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Preparation of NiCoP-decorated g-C3N4 as an efficient photocatalyst for H2O2 production

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Abstract

The development of high-efficiency economic photocatalyst for H2O2 production is of great significance for renewable energy technologies. Here, we use a successive in situ growth and phosphating method successfully prepared NiCoP/g-C3N4 composite photocatalyst. NiCoP was uniformly dispersed in the form of nanoparticles on the surface of g-C3N4 nanosheet as a cocatalyst. The obtained NiCoP/g-C3N4 composite showed excellent performance in photocatalytic production of H2O2, which was due to NiCoP, has a better electronic conductivity to efficiently transfer charge, improves charge separation efficiency and enhances visible light absorption. This study can provide an effective theoretical basis for the design of bimetallic phosphide modified photocatalysts for photocatalytic production of H2O2.

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Acknowledgements

This work was financially supported by the National Natural Science Foundation of China (21777044, 5171101651, 21677048 and 21811540394), the National Key Research and Development Program (2016YFA0204200), the National Water Pollution Control and Treatment Science and Technology Major Project (2017ZX07207002) and the Fundamental Research Funds for the Central Universities (222201714061, 222201915012, 222201814053, 222201917009 and 222201818014).

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Authors and Affiliations

  1. Key Laboratory for Advanced Materials and Joint International Research Laboratory of Precision Chemistry and Molecular Engineering, Feringa Nobel Prize Scientist Joint Research Center, School of Chemistry and Molecular Engineering, East China University of Science and Technology, 130 Meilong Road, Shanghai, 200237, People’s Republic of China

    Yulan Peng, Lingzhi Wang & Jinlong Zhang

  2. IRCELYON, CNRS-UMR 5256, Université Lyon 1, 2 Avenue A. Einstein, 69626, Villeurbanne Cedex, France

    Yulan Peng & Stéphane Daniele

  3. State Environmental Protection Key Laboratory of Environmental Risk Assessment and Control on Chemical Process, School of Resources and Environmental Engineering, East China University of Science and Technology, 130 Meilong Road, Shanghai, 200237, People’s Republic of China

    Liang Zhou, Juying Lei & Yongdi Liu

  4. Shanghai Institute of Pollution Control and Ecological Security, Shanghai, 200092, People’s Republic of China

    Juying Lei & Yongdi Liu

  5. National Engineering Laboratory for Industrial Wastewater Treatment, East China University of Science and Technology, Shanghai, 200237, China

    Juying Lei & Yongdi Liu

Authors
  1. Yulan Peng
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  2. Liang Zhou
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  3. Lingzhi Wang
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  4. Juying Lei
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  5. Yongdi Liu
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  6. Stéphane Daniele
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  7. Jinlong Zhang
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Correspondence to Juying Lei or Jinlong Zhang.

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Peng, Y., Zhou, L., Wang, L. et al. Preparation of NiCoP-decorated g-C3N4 as an efficient photocatalyst for H2O2 production. Res Chem Intermed 45, 5907–5917 (2019). https://doi.org/10.1007/s11164-019-04009-6

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