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Recent advances in transition metal chalcogenides for lithium-ion capacitors

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Abstract

Transition metal chalcogenides (TMCs) and TMCs-based nanocomposites have attracted extensive attention due to their versatile material species, low cost, and rich physical and chemical characteristics. As anode materials of lithium-ion capacitors (LICs), TMCs have exhibited high theoretical capacities and pseudocapacitance storage mechanism. However, there are many intrinsic challenges, such as low electrical conductivity, repeatedly high-volume changes and sluggish ionic diffusion kinetics. Hence, many traditional and unconventional techniques have been reported to solve these critical problems, and many innovative strategies are also used to prepare high quality anode materials for LICs. In this mini review, a detailed family member list and comparison of TMCs in the field of lithium-ion capacitors have been summarized firstly. Then, many rectification stratagems and recent researches of TMCs have been exhibited and discussed. In the end, as an outcome of these discussions, some further challenges and perspectives are envisioned to promote the application of TMCs materials for lithium-ion capacitors.

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摘要

过渡金属硫族化合物 (TMCs) 和基于TMCs的纳米复合材料由于其材料种类多样, 成本低和丰富的物理和化学特性而受到广泛关注. 作为锂离子电容器的负极材料, TMCs具有较高的理论比容量和赝电容存储机制, 然而仍存在许多固有的挑战, 例如低电导率, 反复的高体积变化和缓慢的离子扩散动力学. 因此, 基于上述问题已经报道了许多传统和非常规解决策略, 并且许多具有创新性的方法被用于制备高性能锂离子电容器负极材料. 这篇综述首先汇总了用于锂离子电容器负极的TMCs材料, 并对各种TMCs的性能进行了比较。然后讨论了TMCs的许多改性策略和最新研究进展. 最后, 作为这些讨论的结果, 对TMCs材料在锂离子电容器中发展的前景进行了分析和展望.

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Acknowledgements

This study was financially supported by the National Natural Science Foundation of China (No. 51907193), the Key Research Program of Frontier Sciences, CAS (No. ZDBS-LY-JSC047), the Youth Innovation Promotion Association CAS (No. 2020145) and Dalian National Laboratory for Clean Energy Cooperation Fund, the CAS (No. DNL201915).

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Authors and Affiliations

  1. Institute of Electrical Engineering, Chinese Academy of Sciences, Beijing, 100190, China

    Lei Wang, Xiong Zhang, Chen Li, Xian-Zhong Sun, Kai Wang & Yan-Wei Ma

  2. School of Engineering Sciences, University of Chinese Academy of Sciences, Beijing, 100049, China

    Lei Wang, Xiong Zhang, Kai Wang & Yan-Wei Ma

  3. Institute of Electrical Engineering and Advanced Electromagnetic Drive Technology, Qilu Zhongke, Jinan, 250013, China

    Xiong Zhang, Chen Li, Xian-Zhong Sun, Kai Wang & Yan-Wei Ma

  4. CAS Key Laboratory of Carbon Materials, Institute of Coal Chemistry, Chinese Academy of Sciences, Taiyuan, 030001, China

    Fang-Yuan Su

  5. State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian, 116023, China

    Fang-Yan Liu

  6. Dalian National Laboratory for Clean Energy, Chinese Academy of Sciences, Dalian, 116023, China

    Xiong Zhang, Fang-Yuan Su & Fang-Yan Liu

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  1. Lei Wang
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Wang, L., Zhang, X., Li, C. et al. Recent advances in transition metal chalcogenides for lithium-ion capacitors. Rare Met. 41, 2971–2984 (2022). https://doi.org/10.1007/s12598-022-02028-8

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