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Energy storage and piezoelectric properties of lead‐free SrTiO3-modified 0.965Bi0.5Na0.5TiO3–0.035BaTiO3 ceramics

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Abstract

This manuscript reports the synthesis and piezoelectric properties of strontium titanate, SrTiO3-modified bismuth sodium titanate-barium titanate, 0.965Bi0.5Na0.5TiO3–0.035BaTiO3, (BNBT-xST, x = 0.00−0.30) ceramics produced by facile low temperature sol–gel and hydrothermal methods. Close inspection of the X-ray diffraction profile through Rietveld refinement indicates ST modification in BNBT leads to a phase transition from the dominant rhombohedral phase to a single tetragonal phase. This structural transition leads to enhancement of electromechanical and energy storage properties. A large dynamic piezoelectric coefficient (d*33 = 350 pC/V) was observed for BNBT-0.1ST sample. High energy storage density (Wrec = 0.37) and large energy storage efficiency (η = 75%) were observed at 75 °C for the BNBT-0.3ST sample. The energy storage response of the tunable ferrorelectric ceramics suggests their possible use for high-performance dielectric capacitor applications.

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Authors and Affiliations

  1. Department of Engineering Physics, McMaster University, 1280 Main Street West, Hamilton, ON, L8S 4L7, Canada

    Muhammad Munir & Ayse Turak

  2. School of Materials Science and Engineering, Changwon National University, Changwon, 51140, South Korea

    Muhammad Habib, Salman Ali Khan, Myong-Ho Kim, Soonil Lee & Tae-Kwon Song

  3. Department of Materials Convergence and System Engineering, Changwon National University, Changwon, 51140, South Korea

    Soonil Lee

  4. Department of Materials Science and Engineering, Institute of Space Technology, Islamabad, 44000, Pakistan

    Abrar H Baluch

  5. Department of Space Science, Institute of Space Technology, Islamabad, 44000, Pakistan

    Ali Hussain

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Munir, M., Habib, M., Khan, S.A. et al. Energy storage and piezoelectric properties of lead‐free SrTiO3-modified 0.965Bi0.5Na0.5TiO3–0.035BaTiO3 ceramics. J Mater Sci: Mater Electron 32, 10712–10725 (2021). https://doi.org/10.1007/s10854-021-05728-6

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