Metallurgical and Materials Transactions A

, Volume 45, Issue 1, pp 85–97

A Next-Generation Hard X-Ray Nanoprobe Beamline for In Situ Studies of Energy Materials and Devices

  • Jörg Maser
  • Barry Lai
  • Tonio Buonassisi
  • Zhonghou Cai
  • Si Chen
  • Lydia Finney
  • Sophie-Charlotte Gleber
  • Chris Jacobsen
  • Curt Preissner
  • Chris Roehrig
  • Volker Rose
  • Deming Shu
  • David Vine
  • Stefan Vogt
Symposium: Neutron and X-Ray Studies of Advanced Materials VI: Diffraction Centennial and Beyond

DOI: 10.1007/s11661-013-1901-x

Cite this article as:
Maser, J., Lai, B., Buonassisi, T. et al. Metall and Mat Trans A (2014) 45: 85. doi:10.1007/s11661-013-1901-x

Abstract

The Advanced Photon Source is developing a suite of new X-ray beamlines to study materials and devices across many length scales and under real conditions. One of the flagship beamlines of the APS upgrade is the In Situ Nanoprobe (ISN) beamline, which will provide in situ and operando characterization of advanced energy materials and devices under varying temperatures, gas ambients, and applied fields, at previously unavailable spatial resolution and throughput. Examples of materials systems include inorganic and organic photovoltaic systems, advanced battery systems, fuel cell components, nanoelectronic devices, advanced building materials and other scientifically and technologically relevant systems. To characterize these systems at very high spatial resolution and trace sensitivity, the ISN will use both nanofocusing mirrors and diffractive optics to achieve spots sizes as small as 20 nm. Nanofocusing mirrors in Kirkpatrick–Baez geometry will provide several orders of magnitude increase in photon flux at a spatial resolution of 50 nm. Diffractive optics such as zone plates and/or multilayer Laue lenses will provide a highest spatial resolution of 20 nm. Coherent diffraction methods will be used to study even small specimen features with sub-10 nm relevant length scale. A high-throughput data acquisition system will be employed to significantly increase operations efficiency and usability of the instrument. The ISN will provide full spectroscopy capabilities to study the chemical state of most materials in the periodic table, and enable X-ray fluorescence tomography. Insitu electrical characterization will enable operando studies of energy and electronic devices such as photovoltaic systems and batteries. We describe the optical concept for the ISN beamline, the technical design, and the approach for enabling a broad variety of in situ studies. We furthermore discuss the application of hard X-ray microscopy to study defects in multi-crystalline solar cells, one of the lines of inquiries for which the ISN is being developed.

Copyright information

© The Minerals, Metals & Materials Society and ASM International 2013

Authors and Affiliations

  • Jörg Maser
    • 1
  • Barry Lai
    • 1
  • Tonio Buonassisi
    • 2
  • Zhonghou Cai
    • 1
  • Si Chen
    • 1
  • Lydia Finney
    • 1
  • Sophie-Charlotte Gleber
    • 1
  • Chris Jacobsen
    • 1
  • Curt Preissner
    • 1
  • Chris Roehrig
    • 1
  • Volker Rose
    • 1
  • Deming Shu
    • 1
  • David Vine
    • 1
  • Stefan Vogt
    • 1
  1. 1.Argonne National LabArgonneUSA
  2. 2.Massachusetts Institute of TechnologyCambridgeUSA

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