Abstract
BaTiO3/(ZnO)x ceramics (x = 0, 2, 5 and 10 wt%) were produced via solid state reaction by using high energy ball milling. The morphological, structural, spectral, optical, electrical and dielectric properties were systematically investigated. X-ray diffraction indicated that all ceramics crystallize in the tetragonal structure. The grains size increases with ZnO additions. The optical band gap energy (Eg) was also evaluated and found to reduce with increasing ZnO concentration. The dielectric and electric properties revealed that an optimal ZnO content lead to obtain ceramic with high dielectric constant and low tangent loss, which are encouraging for radio frequencies and microwaves applications.
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L. Xiaochi, W. Bian, Y. Li, H. Zhu, F. Zhenxiao, Q. Zhang, Influence of inverse spinel structured CuGa2O4 on microwave dielectric properties of normal spinel ZnGa2O4 ceramics. J. Am. Ceram. Soc. 101, 1646–1654 (2018)
L. Xiaochi, W. Bian, C. Min, F. Zhenxiao, Q. Zhang, H. Zhu, Cation distribution of high-performance Mn-substituted ZnGa2O4 microwave dielectric ceramics. Ceram. Int. 44, 10028–10034 (2018)
C.D. Chandler, C. Roger, M.J. Hampdensmith, Chemical aspects of solution routes to perovskite-phase mixed-metal oxides from metal-organic precursors. Chem. Rev. 93, 1205–1241 (1993)
M.A. Pena, J.L.G. Fierro, Chemical structures and performance of perovskite oxides. Chem. Rev. 101, 1981–2017 (2001)
J. Harada, T. Pedersen, Z. Barnea, X-Ray and neutron diffraction study of tetragonal barium titanate. Acta Crystall. a-Crys. A 26, 336 (1970)
F.I.H. Rhouma, A. Dhahri, J. Dhahri, H. Belmabrouk, M.A. Valente, Structural and dielectric properties of Ba0.8La0.133Ti0.90Sn0.1O3. Solid State Commun. 152, 1874–1879 (2012)
M.Z.C. Hu, G.A. Miller, E.A. Payzant, C.J. Rawn, Homogeneous (co)precipitation of inorganic salts for synthesis of monodispersed barium titanate particles. J. Mater. Sci. 35, 2927–2936 (2000)
S. Dudley, T. Kalem, M. Akinc, Conversion of SiO2 diatom frustules to BaTiO3 and SrTiO3. J. Am. Ceram. Soc. 89, 2434–2439 (2006)
V. Paunovic, L. Zivkovic, Influence of Rare-earth additives (La, Sm and Dy) on the microstructure and dielectric properties of doped BaTiO3 ceramics. Sci. Sinter. 42, 69–79 (2010)
H.A. Moghaddam, M.R. Mohammadi, TiO2-BaTiO3 nanocomposite for electron capture in dye-sensitized solar cells. J. Am. Ceram. Soc. 100, 2144–2153 (2017)
H.A. Moghaddam, M.R. Mohammadi, S.M.S. Reyhani, Improved photon to current conversion in nanostructured TiO2 dye-sensitized solar cells by incorporating cubic BaTiO3 particles deliting incident. Sol. Energy 132, 1–14 (2016)
Y.M. Zhang, M.H. Cao, Z.H. Yao, Z.J. Wang, Z. Song, A. Ullah, H. Hao, H.X. Liu, Effects of silica coating on the microstructures and energy storage properties of BaTiO3 ceramics. Mater. Res. Bull. 67, 70–76 (2015)
W.H. Tzing, W.H. Tuan, H.L. Lin, The effect of microstructure on the electrical properties of NiO-doped BaTiO3. Ceram. Int. 25, 425–430 (1999)
T. Nagai, K. Iijima, H.J. Hwang, M. Sando, T. Sekino, K. Niihara, Effect of MgO doping on the phase transformations of BaTiO3. J. Am. Ceram. Soc. 83, 107–112 (2000)
Y. Sakabe, N. Wada, T. Hiramatsu, T. Tonogaki, Dielectric properties of fine-grained BaTiO3 ceramics doped with CaO. Jpn. J. Appl. Phys. 41, 6922–6925 (2002)
Y.H. Song, J.H. Hwang, Y.H. Han, Effects of Y2O3 on temperature stability of acceptor-doped BaTiO3. Jpn. J. Appl. Phys. 44, 1310–1313 (2005)
R. Saravanan, V.K. Gupta, E. Mosquera, F. Gracia, Preparation and characterization of V2O5/ZnO nanocomposite system for photocatalytic application. J. Mol. Liq. 198, 409–412 (2014)
A.M. Al-syadi, V.K. Gupta, E. Mosquera, M.M. El-Desoky, M.S. Al-Assiri, Impedance spectroscopy of V2O5–Bi2O3–BaTiO3 glass–ceramics. Solid State Sci. 26, 72–82 (2014)
N. Zhang, L. Li, J. Chen, J. Yu, ZnO-doped BaTiO3-Na0.5Bi0.5TiO3-Nb2O5-based ceramics with temperature-stable high permittivity from − 55 °C to 375 °C. Mater. Lett. 138, 228–230 (2015)
T. Wang, X. Wei, Q. Hu, L. Jin, Z. Xu, Y. Feng, Effects of ZnNb2O6 addition on BaTiO3 ceramics for energy storage. Mater. Sci. Eng. B 178, 1081–1086 (2013)
Y. Yan, C. Ning, Z. Jin, H. Qin, W. Luo, G. Liu, The dielectric properties and microstructure of BaTiO3 ceramics with ZnO–Nb2O5 composite addition. J. Alloys. Compd. 646, 748–752 (2015)
Q.K. Muhammad, M. Waqar, M.A. Rafiq, M.N. Rafiq, M. Usman, M.S. Anwar, Structural, dielectric, and impedance study of ZnO doped barium zirconium titanate (BZT) ceramics. J. Mater. Sci. 51, 10048–10058 (2016)
Y. Iqbal, A. Jamal, The effect of Ta2O5- and ZnO-doping on the Curie temperature of BaTiO3. J. Phys 371, 012035 (2012)
A.C. Caballero, J.F. Fernández, C. Moure, P. Durán, Y.M. Chiang, Grain growth control and dopant distribution in ZnO-doped BaTiO3. J. Am. Ceram. Soc. 81, 939–944 (1998)
M. Atif, S. Ahmed, M. Nadeem, M.K. Ali, M. Idrees, R. Grossinger, R.S. Turtelli, Role of competing phases in the structural, magnetic and dielectric relaxation for (1 − x)CoFe2O4 + (x)BaTiO3 composites. Ceram. Int. 42, 14618–14626 (2016)
S. Lather, A. Gupta, J. Dalal, V. Verma, R. Tripathi, A. Ohlan, Effect of mechanical milling on structural, dielectric and magnetic properties of BaTiO3-Ni0.5Co0.5Fe2O4 multiferroic nanocomposites. Ceram. Int. 43, 3246–3251 (2016)
S. Kappadan, T.W. Gebreab, S. Thomas, N. Kalarikkal, Tetragonal BaTiO3 nanoparticles: an efficient photocatalyst for the degradation of organic pollutants. Mater. Sci. Semicond. Process 51, 42–47 (2016)
Y. Yan, L. Liu, C. Ning, Y. Yang, C.J. Xia, Y.T. Zou, S.Y. Liu, X.X. Wang, K.H. Liu, X.K. Liu, G. Liu, Improved electrical properties of SiO2-added BaTiO3 ceramics by microwave sintering. Mater. Lett. 165, 135–138 (2016)
Y. Slimani, H. Gungunes, M. Nawaz, A. Manikandan, H.S. El Sayed, M.A. Almessiere, H. Sozeri, S.E. Shirsath, I. Ercan, A. Baykal, Magneto-optical and microstructural properties of spinel cubic copper ferrites with Li-Al co-substitution. Ceram. Int. 44, 14242–14250 (2018)
P.G. Wang, C.M. Fan, Y.W. Wang, G.Y. Ding, P.H. Yuan, A dual chelating sol-gel synthesis of BaTiO3 nanoparticles with effective photocatalytic activity for removing humic acid from water. Mater. Res. Bull. 48, 869–877 (2013)
Z.A. Garmaroudi, M.R. Mohammadi, Design of TiO2 dye-sensitized solar cell photoanode electrodes with different microstructures and arrangement modes of the layers. J. Sol–Gel Sci. Techn. 76, 666–678 (2015)
Y.C. Teh, A.A. Saif, Influence of annealing temperature on structural and optical properties of sol-gel derived Ba0.9Gd0.1TiO3 thin films for optoelectronics. J. Alloys. Compd. 703, 407–413 (2015)
L.V. Maneeshya, P.V. Thomas, K. Joy, Effects of site substitutions and concentration on the structural, optical and visible photoluminescence properties of Er doped BaTiO3 thin films prepared by RF magnetron sputtering. Opt. Mater. 46, 304–309 (2015)
T.G. Reddy, B.R. Kumar, T.S. Rao, J.A. Ahmad, Structural and dielectric properties of barium bismuth titanate (BaBi4Ti4O15) ceramics. Int. J. Appl. Eng. Res. 6, 571–580 (2011)
P. Jaita, A. Watcharapasorn, N. Kumar, D.P. Cann, S. Jiansirisomboon, Large electric field-induced strain and piezoelectric responses of lead-free Bi0.5(Na0.80K0.20)0.5TiO3-Ba(Ti0.90Sn0.10)O3 ceramics near morphotropic phase boundary. Electron. Mater. Lett. 11, 828–835 (2011)
X.X. Dong, H.W. Chen, M. Wei, K.T. Wu, J.H. Zhang, Structure, dielectric and energy storage properties of BaTiO3 ceramics doped with YNbO4. J. Alloys. Compd. 744, 721–727 (2018)
K. Kumari, A. Prasad, K. Prasad, Dielectric, Impedance/modulus and conductivity studies on [Bi0.5(Na1-xKx)0.5]0.94Ba0.06TiO3,[0.16 ≤ x ≤ 0.20] leadfree ceramics. Am. J. Mater. Sci. 6, 1–8 (2016)
A.K. Jonscher, The ‘universal’dielectric response. Nature 267, 673 (1977)
L. Singh, U.S. Rai, K. Mandal, B.C. Sin, S.I. Lee, Y. Lee, Dielectric, AC-impedance, modulus studies on 0.5BaTiO3· 0.5CaCu3Ti4O12 nano-composite ceramic synthesized by one-pot, glycine-assisted nitrate-gel route. Ceram. Int. 40, 10073–10083 (2014)
A. Rouahi, A. Kahouli, F. Challali, M.-P. Besland, C. Vallée, B. Yangui, S. Salimy, A. Goullet, A. Sylvestre, Impedance and electric modulus study of amorphous TiTaO thin films: highlight of the interphase effect. J. Phys. D 46, 065308 (2013)
A. Selmi, O. Khaldi, M. Mascot, F. Jomni, J. Carru, Dielectric relaxations in Ba0.85Sr0.15TiO3 thin films deposited on Pt/Ti/SiO2/Si substrates by sol–gel method. J. Mater. Sci. 27, 11299–11307 (2016)
M. Sahu, S.K. Pradhan, S. Hajra, B.K. Panigrahi, R. Choudhary, Studies of structural, electrical, and excitation performance of electronic material: europium substituted 0.9(Bi0.5Na0.5TiO3)–0.1(PbZr0.48Ti0.52O3). Appl. Phys. A 125, 183 (2019)
C. Rayssi, S.E. Kossi, J. Dhahri, K. Khirouni, Frequency and temperature-dependence of dielectric permittivity and electric modulus studies of the solid solution Ca0.85Er0.1Ti1−xCo4x/3O3 (0 ≤ x ≤ 0.1). RSC Adv. 8, 17139–17150 (2018)
R. Schmidt, S. Pandey, P. Fiorenza, D.C. Sinclair, Non-stoichiometry in “CaCu3Ti4O12” (CCTO) ceramics. RSC Adv. 3, 14580–14589 (2013)
A. Rouahi, A. Kahouli, A. Sylvestre, E. Defay, B. Yangui, Impedance spectroscopic and dielectric analysis of Ba0.7Sr0.3TiO3 thin films. J. Alloys. Compd. 529, 84–88 (2012)
Acknowledgments
The authors highly acknowledged the supports of the Institute for Research & Medical Consultations (Projects application No. 2017-IRMC-S-3, No. 2017-576-IRMC and No. 2018-IRMC-S-2) of Imam Abdulrahman Bin Faisal University (IAU—Saudi Arabia).
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Slimani, Y., Selmi, A., Hannachi, E. et al. Impact of ZnO addition on structural, morphological, optical, dielectric and electrical performances of BaTiO3 ceramics. J Mater Sci: Mater Electron 30, 9520–9530 (2019). https://doi.org/10.1007/s10854-019-01284-2
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DOI: https://doi.org/10.1007/s10854-019-01284-2