Abstract
The purpose of this research was to study chemical characteristics of precipitation in Peradeniya (Latitude 6.973701, Longitude 79.915256), Kandy District in Sri Lanka. This study was conducted during 2012 to 2014, and wet precipitation was analyzed for pH, conductivity, Na+, NH4+, K+, Mg2+, Ca2+, F−, Cl−, NO3−, SO42−, Pb, Cu, Mn, Al, Zn, and Fe for a total of 125 samples. Less than 2% events of acidic precipitation were recorded, and the VWA of the major ionic species present in precipitation samples were in the order of Ca2+ > Na+ > Cl− > NH4+ > SO42− > K+ > NO3− > Mg2+. Neutralization of acidity of precipitation is much more related to CaCO3 than NH3, and the presence of high content of Ca2+ strongly supports this fact. When considering marine contribution, SO42−/Na+, Ca2+/Na+, Mg2+/Na+, and K+/Na+ ratios are higher than the reference value suggesting that contribution of sources other than marine. Concentration of Zn is the highest while that of Mn is the lowest. Principal component analysis identified probable sources for major ionic and elemental sources as both natural and anthropogenic sources such as vehicular emission due to heavy traffic, waste incineration, bio mass burning, brass industry, and construction.
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References
Alastuey, A., Querol, X., Chaves, A., Lopezsoler, A., & Ruiz, C. R. (2001). Wet-only sequential deposition in a rural area in north-eastern Spain. Tellus Series B: Chemical and Physical Meteorology, 53, 40–52. https://doi.org/10.3402/tellusb.v53i1.16535.
Alkhashman, O. (2005). Study of chemical composition in wet atmospheric precipitation in Eshidiya area, Jordan. Atmospheric Environment, 39, 6175–6183. https://doi.org/10.1016/j.atmosenv.2005.06.056.
Amodio, M., Catino, S., Dambruoso, P. R., de Gennaro, G., Di Gilio, A., Giungato, P., & Tutino, M. (2014). Atmospheric deposition: sampling procedures, analytical methods, and main recent findings from the scientific literature. Advances in Meteorology, 2014, 27. https://doi.org/10.1155/2014/161730.
Bhaskar, V. V., & Rao, P. S. P. (2017). Annual and decadal variation in chemical composition of rain water at all the ten GAW stations in India. Journal of Atmospheric Chemistry, 74(1), 23–53. https://doi.org/10.1007/s10874-016-9339-3.
Bisht, D. S., Srivastava, A. K., Joshi, H., Ram, K., Singh, N., Naja, M., & Tiwari, S. (2017). Chemical characterization of rainwater at a high-altitude site “Nainital” in the central Himalayas, India. Environmental Science and Pollution Research, 24(4), 3959–3969. https://doi.org/10.1007/s11356-016-8093-z.
Cao, Y. Z., Wang, S., Zhang, G., Luo, J., & Lu, S. (2009). Chemical characteristics of wet precipitation at an urban site of Guangzhou, South China. Atmospheric Research, 94(3), 462–469. https://doi.org/10.1016/j.atmosres.2009.07.004.
Carvalho, S. C. P., de Lima, J. L. M. P., & de Lima, M. I. P. (2014). Rainwater sequential sampler: assessing intra-event water composition variability. Journal of Engineering and Technology Research, 1(1), 1–7http://journal.iugaza.edu.ps/index.php/JERT/article/view/26.
Chathuranga, R. A. J., Liyandeniya, A. B., Dharmapriya, T. N., Deeyamulla, M. P., & Priyantha, N. (2020). Risk assessment and source apportionment of wet bulk deposition in three typical sites of Gampaha District, Sri Lanka. SN Applied Sciences, 2, 1394. https://doi.org/10.1007/s42452-020-3007-6.
Chen, L., Peng, S., Liu, J., & Hou, Q. (2012). Dry deposition velocity of total suspended particles and meteorological influence in four locations in Guangzhou, China. Journal of Environmental Sciences, 24(4), 632–639. https://doi.org/10.1016/S1001-0742(11)60805-X.
Ghorani-Azam, A., Riahi-Zanjani, B., & Balali-Mood, M. (2016). Effects of air pollution on human health and practical measures for prevention in Iran. Journal of Research in Medical Sciences, 21(5), 65. https://doi.org/10.4103/1735-1995.189646.
Herrera, J., Rodríguez, S., & Baéz, A. P. (2009). Chemical composition of bulk precipitation in the metropolitan area of Costa Rica, Central America. Atmospheric Research, 94(2), 151–160. https://doi.org/10.1016/j.atmosres.2009.05.004.
Huang, Y., Wang, Y., & Zhang, L. (2008a). Long-term trend of chemical composition of wet atmospheric precipitation during 1986-2006 at Shenzhen City, China. Atmospheric Environment, 42(16), 3740–3750. https://doi.org/10.1016/j.atmosenv.2007.12.063.
Huang, K., Zhuang, G., Xu, C., Wang, Y., & Tang, A. (2008b). The chemistry of the severe acidic precipitation in Shanghai, China. Atmospheric Research, 89(1–2), 149–160. https://doi.org/10.1016/j.atmosres.2008.01.006.
Huang, F., Zhou, J., Chen, N., Li, Y., Li, K., & Wu, S. (2019). Chemical characteristics and source apportionment of PM2.5 in Wuhan, China. Journal of Atmospheric Research, 76(3), 245–262. https://doi.org/10.1007/s10874-019-09395-0.
Ileperuma, O. (2015). Model assessment of acid deposition potential by SOx in Sri Lanka. Journal of the National Science Foundation of Sri Lanka, 43(3), 281. https://doi.org/10.4038/jnsfsr.v43i3.7956.
Jayalath, K. G., Deeyamulla, M. P., & de Silva, R. C. L. (2020). Atmospheric deposition of polycyclic aromatic hydrocarbons (PAHs) around two metropolitan areas in Sri Lanka using moss as a biomonitor. Pollution Research, 39(3), 626–631.
Kim, Y., Wellum, G., Mello, K., Strawhecker, K. E., Thoms, R., Giaya, A., & Wyslouzil, B. E. (2016). Effects of relative humidity and particle and surface properties on particle resuspension rates. Aerospace Science and Technology, 50(4), 339–352. https://doi.org/10.1080/02786826.2016.1152350.
Lee, B. K., Hong, S. H., & Lee, D. S. (2000). Chemical composition of precipitation and wet deposition of major ions on the Korean peninsula. Atmospheric Environment, 34(4), 563–575. https://doi.org/10.1016/S1352-2310(99)00225-3.
Li, Y. C., Zhang, M., Shu, M., Ho, S. S. H., Liu, Z. F., Wang, X. X., & Zhao, X. Q. (2016). Chemical characteristics of rainwater in Sichuan basin, a case study of Ya’an. Environmental Science and Pollution Research, 23(13), 13088–13099. https://doi.org/10.1007/s11356-016-6363-4.
Liyandeniya, A. B., Deeyamulla, M. P., & Priyantha, N. (2020a). Atmospheric chemical composition of bulk deposition at two geographically distinct locations in Sri Lanka. Environmental Monitoring and Assessment, 192(452), 452. https://doi.org/10.1007/s10661-020-08412-0.
Liyandeniya, A. B., Deeyamulla, M. P., & Priyantha, N. (2020b). Source apportionment of rainwater chemical composition in wet precipitation at Kelaniya in Sri Lanka. Air Quality and Atmospheric Health. https://doi.org/10.1007/s11869-020-00903-w.
Mahato, K., Singh, K., Singh, K., & Tiwari, K. (2016). Assessment of major ionic compositions and anthropogenic influences in the rainwater over a coal mining environment of Damodar River basin, India. Pollution, 2(4), 461–474. https://doi.org/10.7508/pj.2016.04.008.
Martins, E. H., Nogarotto, D. C., Mortatti, J., & Pozza, S. A. (2019). Chemical composition of rainwater in an urban area of the southeast of Brazil. Atmospheric Pollution Research, 10(2), 520–530. https://doi.org/10.1016/j.apr.2018.10.003.
Migliavacca, D., Teixeira, E., Wiegand, F., Machado, A., & Sanchez, J. (2005). Atmospheric precipitation and chemical composition of an urban site, Guaba hydrographic basin, Brazil. Atmospheric Environment, 39(10), 1829–1844. https://doi.org/10.1016/j.atmosenv.2004.12.005.
Morales-Baquero, R., Pulido-Villena, E., & Reche, I. (2013). Chemical signature of saharan dust on dry and wet atmospheric deposition in the south-western mediterranean region. Tellus Series B: Chemical and Physical Meteorology, 65(1), 1–12. https://doi.org/10.3402/tellusb.v65i0.18720.
Park, S. M., Seo, B. K., Lee, G., Kahng, S. H., & Jang, Y. (2015). Chemical composition of water soluble inorganic species in precipitation at Shihwa Basin, Korea. Atmosphere, 6(6), 732–750. https://doi.org/10.3390/atmos6060732.
Rao, P. S. P., Tiwari, S., Matwale, J. L., Pervez, S., Tunved, P., Safai, P. D., & Hopke, P. K. (2016). Sources of chemical species in rainwater during monsoon and non-monsoonal periods over two mega cities in India and dominant source region of secondary aerosols. Atmospheric Environment, 146, 90–99. https://doi.org/10.1016/j.atmosenv.2016.06.069.
Rathnayaka, I. M. S. K., Dharmapriya, T. N., Liyandeniya, A. B., Deeyamulla, M. P., & Priyantha, N. (2020). Trace metal composition of bulk precipitation in selected locations of Kandy District, Sri Lanka. Water, Air, & Soil Pollution, 231, 492. https://doi.org/10.1007/s11270-020-04840-3.
Sakihama, H., Ishiki, M., & Tokuyama, A. (2008). Chemical characteristics of precipitation in Okinawa Island, Japan. Atmospheric Environment, 42(10), 2320–2335. https://doi.org/10.1016/j.atmosenv.2007.12.026.
Schröder, W., Nickel, S., Schönrock, S., Schmalfuß, R., Wosniok, W., Meyer, M., & Zechmeister, H. G. (2017). Bioindication and modelling of atmospheric deposition in forests enable exposure and effect monitoring at high spatial density across scales. Annals of Forest Science, 74(2), 31. https://doi.org/10.1007/s13595-017-0621-6.
Shi, X. M., Song, L., Liu, W. Y., Lu, H. Z., Qi, J. H., Li, S., & Wu, C. S. (2017). Epiphytic bryophytes as bio-indicators of atmospheric nitrogen deposition in a subtropical montane cloud forest: response patterns, mechanism, and critical load. Environmental Pollution, 229, 932–941. https://doi.org/10.1016/j.envpol.2017.07.077.
Tositti, L., Pieri, L., Brattich, E., Parmeggiani, S., & Ventura, F. (2018). Chemical characteristics of atmospheric bulk deposition in a semi-rural area of the Po Valley (Italy). Journal of Atmospheric Chemistry, 75(1), 97–121. https://doi.org/10.1007/s10874-017-9365-9.
Weerasundara, L., Amarasekara, R. W. K., Magana-Arachchi, D. N., Ziyath, A. M., Karunaratne, D. G. G. P., Goonetilleke, A., & Vithanage, M. (2017). Microorganisms and heavy metals associated with atmospheric deposition in a congested urban environment of a developing country: Sri Lanka. Science of the Total Environment, 584–585, 803–812. https://doi.org/10.1016/j.scitotenv.2017.01.121.
Weerasundara, L., Magana-Arachchi, D. N., Ziyath, A. M., Goonetilleke, A., & Vithanage, M. (2018). Health risk assessment of heavy metals in atmospheric deposition in a congested city environment in a developing country: Kandy City, Sri Lanka. Journal of Environmental Management, 220, 198–206. https://doi.org/10.1016/j.jenvman.2018.04.036.
Weyhenmeyer, G. A., & Karlsson, J. (2009). Nonlinear response of dissolved organic carbon concentrations in boreal lakes to increasing temperatures. Limnology and Oceanography, 54(6 PART 2), 2513–2519. https://doi.org/10.4319/lo.2009.54.6_part_2.2513.
Wu, Q., & Han, G. (2015). Sulfur isotope and chemical composition of the rainwater at the three gorges reservoir. Atmospheric Research, 155, 130–140. https://doi.org/10.1016/j.atmosres.2014.11.020.
Yu, H., He, N., Wang, Q., Zhu, J., Gao, Y., Zhang, Y., & Yu, G. (2017). Development of atmospheric acid deposition in China from the 1990s to the 2010s. Environmental Pollution, 231(3), 182–190. https://doi.org/10.1016/j.envpol.2017.08.014.
Zhang, M., Wang, S., Wu, F., Yuan, X., & Zhang, Y. (2007). Chemical compositions of wet precipitation and anthropogenic influences at a developing urban site in southeastern China. Atmospheric Research, 84(4), 311–322. https://doi.org/10.1016/j.atmosres.2006.09.003.
Zhu, G., Guo, Q., Chen, T., Lang, Y., Peters, M., Tian, L., & Wang, C. (2016). Chemical and sulfur isotopic composition of precipitation in Beijing, China. Environmental Science and Pollution Research, 23(6), 5507–5515. https://doi.org/10.1007/s11356-015-5746-2.
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This study received financial support from the National Research Council of Sri Lanka (Grant No. NRC/11/127) in providing equipment and other expenses.
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Liyandeniya, A.B., Deeyamulla, M.P., Abeysundara, S.P. et al. Chemical characteristics of wet precipitation at Peradeniya in Sri Lanka. Environ Monit Assess 193, 14 (2021). https://doi.org/10.1007/s10661-020-08772-7
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DOI: https://doi.org/10.1007/s10661-020-08772-7