : L^1(\mathbb {T}^n) \longrightarrow [0,\infty ]\) by
2 Statement and discussion of the main results
In this section, we give the precise formulation of our setting and main results. Throughout this article, we assume \(n \in \mathbb {N}\), \(n \ge 2\). Since we are interested in the case of prescribed volume fraction, we introduce the class of admissible functions
for some fixed parameter \(0< \theta < 1\). We also fix the function \({\mathcal K}: \mathbb {R}^n \longrightarrow \mathbb {R}\) and define \({\mathcal K}_\epsilon (z) := \frac{1}{\epsilon ^n} {\mathcal K}(\frac{z}{\epsilon })\). We recall the energy functional
when \(u \in {\mathcal A}\), and \(E_{\gamma ,\epsilon }[u] = +\infty \) for all \(u \in L^1(\mathbb {T}^n) \setminus {\mathcal A}\). The kernel \({\mathcal K}\) is subject to the following conditions:
-
(H1)
\({\mathcal K}\) is radial.
-
(H2)
\( |z| \, {\mathcal K}(z) \in L^1(\mathbb {R}^n)\).
-
(H3)
\(\displaystyle \int _{\mathbb {R}^n\setminus B_r(0)} {\mathcal K}(z) \ dz \ge 0\) for all \(r > 0\).
By a slight abuse of notation we also write \({\mathcal K}(z) = {\mathcal K}(|z|)\). The imposed conditions (H1)–(H3) are different from the conditions imposed on the family of kernels considered in [16] (see also [40] and [33, Theorem 1.2]): although our family of kernels arises as \(L^1\)–dilates of \({\mathcal K}\), we relax the assumption of the non–negativity of \({\mathcal K}_\epsilon \) by (H3).
As the quantity \(E_{\gamma ,\epsilon }\) is the difference of two positive terms with the same scaling, uniform control of the energy of a sequence of shapes in general does not a priori lead to control of the perimeter. However, we identify the critical parameter
such that for \(0< \gamma < \gamma _{\textrm{crit}}\) the perimeter is controlled by the energy, while the perimeter is not controled for \(\gamma > \gamma _{\textrm{crit}}\).
Theorem 2.1
(Compactness and non–compactness) Let \(n \ge 2\) and suppose that \({\mathcal K}\) satisfies (H1)–(H3).
-
(i)
Compactness: Let \(0 \le \gamma < \gamma _\textrm{crit}\). Then for any sequence \(u_\epsilon \in L^1(\mathbb {T}^n)\) with \(\sup _{\epsilon } E_{\gamma ,\epsilon }[u_\epsilon ] < \infty \) there exists \(u \in {\mathcal A}\) and a subsequence (not relabeled) such that
$$\begin{aligned} u_\epsilon \xrightarrow {\epsilon \rightarrow 0} u{} & {} \text {in } L^1(\mathbb {T}^n). \end{aligned}$$ -
(ii)
Non–compactness: Let \(\gamma \ge \gamma _{\textrm{crit}}\). Then there exists a sequence \(u_\epsilon \in {\mathcal A}\) such that \(\sup _{\epsilon } E_{\gamma ,\epsilon }[u_\epsilon ] < \infty \), but there is no \(u \in {\mathcal A}\) such that \(u_\epsilon \rightarrow u\) in \(L^1(\mathbb {T}^n)\) for any subsequence.
Theorem 2.1 identifies the subcritical parameter regime \(0 \le \gamma < \gamma _{\textrm{crit}}\) and the supercritical parameter regime \(\gamma \ge \gamma _{\textrm{crit}}\). We learn that the local term dominates in the subcritical regime, while in the supercritical regime the destabilising effect of the non–local interaction takes over. The failure of compactness is reflected in uniform lower bounds of the energy and the behaviour of minimising sequences:
Corollary 2.2
(Lower bound of the energy) Let \(n \ge 2\) and suppose that \({\mathcal K}\) satisfies (H1)–(H3).
-
(i)
Let \(0 \le \gamma \le \gamma _{\textrm{crit}}\). Then \(E_{\gamma ,\epsilon } \ge 0\) for every \(\epsilon > 0\).
-
(ii)
Let \(\gamma > \gamma _{\textrm{crit}}\). Then there exists a sequence \(u_\epsilon \in {\mathcal A}\) such that
$$\begin{aligned} E_{\gamma ,\epsilon }[u_\epsilon ] \xrightarrow {\epsilon \rightarrow 0} -\infty . \end{aligned}$$(5)Moreover \(\displaystyle {\liminf _{\epsilon \rightarrow 0} P[u_\epsilon ] = \infty }\) for any sequence, such that (5) holds.
We note that in the critical case \(\gamma = \gamma _{\textrm{crit}}\), the family of energies \(E_{\gamma _{\textrm{crit}},\epsilon }\) does not have the compactness property even though it is bounded from below. This is due to the fact that \(0 \le E_{\gamma _{\textrm{crit}},\epsilon }[u] \rightarrow 0\) for polytopes (see Proposition 4.3 and 4.4), which are able to approximate any shape of finite perimeter (see (9)). In this case, higher order effects play a role and the theory of higher order \(\Gamma \)–expansions, developed in [3], should be suitable.
As explained in the introduction, we are interested in the limiting behaviour of minimising sequences as \(\epsilon \rightarrow 0\). We show that our family of non–local energies \(\Gamma \)–converges to a local energy functional:
Theorem 2.3
(\(\Gamma \)–convergence) Let \(n \ge 2\) and suppose that \({\mathcal K}\) satisfies (H1) – (H3). Let \(0 \le \gamma \le \gamma _{\textrm{crit}}\). Then \(E_{\gamma ,\epsilon } {\mathop {\longrightarrow }\limits ^{\Gamma }} E_{\gamma ,0}\) with respect to the \(L^1\)–topology, where
In particular, for every \(u \in L^1(\mathbb {T}^n)\) we have:
-
(i)
Liminf inequality: For every sequence \(u_\epsilon \in L^1(\mathbb {T}^n)\) such that \(u_\epsilon \rightarrow u\) in \(L^1(\mathbb {T}^n)\) we have \(E_{\gamma ,0}[u] \le \liminf _{\epsilon \rightarrow 0} E_{\gamma ,\epsilon }[u_\epsilon ]\).
-
(ii)
Limsup inequality: There is a sequence \(u_\epsilon \in L^1(\mathbb {T}^n)\) such that \(u_\epsilon \rightarrow u\) in \(L^1(\mathbb {T}^n)\) and \(\limsup _{\epsilon \rightarrow 0} E_{\gamma ,\epsilon }[u_\epsilon ] \le E_{\gamma ,0}[u]\).
Although the non–local term leads to a reduction of the interfacial cost by a factor of \(\frac{\gamma }{\gamma _{\textrm{crit}}}\) in the subcritical regime, the limit problem is simply the isoperimetric problem with a suitably modified prefactor.
In the physcial relevant dimension \(n = 2\), the minimiser of the limit problem is known (see [11, Theorem 4.1]). Up to translation and rotation, it is given by \(u = \chi _\Omega \), where \(\Omega \subset \mathbb {T}^2\) is a ball or the complement of a ball if
and by a single laminate otherwise. If equality holds, both ball (or its complement) and laminate are solutions. The isoperimetric problem in higher dimensions seems to be an open problem (see e.g. [43]).
Since our admissible class of functions is restricted to functions with values in \(\{0,1\}\), both main theorems hold true with respect to the \(L^p\)–topology for any \(p \in [1,\infty )\). Furthermore, we note that the main theorems also hold without the assumption of a fixed volume fraction, i.e. for admissible class of functions \({\mathcal A}= BV(\mathbb {T}^n,\{0,1\})\) as can be shown with minor modifications of the proofs.
Strategy of the proofs In the following we give an overview of the central strategy of the proofs for the theorems, noting that the detailed proofs are given in Sect. 4.2. Central to our proofs is the formulation of the energy in terms of the symmetrised autocorrelation function (see Lemma 4.2). At this stage, the radial symmetry of the kernel is crucial and the prefactor \(\epsilon ^{-1}\) of the non–local term ensures that the weight in the reformulation is an approximation of the identity. This implies that the limiting behaviour of the energy only depends on the autocorrelation function near the origin and the weight associated to the kernel \({\mathcal K}\) (rather than the kernel itself), which allows to treat kernels which also have negative values (see (H3)).
The lower bound in Theorem 2.3 follows from sharp estimates of the autocorrelation function. The upper bound requires higher regularity of the autocorrelation function near the origin in order to pass to the limit. For this purpose, we show that the autocorrelation function is a polynomial near the origin for polytopes (see Lemma 3.3). The reformulation of the energy in terms of the autocorrelation function allows for a splitting into behaviour near the origin (which is regular for polytopes as the autocorrelation function is a polynomial) and far from the origin (which is small since the weight is an approximation of the identity). The remainder of the proof of the upper bound follows from approximation with polytopes (see (9)).
Relation to biological model and comparision of sharp and diffuse interface models As explained in the introduction, the underlying biological model is a diffuse interface model (see (2)). In the Modica–Mortola theory, there is a connection between diffuse and sharp interface energies in the framework of \(\Gamma \)–convergence, namely (see [11, 36])
as \(\epsilon \rightarrow 0\), where
Naively, this would suggest to correspondingly replace the diffuse interface term in (2) by its sharp interface counterpart as in (6). In particular, we note that for \({\mathcal K}\) being the solution to
\({\mathcal F}_{q,\epsilon }\) in (2) is a corresponding diffuse interface model of \(E_{\gamma ,\epsilon }\) as described above. The energy \({\mathcal F}_{q,\epsilon }\) has been considered in [18] where it was shown that there exists \(\bar{q} > 0\), such that \({\mathcal F}_{q,\epsilon }\) \(\Gamma \)–converges to a constant multiple of the perimeter functional for all \(0< q < \bar{q}\). We note that the results of [18] do not contain a characterisation or estimation of \(\bar{q}\), nor the constant appearing in their \(\Gamma \)–limit. This is due to a nonlinear interpolation inequality shown in [9], which has no explicit description of the constants involved (see also [13]). On the other hand our result shows that the critical value \(q_{\textrm{crit}}\) of the corresponding sharp interface model (using the relations (6) and (7)) is given by
For \({\mathcal K}\) as in (8), we can explicitely compute the corresponding critical value of the sharp interface model and it is given by \(\gamma _{\textrm{crit}} = 1\) (Lemma A.1). However, one cannot equate the parameter \(q_{\textrm{crit}}\) with the corresponding critical value \(\bar{q}\) in [18]. Indeed, for a suitable doublewell potential with \(\Vert W\Vert _{L^\infty (0,1)} < \frac{1}{16}\) we would get \(q_{\textrm{crit}} < 0\). This shows, that \(\bar{q} = q_{\textrm{crit}}\) cannot hold, since the result of [18] shows that \(\bar{q} > 0\). This is probably due to the fact that the sharp interface model neglects effects which might occur of properties of the non–linearity (i.e. the double well potential W) such as asymmetry, compressibility of the chemical substance, or behaviour at infinity or the roots. In particular, the interpolation inequality used in [18] in order to show \(\bar{q} > 0\) only works for double well potentials W which have quadratic roots and superquadratic growth (see also [13, Section 3]). The sharp interface model does not contain information about the double well potential W other than the quantity \(\int _0^1 \sqrt{W(s)} \ ds\), which is unrelated to the aformentioned properties.
Our main result is similar to that of [18] in that we find two regimes for a parameter related to the relative strength of the non–local interaction (for our energy \(\gamma \), in [18] it is q), and the limit problem in the subcritical regime is the isoperimetric problem. The interpretation is the same as in [18], namely in the subcritical parameter regime, fine scale pattern formation does not occur in contrast to experimental results (e.g. stripe patterns or hexagonal array of balls, see [26, 44]). We conjecture fine scale patterns to form for the critical value \(\gamma = \gamma _{\textrm{crit}}\), which is subject of current research.
Although the reformulation of the non–local part in terms of the autocorrelation function (see Lemma 4.2) is also valid for the diffuse interface model (2), our methods used for the sharp interface model (3) fail for two main reasons. First, the autocorrelation function lacks useful properties for Sobolev functions \(u \in H^1(\mathbb {T}^n)\) such as \(c'_u(0) = 0\) in contrast to Proposition 3.2 (iii). Second, the energy is not anymore solely representable by the autocorrelation function due to the non–linearity W, i.e. the diffuse interface model is not linear in the space of autocorrelation functions, which our methods heavily rely on.
Remark 2.4
(Domains with arbitrary periodicity) The choice of the unit flat torus in contrast to flat tori with side length \(\ell > 0\) is justified by the scaling of the energy with respect to the reference domain. More precisely, let \(\mathbb {T}^n_\ell := \mathbb {R}^n/(\ell \mathbb {Z})^n\) and define
Let \(u \in BV(\mathbb {T}^n,\{0,1\})\) and define the rescaled function \(u_\ell \in BV(\mathbb {T}_\ell ^n,\{0,1\})\) via \(u_\ell (x) := u(\frac{x}{\ell })\). Then it holds
Thus, the limiting behaviour \(\epsilon \rightarrow 0\) as well as the subsequent analysis can be reduced to the case of the unit flat torus and the citical value \(\gamma _{\textrm{crit}}\) is independent of the choice of \(\ell \).
3 Autocorrelation function
We introduce the radially symmetrised autocorrelation function.
Definition 3.1
(Autocorrelation function) Let \(u \in L^1(\mathbb {T}^n)\). We define the autocorrelation function \(C_u: \mathbb {R}^n \longrightarrow \mathbb {R}\) by
We also define its radially symmetrised version \(c_u: \mathbb {R}_+ \longrightarrow \mathbb {R}\) by
Since \(C_u\) is \((0,1)^n\)–periodic, we can identify \(C_u\) with a function on the flat torus \(\mathbb {T}^n\). Note that \(c_u\) is generally not periodic.
The autocorrelation function was studied in the whole space setting (see [19, 31]). It is linked to the covariogram of a set \(\Omega \subset \mathbb {R}^n\) which is defined by
In [19] it was shown that \(g_\Omega \) is a Lipschitz function if and only if \(\Omega \) is a set of finite perimeter. The author also presents formulas for the perimeter of \(\Omega \) in terms of the covariogram, which we will also exploit in this work (adjusted to subsets of the flat torus \(\mathbb {T}^n\), see also [27]).
The covariogram has also been investigated in the context of convex geometry (see e.g. [4, 35, 39]). In [35] it was shown that under certain smoothness conditions of the boundary of a set, the covariogram of a convex body is smooth and they also present formulas for the first and second derivatives in this case. Further applications are random sets [5, 19, 30] and micromagnetism [27].
We briefly recall basic properties of the autocorrelation function:
Proposition 3.2
(Basic properties of the autocorrelation function) Let \(u \in BV(\mathbb {T}^n,\{0,1\})\). Then \(C_u\) and \(c_u\) are Lipschitz continuous and it holds:
-
(i)
\(0 \le C_u(x) \le C_u(0) = \Vert u\Vert _{L^1(\mathbb {T}^n)} \qquad \) for all \(x \in \mathbb {T}^n\).
-
(ii)
\(0 \le c_u(r) \le c_u(0) = \Vert u\Vert _{L^1(\mathbb {T}^n)} \qquad \) for all \(r > 0\).
-
(iii)
\(\displaystyle { \Vert c_u'\Vert _{L^\infty (0,\infty )} = -c_u'(0) = \frac{\omega _{n - 1}}{n \omega _n} \int _{\mathbb {T}^n} |\nabla u|}\).
Proof
See [27, Proposition 2.3 and Proposition 2.4]. \(\square \)
For the proof of the upper bound of Theorem 2.3, in order to pass to the limit \(\epsilon \rightarrow 0\), we need higher regularity than Lipschitz continuity of the autocorrelation function near the origin. However, one cannot expect higher regularity in general since e.g. \(c''_{\chi _\Omega }(0) = +\infty \) when \(\Omega \) has a cusp. We will work around this issue by showing that the autocorrelation function of polytopes is a polynomial near the origin, and hence regular. The desired limit for a general shape of finite perimeter will be dealt with via approximation by polytopes, i.e. for every \(u \in BV(\mathbb {T}^n,\{0,1\})\) there exists a sequence of polytopes \(\Omega _k \subset \mathbb {T}^n\) such that (see [17])
The following result is known in the full space setting for convex polytopes for \(n = 2\) (see [20, 39]), but we were not able to find versions of it for arbitrary polytopes. We note that a closed set \(\Omega \subset \mathbb {T}^n\) is said to be a polytope, if the restriction of its canonical embedding to \([0,1]^n\) is a polytope in \(\mathbb {R}^n\).
Lemma 3.3
(Autocorrelation function for polytopes) Let \(\Omega \subset \mathbb {T}^n\) be a polytope and let \(u := \chi _\Omega \). Then there exists \(0< R < 1\) and \(a_2,\ldots ,a_n \in \mathbb {R}\) with \(a_2 \ge 0\) such that
Proof
In [27, Lemma 2.5] it was shown that (10) holds for stripes with \(a_2, \ldots , a_n = 0\). Since the only polytopes which do not have corners are stripes, we can without loss of generality assume that \(\Omega \) has at least one corner. We denote the set of corners of \(\Omega \) by \({\mathcal C}\). We define
where for any \(p \in {\mathcal C}\) we set
Let \(r > 0\), \(w \in {\mathbb {S}}^{n - 1}\) and let \(\Omega _{rw} := \Omega + rw\). Then
where \(\bigtriangleup \) denotes the symmetric difference.
Since \(C_u(0) = \Vert u\Vert _{L^1(\mathbb {T}^n)} = |\Omega |\) by Proposition 3.2 (i) it hence remains to calculate \(|\Omega \bigtriangleup \Omega _{rw}|\) and its dependence on r.
We assume that \(w \not \in {\mathcal S}\), where \({\mathcal S}\subset {\mathbb {S}}^{n-1}\) is the negligible set of vectors which are tangential to any of the (finitely many) faces of \(\Omega \). By the choice of R, the number of faces N of \(\Omega \bigtriangleup \Omega _{rw}\) is then independent of \(r \in (0,R)\) and independent of w (see Fig. 1). Furthermore, there exist convex trapezoids \(T_{rw}^{(1)},\ldots T_{rw}^{(N)} \subset \mathbb {T}^n\) with pairwise disjoint interiors such that (see Fig. 2)
Each of these convex trapezoids \(T_{rw}^{(i)}\), \(i \in \{1,\ldots , N\}\), is determined by a system of linear inequalities
where for \(x,y \in \mathbb {T}^n\) we denote \(x \le y\) if and only if \(x_j \le y_j \! \mod 1\) for every \(j \in \{1,\ldots ,n\}\) and for some matrices \(A^{(i)} \in \mathbb {R}^{2N \times n}\) and vectors \(b^{(i)} \in \mathbb {T}^{2N}\). By a slicing argument there exist \(d_1^{(i)}(w), \ldots , d_n^{(i)}(w) \in \mathbb {R}\) such that (see Fig. 3)
More precisely, for \(x = (x_1,x')\), there exist at most 2N intervals \(I_{m_1} = [f_{m_1}(x', rw), g_{m_1}(x',rw)]\), where \(f_{m_1}\) and \(g_{m_1}\) depend in an affine way on \(x'\) and rw, and convex polytopes \(K_{m_1} \subset \mathbb {T}^{n - 1}\) such that
The integrand is now a polynomial in r of degree 1 and the set of integration is again a convex polytope of the form (11) (reduced in dimension, with different matrices \(A^{(i)}\) and \(b^{(i)}\)). Iteratively, we obtain in the l-th step convex polytopes \(K_{m_1,\ldots ,m_l}\) and a polynomial \(f_{m_1,\ldots ,m_l}\) of degree l such that
The algorithm terminates after n steps and leaves a polynomial in r of degree n as described in (12). The assertion now follows from (12) by combining the above identities, i.e.
for all \(r \in (0,R)\). Averaging with respect to w then yields
for some \(a_1,\ldots ,a_n \in \mathbb {R}\). Proposition 3.2 (iii) shows that \(a_1 = - \frac{\omega _{n - 1}}{n \omega _n} P[u]\). By (13) we have \(c''(0) = 2 a_2\). In view of Proposition 3.2 (iii) we have \(c''(0) \ge 0\) and hence \(a_2 \ge 0\). More precisely, from the regularity of the autocorrelation function we have
\(\square \)
Remark 3.4
(Full space setting) We note that with analogous arguments the result of Lemma 3.3 also holds in the full space setting.
4 Compactness and \(\Gamma \)–convergence
4.1 Reformulation of the energy
For the subsequent analysis it is convenient to use the integrated kernel
instead of the kernel itself. We collect some basic properties of \(\Phi \) which follow from our assumptions on \({\mathcal K}\):
Proposition 4.1
(Basic properties of \(\Phi \)) Assume \({\mathcal K}\) satisfies (H1)–(H3). Let \(\Phi : (0,\infty ) \longrightarrow \mathbb {R}\) be given by (14) and let \(\Phi _\epsilon (r) := \frac{1}{\epsilon }\Phi (\frac{r}{\epsilon })\). Then \(\Phi \in L^1(0,\infty )\) with \(\Phi \ge 0\). Furthermore,
-
(i)
\(\displaystyle \lim _{r\rightarrow \infty } r \Phi (r) = \lim _{r\rightarrow 0} r \Phi (r) = 0\).
-
(ii)
\(\displaystyle \int _0^\infty \Phi (r) \ dr = \int _{\mathbb {R}^n} |z| \, {\mathcal K}(z) \ dz < \infty \).
-
(iii)
\(\displaystyle \int _0^1 r^j \Phi _\epsilon (r) \ dr \xrightarrow {\epsilon \rightarrow 0} 0\) for \(j \ge 1\).
Proof
By definition of \(\Phi \) and (H3) we have \(\Phi \ge 0\) and
By definition of \(\Phi \) and assumption (H2) we have
as \(R \rightarrow \infty \). Moreover, it follows from the Dominated Convergence Theorem
which shows that (i) holds. Integrating by parts we get for \(0< \varrho< R < \infty \)
which yields (ii) in the limits \(\varrho \rightarrow 0\) and \(R \rightarrow \infty \) by (i) and the Dominated Convergence Theorem. Assertion (iii) holds since \(\Phi \in L^1(0,\infty )\). \(\square \)
We are ready to rewrite the nonlocal term in \(E_{\gamma ,\epsilon }\) in terms of the symmetrised autocorrelation function and the integrated kernel \(\Phi \):
Lemma 4.2
(Representation of energy by autocorrelation function) Let \(\gamma , \epsilon > 0\) and suppose \({\mathcal K}\) satisfies (H1)–(H3). Let \(\Phi \) be given by (14) and let \(\Phi _\epsilon (r) := \frac{1}{\epsilon }\Phi (\frac{r}{\epsilon })\). Then
where \(\gamma _{\textrm{crit}}\) is represented in terms of \(\Phi \) via
Proof
We first note that the representation (16) follows from (4) together with Proposition 4.1 (ii), and \(\gamma _{\textrm{crit}} > 0\) since \(\Phi \ge 0\). Since u only takes values in \(\{0,1\}\) we have with Proposition 3.2 (i)
where in the last line we switched to polar coordinates. Let \(0< \varrho< R < \infty \). Noting that \(c_u\) is Lipschitz (Proposition 3.2), we integrate by parts to obtain
noting that \(\Phi _\epsilon (r) = \frac{1}{\epsilon }\Phi (\frac{r}{\epsilon })\). Using Proposition 3.2 (iii) we obtain
Thus the boundary terms in (17) vanish in the limit \(\varrho \rightarrow 0\) and \(R \rightarrow \infty \) by Proposition 4.1 (i). It follows from the Dominated Convergence Theorem and the computations above that
The claim follows by inserting (18) into (3) and using Proposition 3.2 (iii) to rewrite P[u] in terms of \(c'_u(0)\). \(\square \)
4.2 Proofs of the main theorems
We next use the reformulation of the energy \(E_{\gamma ,\epsilon }\) from Lemma 4.2 to show that the limit energy is a pointwise lower bound. This will simplify the proof of the compactness in Theorem 2.1 and the liminf inequality of Theorem 2.3. It relies on the bound \(c_u'(0) = \min _{r \ge 0} c_u'(r)\) for all \(u \in {\mathcal A}\) (Proposition 3.2 (iii)).
Proposition 4.3
(Lower bound for the energy) Let \(\gamma , \epsilon > 0\) and suppose that \({\mathcal K}\) satisfies (H1)–(H3). Then
Proof
By Proposition 4.1 (iii), Proposition 3.2 (iii) and Lemma 4.2 we obtain
\(\square \)
The next proposition is a convergence result and simplifies the non compactness (Theorem 2.1 (ii) and limsup inequality of Theorem 2.3. The key observation is that the family of integral kernels \(\Vert \Phi \Vert _{L^1(0,\infty )}^{-1} \Phi _\epsilon \) forms an approximation of the identity, so we formally achieve with the reformulation of the energy (see Lemma 4.2)
However, for general functions \(u \in {\mathcal A}\) it is not clear if the convergence \(E_{\gamma ,\epsilon }[u] \rightarrow E_{\gamma ,0}[u]\) holds pointwise since the function \(c_u'\) is not differentiable at the origin in general. We hence consider the smaller class of polytopal domains. This is where we use the formula for the autocorrelation function for polytopes (see Lemma 3.3).
Proposition 4.4
(Pointwise convergence for polytopes) Let \(\gamma > 0\) and suppose \({\mathcal K}\) satisfies (H1)–(H3). Let \(\Omega \subset \mathbb {T}^n\) be a polytope and let \(u = \chi _\Omega \). Then
Proof
Let \(\epsilon > 0\). It suffices to show that the non–local term converges, i.e. (see Lemma 4.2 and (18))
Lemma 3.3 yields the existence of \(a_1,\ldots , a_{n - 1} \in \mathbb {R}\) and \(0< R < 1\) such that
We use this identity to compute
For the first integral, we observe that by monotone convergence
For the second integral we use Proposition 4.1 (iii) to obtain
For the third integral, using Proposition 3.2 (iii) we have
Altogether (20) follows. \(\square \)
We are now in the position to prove the compactness (Theorem 2.1 (i)) and non–compactness (Theorem 2.1 (ii)) of \(E_{\gamma ,\epsilon }\):
Proof of Theorem 2.1
In order to prove assertion (i) we use Proposition 4.3 to obtain
uniformly in \(\epsilon \). Using the \(L^1\)–compactness of the perimeter functional proves the claim. In order to prove assertion (ii) we construct a sequence of laminates with the desired properties. We define \(\Omega := (0,\theta ) \times [0,1)^{n - 1} \subset \mathbb {T}^n\) and \(v_k(x) := \chi _{\Omega }(kx)\). Then \(P[v_k] = 2^{k + 1}\) and \(v_k \in {\mathcal A}\) for all \(k \in \mathbb {N}\). Moreover, there does not exist a subsequence of \(v_k\) which converges in \(L^1\). Indeed, assume there exists a subsequence (not relabeled) and \(v \in L^1(\mathbb {T}^n,\{0,1\})\), such that \(v_k \rightarrow v\) in \(L^1\) as \(k \rightarrow \infty \). Then \(\Vert v\Vert _{L^1(\mathbb {T}^n)} = \theta \). We note that \(v_k \rightharpoonup ^* \theta \) in \(L^\infty \) as \(k \rightarrow \infty \) (see [7, Example 2.7]) and thus
a contradiction. Further, from Proposition 4.4 we obtain
since \(\gamma \ge \gamma _{\textrm{crit}}\). Hence, for all \(k \in \mathbb {N}\) there exists \(\epsilon ^*(k)\) such that
For \(\frac{1}{2} \min \{\frac{1}{k + 1}, \epsilon ^*(k + 1)\} \le \epsilon \le \frac{1}{2} \min \{\frac{1}{k}, \epsilon ^*(k)\}\), we choose \(u_\epsilon = v_k\). Then there does not exist an \(L^1\)–convergent subsequence as was shown above, and
from which the claim follows. \(\square \)
From the techniques used to prove Theorem 2.1, we are now able to show Corollary 2.2:
Proof of Corollary 2.2
Assertion (i) follows directly from Proposition 4.3. In order to show assertion (ii), let \(v_k\) and \(u_\epsilon \) as in the proof of Theorem 2.1 (ii). Then
from which the claim follows since \(\gamma > \gamma _{\textrm{crit}}\). In order to prove the necessity of a sequence with unbounded perimeter, we argue by contradiction: assume that (after selection of a subsequence) \(P[u_\epsilon ] \lesssim 1\), then \(-1 \lesssim E_{\gamma ,\epsilon }[u_\epsilon ]\) by Proposition 4.3, which contradicts (5). \(\square \)
We are now in the position to prove the \(\Gamma \)–convergence of \(E_{\gamma ,\epsilon }\):
Proof of Theorem 2.3
For the liminf inequality, let \(u_\epsilon \rightarrow u\) in \(L^1(\mathbb {T}^n)\). By Theorem 2.1 (i) we can assume without loss of generality that \(u_\epsilon , u \in {\mathcal A}\). From the lower semicontinuity of the perimeter functional and Proposition 4.3 we obtain
To show the limsup inequality, we use Proposition 4.4 and an approximation using polytopes. If \(u \notin {\mathcal A}\), the statement is obvious. So let \(u \in {\mathcal A}\). Then there exists a sequence of polytopes \(\Omega _k \subset \mathbb {T}^n\), such that (see (9))
By a rescaling of \(\Omega _k\), we can without loss of generality assume that \(v_k := \chi _{\Omega _k} \in {\mathcal A}\). We proceed similarly as in the proof of Theorem 2.1. By Proposition 4.4 we have \(E_{\gamma ,\epsilon }[v_k] \rightarrow E_{\gamma ,0}[v_k]\) as \(\epsilon \rightarrow 0\) for any \(k \in \mathbb {N}\). Hence, for all \(k \in \mathbb {N}\) there exists \(\epsilon ^*(k)\) such that
For \(\frac{1}{2} \min \{\frac{1}{k + 1}, \epsilon ^*(k + 1)\}< \epsilon < \frac{1}{2} \min \{\frac{1}{k}, \epsilon ^*(k)\}\) we choose \(u_\epsilon = v_k\). Then
from which the claim follows. \(\square \)
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Acknowledgements
D.B. would like to warmly thank M. Mercker, T. Stiehl, J. Fabiszisky, B. Brietzke, C. Tissot and A. Tribuzio for valuable discussions on the topic. This work is funded by the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) under Germany’s Excellence Strategy EXC-2181/1-39090098 (the Heidelberg STRUCTURES Cluster of Excellence). The authors like to thank the anonymous referee for carefully reading the manuscript and helpful suggestions.
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A. Appendix
A. Appendix
In the following Lemma, we present some examples of admissible kernels.
Lemma A.1
Let \(s \in (1,2]\) and let \({\mathcal K}^{(s)} \in L^1(\mathbb {R}^n)\) be the unique solution to
Then \({\mathcal K}^{(s)}\) satisfies (H1)–(H3). Moreover, for \(s = 2\) we have
and the associated critical value \(\gamma _{\textrm{crit}}^{(2)}\) (cf. (4)) is given by \(\gamma _{\textrm{crit}}^{(2)} = 1\).
Proof
We first note that the equation can be solved explicitly with Fourier methods. More precisely it holds
Since the Fourier transform is an injective map \(\widehat{\bullet }: L^1(\mathbb {R}^n) \longrightarrow C^0_b(\mathbb {R}^n)\), the solution of (24) is unique. Since \(\widehat{\mathcal K}^{(s)}\) is radial, so is \({\mathcal K}^{(s)}\) and thus (H1). We treat the cases \(s = 2\) and \(s \ne 2\) separately. If \(1< s < 2\), we get from [32, Lemma 1.2] that \({\mathcal K}^{(s)} \ge 0\) and \(|{\mathcal K}^{(s)}(r)| \lesssim r^{-n - s}\) for \(r \ge 1\) which directly yield both (H2) and (H3). If \(s = 2\), switching to polar coordinates in (24), \({\mathcal K}^{(2)}\) solves
Substituting \({\mathcal K}^{(2)}(r) := r^{1 - \frac{n}{2}} g(r)\), we obtain
This is the modified Bessel equation. The unique decaying solution is given by \(g = K_{\frac{n}{2} - 1}\), where \(K_\nu \) denotes the decaying modified Bessel function of the second kind of genus \(\nu \ge 0\), i.e.
Altogether, we obtain
where \(a = (2\pi )^{-\frac{n}{2}}\) such that \(\Vert {\mathcal K}^{(2)}\Vert _{L^1(\mathbb {R}^n)} = 1\). Since \(K_\nu \ge 0\) for all \(\nu \ge 0\), it follows (H3). The identity (25) and (H2) follow from [24, p.676]. \(\square \)
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Brazke, D., Knüpfer, H. & Marciniak–Czochra, A. \(\Gamma \)–limit for a sharp interface model related to pattern formation on biomembranes. Calc. Var. 62, 94 (2023). https://doi.org/10.1007/s00526-022-02413-2
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DOI: https://doi.org/10.1007/s00526-022-02413-2