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Dynamical theory of spectroscopy with femtosecond pulse excitation (I)

Dynamics of absorption and emission processes

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Abstract

A dynamical theory of spectroscopy with femtosecond pulse excitation is developed and is applied to studying the one-photon absorption and two-photon emission processes. Unlike the previous theories, this theory can treat all kinds of optical process from ultrashort pulse to CW limit in a consistent picture, because the exact equation of emission rate obtained from this theory can correctly reduce to the Kramers-Heisenberg-Dirac (KHD) expression.

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Authors and Affiliations

  1. Department of Chemistry, Fudan University, 200433, Shanghai, China

    Jing Lu, Soo-Ying Lee & Kangnian Fan

  2. Department of Chemistry, National University of Singaplre, 119260, Singapore

    Jing Lu & Soo-Ying Lee

Authors
  1. Jing Lu
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  2. Soo-Ying Lee
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  3. Kangnian Fan
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Lu, J., Lee, SY. & Fan, K. Dynamical theory of spectroscopy with femtosecond pulse excitation (I). Sci. China Ser. A-Math. 40, 958–966 (1997). https://doi.org/10.1007/BF02878675

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  • DOI: https://doi.org/10.1007/BF02878675

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