Critical review of Fenton and photo-Fenton wastewater treatment processes over the last two decades

Machado, F.; Teixeira, A. C. S. C.; Ruotolo, L. A. M.

doi:10.1007/s13762-023-05015-3

Critical review of Fenton and photo-Fenton wastewater treatment processes over the last two decades

Review
Published: 07 June 2023

Volume 20, pages 13995–14032, (2023)
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Abstract

Water pollution is currently one of the major problems that the scientific community must solve in the twenty-first century. This issue is made even more challenging by the fact that conventional effluent treatment processes usually show poor degradation performance for a variety of recalcitrant chemical components, remaining present after simple treatments. In this scenario, advanced oxidative processes emerge as a possible solution. Due to their simplicity, the Fenton and photo-Fenton processes have attracted the attention of the scientific community for decades. This review presents a critical analysis of the feasibility of these processes for full-scale diffusion. Seeking to elucidate this point, a broad review of the literature on Fenton and photo-Fenton processes is carried out, focusing on homogeneous processes, in the last two decades (2000–2021). With this review, the authors intend to fill part of the gap of studies in the literature about the potential applicability of scaling up the Fenton and photo-Fenton processes. Fundamentals, characteristics, process parameters, chemical and photochemical reactor designs, and scale-up challenges are examined in detail. Examples of applications of these oxidative processes in pilot and full-scale conditions are presented. Finally, this review concludes with current trends and future perspectives with the aim of helping researchers in the field to direct their topics and contribute to further development of scale-up studies in advanced oxidative processes, especially with Fenton reactions.

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Fundamentals and Applications of the Photo-Fenton Process to Water Treatment

Bio-electro-Fenton: A New Combined Process – Principles and Applications

Zero Fenton sludge discharge: a review on reuse approach during wastewater treatment by the advanced oxidation process

Article 13 January 2021

Abbreviations

AOP:: Advanced oxidation processes
[C]:: Concentration
BCR:: Bubble column reactor
BOD:: Biochemical oxygen demand
CFD:: Computational fluid dynamics
CIEMAT:: Centro de Investigaciones Energéticas, Medioambientales y Tecnológicas
COD:: Chemical oxygen demand
CPC:: Compound parabolic concentrator
CSTR:: Continuous stirred-tank reactor
D_col :: Column diameter
D_out :: Outer diameter
D_in :: Inner diameter
Dp:: Particle diameter
DFT:: Density functional theory
DNS:: Direct numerical simulation
DOC:: Dissolved organic carbon
EDDS:: Ethylenediamine-N, N'-disuccinic acid
FBR:: Fluidized bed reactor
FFR:: Falling film reactor
H_col :: Column height
HPLC:: High-performance liquid chromatography
IUPAC:: International union of pure and applied chemistry
k:: Reaction rate constant
k_diff :: Diffusion constant
L:: Length
MCS:: Monte carlo simulations
MDS:: Molecular dynamics simulations
PC:: Planar collector
PTC:: Parabolic-trough collectors
RPC:: Raceway pond reactor
SBR:: Sequencing batch reactor
SEC:: Solar energy collectors
T:: Temperature
TOC:: Total organic carbon
T_R :: Residence time
TST:: Transition state theory
V_R :: Reactor volume
V_T :: Total volume

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Acknowledgements

The authors express their gratitude to the National Council for Scientific and Technological Development (CNPq, Grant No. 311230/2020-2), São Paulo State Research Foundation (FAPESP, Grant Nos. 2017/19838-5 and 2020/12706-9), and to the Coordination for the Improvement of Higher Education Personnel – Brazil (CAPES) – Finance Code 001.

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F. Machado
Present address: Institute of Chemistry, University of São Paulo, Av Professor Lineu Prestes, 748, São Paulo, SP, 05508-00, Brazil

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Department of Chemical Engineering, Federal University of São Carlos, Rod. Washington Luiz, Km 235, São Carlos, SP, 13565-905, Brazil
F. Machado & L. A. M. Ruotolo
Research Group in Advanced Oxidation Processes (AdOx), Department of Chemical Engineering, Escola Politécnica, University of São Paulo, Av. Prof. Luciano Gualberto, tr. 3, 380, São Paulo, SP, 05508-010, Brazil
A. C. S. C. Teixeira

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Machado, F., Teixeira, A.C.S.C. & Ruotolo, L.A.M. Critical review of Fenton and photo-Fenton wastewater treatment processes over the last two decades. Int. J. Environ. Sci. Technol. 20, 13995–14032 (2023). https://doi.org/10.1007/s13762-023-05015-3

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Received: 01 August 2022
Revised: 05 May 2023
Accepted: 20 May 2023
Published: 07 June 2023
Issue Date: December 2023
DOI: https://doi.org/10.1007/s13762-023-05015-3

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Critical review of Fenton and photo-Fenton wastewater treatment processes over the last two decades