Abstract
Axially (c-axis)-oriented ZnO thick films with a ∼8.1 μm thickness were fabricated on ZnO seed layer coated substrates by using a filtered preheated hydrothermal solution. The thick films composed of single-crystal ZnO microrods with various diameters were formed by coalescing each nanorod together along their side surfaces. From the X-ray diffraction result a biaxial stress exists was found to exist in the as-grown thick films, and the stress gradually increased with increasing annealing temperatures from 200 to 550 °C due to a degradation in the crystalline quality. The biaxial stress is responsible for the red-shift of the optical band gap of the ZnO thick films. Photoluminescence and Hall results revealed that the optical and the electrical properties of the thick films were degenerated after high-temperature annealing (> 200 °C), which was due to the introduction of point defects, such as oxygen interstitials and zinc vacancies.
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References
M. Wang and L. Zhang, Mater. Lett. 63, 301 (2009).
B. Wen, Y. Huang, J. J. Boland, J. Phys. Chem. C 112, 106 (2008).
A. L. Ding, X. Y. He, P. S. Qui, S. J. Wang and W. G. Luo, Proceedings of the 2000 12th IEEE International Symposium on Applications of Ferroelectrics, edited by S. K. Streiffer, B. J. Gibbons, T. Tsurumi, and M. A. Zurbuchen (Hawaii, U.S.A., July 21–August 2, 2000), p. 515.
G. R. Li et al., Electrochem. Comm. 9, 863 (2007).
J. H. Kim et al., Adv. Funct. Mater. 17, 463 (2007).
Y. Zhang, F. Lu, Z. Wang and L. Zhang, J. Phys. Chem. C 111, 4519 (2007).
J. M. Dreyfors, S. B. Jones and Y. Sayed, Am. Ind. Hyg. Assoc. J. 50, 579 (1989).
J. Qiu et al., Nanotechnology 20, 155603 (2009).
X. Yan, Z. Li, R. Chen and W. Gao, Cryst. Growth Des. 8, 2407 (2007).
K. Govender, D. S. Boyle, P. B. Kenway, P. O’Brien, J. Mater. Chem. 14, 2575 (2004).
A. Sugunan, H. C. Warad, M. Boman and J. Dutta, J. Sol-Gel Sci. Techn. 39, 49 (2006).
J. F. Zang et al., Electroanal. 19, 1008 (2007).
J. Joo, B. Y. Chow, M. Prakash, E. S. Boyden and J. M. Jacobson, Nat. Mater. 10, 596 (2011).
B. Y. Oh, M. C. Jeong, D. S. Kim, W. Lee and J. M. Myoung, J. Cryst. Growth 281, 475 (2005).
Z. B. Fang, Z. J. Yan, Y. S. Tan, X. Q. Liu and Y. Y. Wang, Appl. Surf. Sci. 241, 303 (2005).
M. Wang, J. Wang, W. Chen, Y. Cui and L. Wang, Mater. Chem. Phys. 97, 219 (2006).
B. L. Zhu et al., Jpn. J. Appl. Phys. 45, 7860 (2006).
A. B. Djurišić et al., Nanotechnology 18, 095702 (2007).
M. Suchea, S. Christoulakis, M. Katharakis, N. Vidakis and E. Koudoumas, Thin Solid Films 517, 4303 (2009).
R. Ghosh, D. Basak and S. Fujihara, J. Appl. Phys. 96, 2689 (2004).
Y. F. Li et al., Appl. Phys. Lett. 91, 021915 (2007).
Y. F. Li et al., J. Appl. Phys. 104, 083516 (2008).
L. E. Greene et al., Angew. Chem. Int. Ed. 42, 3031 (2003).
R. B. M. Cross, M. M. D. Souza and E. M. S. Narayanan, Nanotechnology 16, 2188 (2005).
H. Zhou, H. Alves, D. M. Hofmann, W. Kriegseis and B. K. Meyer, Appl. Phys. Lett. 80, 210 (2002).
A. B. Djurišić et al., Nanoscale Phenomena 2, 117 (2007).
H. T. Ng et al., Appl. Phys. Lett. 82, 2023, (2003).
Q. X. Zhao et al., Appl. Phys. Lett. 87, 211912 (2005).
A. B. Djurišić et al., Adv. Funct. Mater. 14, 856 (2004).
J. L. Zhao, X. M. Li, J. M. Bian, W. D. Yu and C. Y. Zhang, Thin Solid Films 515, 1763 (2006).
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Qiu, J., Shin, DM., He, W. et al. Synthesis and physical properties of zinc-oxide textured films by using a filtered preheated hydrothermal. Journal of the Korean Physical Society 65, 1423–1429 (2014). https://doi.org/10.3938/jkps.65.1423
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DOI: https://doi.org/10.3938/jkps.65.1423