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Nuclear spin relaxation of 111Cd at the A site in spinel oxides, CdFe2O4 and CdIn2O4

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Abstract

Local fields in normal spinel oxides, CdFe2O4 and CdIn2O4, were measured by means of time-differential perturbed angular correlation spectroscopy with the 111In(→111Cd) and 111mCd(→111Cd) probes. The spectra obtained with the different probes show contrastive patterns in spite of the same daughter nuclei: the former shows static perturbations with explicit oscillatory structures, whereas for the latter, the angular correlations become gradually isotropic. The exponential-like relaxation patterns of the spectra observed for the 111mCd(→111Cd) probe suggest that the probes occupying the Cd A site experience time-dependent perturbation causing nuclear spin relaxation.

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Acknowledgement

The present work was supported in part by JSPS KAKENHI Grant Number 26286075.

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Authors and Affiliations

  1. Institute of Science and Engineering, Kanazawa University, Kanazawa, Ishikawa, 920-1192, Japan

    W. Sato

  2. National Institute of Technology, Ichinoseki College, Ichinoseki, Iwate, 021-8511, Japan

    S. Komatsuda

  3. Institute for Integrated Radiation and Nuclear Science, Kyoto University, Kumatori, Osaka, 590-0494, Japan

    Y. Ohkubo

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  1. W. Sato
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  2. S. Komatsuda
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  3. Y. Ohkubo
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Correspondence to W. Sato.

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Sato, W., Komatsuda, S. & Ohkubo, Y. Nuclear spin relaxation of 111Cd at the A site in spinel oxides, CdFe2O4 and CdIn2O4. J Radioanal Nucl Chem 316, 1289–1293 (2018). https://doi.org/10.1007/s10967-018-5855-8

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  • DOI: https://doi.org/10.1007/s10967-018-5855-8

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