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Study of hydrogenation processes in radiation-resistant nitride ceramics

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Abstract

This paper presents the results of studying the processes of defect formation caused by irradiation with protons with an energy of 1.5 MeV and doses of 1 × 1015, 1 × 1016, 1 × 1017 ion/cm2 in ceramics based on aluminum nitride. The choice of radiation doses is due to the possibility of modeling atomic displacement (dpa) values of 0.56, 5.6, and 56 dpa, respectively. An analysis of structural changes showed a significant stability of the crystal structure at irradiation doses comparable to 0.56, 5.6, while an increase in the displacements up to 56 dpa leads to a significant increase in distortions of the crystal structure and its disordering due to the effect of accumulation of defects in the structure, as well as to hydrogenation processes. The totality of the data obtained indicates a fairly high degree of resistance to proton irradiation and the subsequent evolution of defects in the structure of nitride ceramics; however, at high doses of radiation, microcracks form in the surface layer, which leads to a sharp deterioration in the strength properties due to a large number of dislocation and point defects.

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References

  1. Z. Du et al., The sound absorption properties of highly porous silicon nitride ceramic foams. J. Alloys Compd. 820, 153067 (2020)

    CAS  Google Scholar 

  2. X. Xiao, Y. Long, Nano-indentation of ion-irradiated nuclear structural materials: a review. Nucl. Mater. Energy 22, 100721 (2019)

    Google Scholar 

  3. Y. Al-Douri, Structural phase transition of boron nitride compound. Solid State Commun. 132(7), 465–470 (2004)

    CAS  Google Scholar 

  4. J.H. Harris, Sintered aluminum nitride ceramics for high-power electronic applications. JOM 50(6), 56–60 (1998)

    CAS  Google Scholar 

  5. O. Boudrifa et al., First-principles prediction of the structural, elastic, thermodynamic, electronic and optical properties of Li4Sr3Ge2N6 quaternary nitride. J. Alloy. Compd. 618, 84–94 (2015)

    CAS  Google Scholar 

  6. A. Rais et al., Copper substitution effect on the structural properties of nickel ferrites. Ceram. Int. 40(9), 14413–14419 (2014)

    CAS  Google Scholar 

  7. A. Neumann et al., Comparative investigation of the biocompatibility of various silicon nitride ceramic qualities in vitro. J. Mater. Sci. 15(10), 1135–1140 (2004)

    CAS  Google Scholar 

  8. A. Bouhemadou et al., Structural, elastic, electronic, chemical bonding and optical properties of Cu-based oxides ACuO (A= Li, Na, K and Rb): An ab initio study. Comput. Mater. Sci. 81, 561–574 (2014)

    CAS  Google Scholar 

  9. D. Prakash et al., Synthesis, purification and microstructural characterization of nickel doped carbon nanotubes for spintronic applications. Ceram. Int. 42(5), 5600–5606 (2016)

    CAS  Google Scholar 

  10. M.H. Bocanegra-Bernal, B. Matovic, Mechanical properties of silicon nitride-based ceramics and its use in structural applications at high temperatures. Mater. Sci. Eng. A 527(6), 1314–1338 (2010)

    Google Scholar 

  11. R. Al-Gaashani et al., XPS and optical studies of different morphologies of ZnO nanostructures prepared by microwave methods. Ceram. Int. 39(3), 2283–2292 (2013)

    CAS  Google Scholar 

  12. M.E.A. Monir et al., Doping-induced half-metallic ferromagnetism in vanadium and chromium-doped alkali oxides K2O and Rb2O: Ab initio method. J. Supercond. Novel Magn. 30(8), 2197–2210 (2017)

    Google Scholar 

  13. A. Bouhemadou et al., Electronic, optical, elastic, thermoelectric and thermodynamic properties of the spinel oxides ZnRh2O4 and CdRh2O4. J. Alloys Compd. 774, 299–314 (2019)

    CAS  Google Scholar 

  14. T.F. Mokgadi et al., Slow and swift heavy ions irradiation of zirconium nitride (ZrN) and the migration behaviour of implanted Eu. Nucl. Instrum. Methods Phys. Res. Sect. B 461, 63–69 (2019)

    CAS  Google Scholar 

  15. H.A. Vasco et al., Effect of swift heavy ion irradiation in the migration behavior of Xe implanted into TiN. Vacuum 163, 59–68 (2019)

    CAS  Google Scholar 

  16. Z. Wu, Wu Yiming, Q. Wang, A comparative investigation on structure evolution of ZrN and CrN coatings against ion irradiation. Heliyon 5(3), e01370 (2019)

    Google Scholar 

  17. W. Werdecker, F. Aldinger, Aluminum nitride-an alternative ceramic substrate for high power applications in microcircuits. IEEE Trans. Compon. Hybrids Manuf. Technol. 7(4), 399–404 (1984)

    Google Scholar 

  18. F.V. Konusov et al., Effect of short-pulsed ion irradiation on the optical and electrical properties of pyrolytic boron nitride. Nucl. Instrum. Methods Phys. Res. Sect. B 447, 1–7 (2019)

    CAS  Google Scholar 

  19. C. Luo et al., Ionoluminescence and photoluminescence study of annealing and ion irradiation effects on zinc oxide. Nucl. Instrum. Methods Phys. Res. Sect. B 471, 7–12 (2020)

    CAS  Google Scholar 

  20. A. L. Kozlovskiy, Study of Optical Properties of Irradiated AlN Ceramic. 13th International Conference “Interaction of Radiation with Solids”, September 30–October 3, 2019, Minsk, Belarus 107–108 (2019)

  21. K. Ikeue, Y. Yamamoto, M. Suzuki, Photocatalytic activity for hydrogen evolution of heteroatom-doped SrTiO3 prepared using a graphitic-carbon nitride nanosheet. Ceramics 3(1), 22–30 (2020)

    Google Scholar 

  22. M.V. Zdorovets et al., Study of helium swelling in nitride ceramics at different irradiation temperatures. Materials 12(15), 2415 (2019)

    CAS  Google Scholar 

  23. J. Ward et al., Influence of proton-irradiation temperature on the damage accumulation in Ti3SiC2 and Ti3AlC2. Scripta Mater. 165, 98–102 (2019)

    CAS  Google Scholar 

  24. K.A. Smith et al., Effect of proton irradiation on anatase TiO2 nanotube anodes for lithium-ion batteries. J. Mater. Sci. 54, 13221–13235 (2019)

    CAS  Google Scholar 

  25. J.-P. Shen et al., Proton-implanted waveguides in neodymium-doped calcium lithium niobium gallium garnet crystals. Results Phys. 15, 102794 (2019)

    Google Scholar 

  26. I.I. Bardyshev et al., Positron nondestructive testing of gamma-neutron irradiated boron nitride ceramics. Prot. Metals Phys. Chem. Surf. 55(5), 1015–1018 (2019)

    CAS  Google Scholar 

  27. J. Tang et al., Effect of proton irradiation on the mobility of two-dimensional electron in AlGaN/AlN/GaN high electron mobility transistors at low temperature. J. Vacuum Sci. Technol. B 38, 023202 (2020)

    Google Scholar 

  28. B. Buyuk et al., Swelling on neutron induced hexagonal boron nitride and hexagonal boron nitride-titanium diboride composites. Vacuum 2, 109350 (2020)

    Google Scholar 

  29. A. Bhattacharya et al., Nano-scale microstructure damage by neutron irradiations in a novel Boron-11 enriched TiB2 ultra-high temperature ceramic. Acta Mater. 165, 26–39 (2019)

    CAS  Google Scholar 

  30. S. Agarwal et al., Neutron irradiation-induced microstructure damage in ultra-high temperature ceramic TiC. Acta Mater. 186, 1–10 (2020)

    CAS  Google Scholar 

  31. T. Koyanagi et al., Progress in development of SiC-based joints resistant to neutron irradiation. J. Eur. Ceram. Soc. 40, 1023–1034 (2020)

    CAS  Google Scholar 

  32. T. Nozawa et al., High-dose, intermediate-temperature neutron irradiation effects on silicon carbide composites with varied fiber/matrix interfaces. J. Eur. Ceram. Soc. 39(8), 2634–2647 (2019)

    CAS  Google Scholar 

  33. G.S. Was, Fundamentals of Radiation Materials Science: Metals and Alloys (Springer, New York, 2016)

    Google Scholar 

  34. T. Yano et al., Neutron irradiation damage in aluminum oxide and nitride ceramics up to a fluence of 4.2 × 1026 n/m2. J. Nucl. Mater. 283, 947–951 (2000)

    Google Scholar 

  35. K. Dukenbayev et al., Investigation of radiation resistance of AlN ceramics. Vacuum 159, 144–151 (2019)

    CAS  Google Scholar 

  36. M. Zdorovets et al., Defect formation in AlN after irradiation with He2+ ions. Ceram. Int. 45(7), 8130–8137 (2019)

    CAS  Google Scholar 

  37. D.M. Spiridonov et al., Spectrally resolved thermoluminescence in electron irradiated AlN submicrocrystals. Radiat. Meas. 122, 91–96 (2019)

    CAS  Google Scholar 

  38. T. Gladkikh et al., Changes in optical and structural properties of AlN after irradiation with C2+ ions of 40 keV. Vacuum 161, 103–110 (2019)

    CAS  Google Scholar 

  39. A. Kozlovskiy et al., Investigation of the radiation resistance of nitride ceramics during irradiation with low-energy. Mater. Res. Express 6(1), 016416 (2018)

    Google Scholar 

  40. K. Dukenbayev et al., The investigation of various type irradiation effects on aluminum nitride ceramic. J. Mater. Sci. 30(9), 8777–8787 (2019)

    CAS  Google Scholar 

  41. J.P. Ziegler, M. D. Ziegler, J. P. Biersack. The program stopping and Range of Ion in Matter (SRIM) 2013 Pro." (2018).

  42. A.V. Trukhanov et al., Control of electromagnetic properties in substituted M-type hexagonal ferrites. J. Alloy. Compd. 754, 247–256 (2018)

    CAS  Google Scholar 

  43. S.V. Trukhanov et al., Crystal structure and magnetic properties of the BaFe12− xInxO19 (x = 0.1–1.2) solid solutions. J. Magn. Magn. Mater. 417, 130–136 (2016)

    CAS  Google Scholar 

  44. T.I. Zubar et al., Anomalies in growth of electrodeposited Ni–Fe nanogranular films. CrystEngComm 21(14), 2464–2464 (2019)

    CAS  Google Scholar 

  45. T.I. Zubar et al., Anomalies in Ni-Fe nanogranular films growth. J. Alloy. Compd. 748, 970–978 (2018)

    CAS  Google Scholar 

  46. A.V. Trukhanov et al., Crystal structure and magnetic properties of the BaFe12− xAlxO19 (x= 0.1–1.2) solid solutions. J. Magn. Magn. Mater. 393, 253–259 (2015)

    CAS  Google Scholar 

Download references

Funding

This research was funded by the Science Committee of the Ministry of Education and Science of the Republic of Kazakhstan (No. AP08051975).

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Correspondence to A. L. Kozlovskiy.

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Kozlovskiy, A.L., Zdorovets, M.V. Study of hydrogenation processes in radiation-resistant nitride ceramics. J Mater Sci: Mater Electron 31, 11227–11237 (2020). https://doi.org/10.1007/s10854-020-03671-6

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  • DOI: https://doi.org/10.1007/s10854-020-03671-6

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