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Effective degradation of high-concentration organic pollutants under broad pH range with Fe(II, III)-doped bio-carbon through sono-Fenton oxidation

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Abstract

To effectively remove toxic organic pollutants from the highly concentrated sewage, a Fe(II, III) and heteroatom (S, N)-incorporated bio-carbon (Fe(II, III)@HIC) was prepared from cicada slough (CS) by one-step hydrothermal process. Fe-doped particles on the material’s surface present a mesh network structure, which helps the dye to adhere. The introduced Fe2+ and Fe3+ endow the prepared Fe(II, III)@HIC with prominent oxidation characteristic toward organic pollutants. Owing to the unique mesh structure and surface properties, the prepared Fe(II, III)@HIC remove 93.69% of Congo red (CR), 99.87% of methylene blue (MB), and 90.32% of tetracycline (TC) from wastewater at concentrations up to 300 mg/L in 240 min. In addition, the removal effect toward organic dye is little affected by pH and concentration of coexisting salt ions. This work provides an ideal strategy for the purification of industrial sewage containing highly concentrated organic pollution.

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Funding

This work was supported by the National Natural Science Foundation of China (No. 52102303), the Opening Project of State Key Laboratory of Polymer Materials Engineering (Sichuan University) (No. sklpme2021-05–09), the Foundation of Education Department of Shaanxi Province (20JK0805), and the Xi’an Science and Technology Plan Project (22GXFW0092, 22GXFW0097).

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Authors and Affiliations

  1. The Faculty of Printing, Packaging Engineering and Digital Media Technology, Xi’an University of Technology, Xi’an Shaanxi, 710048, People’s Republic of China

    ZhenFeng Sun, XueYan Zhao, MeiXia Huo, JiaYi Wang, Fang Ren, YanLing Jin & PengGang Ren

  2. College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University, Chengdu, 610065, People’s Republic of China

    Fang Ren & PengGang Ren

  3. No. 203 Research of Nuclear Industry, Xi’an, Shaanxi, 710086, People’s Republic of China

    Yanli Du

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ZS: methodology, conceptualization, formal analysis, software. XZ: investigation, writing—original draft, software. MH: methodology, visualization. JW: formal analysis, software. YJ: visualization, project administration. FR: data curation. YD: methodology, visualization. PR: writing—review and editing, supervision.

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Sun, Z., Zhao, X., Huo, M. et al. Effective degradation of high-concentration organic pollutants under broad pH range with Fe(II, III)-doped bio-carbon through sono-Fenton oxidation. Biomass Conv. Bioref. (2023). https://doi.org/10.1007/s13399-023-05057-0

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