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Favorable anion adsorption/desorption of high rate NiSe2 nanosheets/hollow mesoporous carbon for battery-supercapacitor hybrid devices

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Abstract

High-rate battery-type cathode materials have attracted wide attention for advanced battery-supercapacitor hybrid (BSH) devices. Herein, a core-shell structure of the hollow mesoporous carbon spheres (HMCS) supported NiSe2 nanosheets (HMCS/NiSe2) is constructed through two-step reactions. The HMCS/NiSe2 shows a max specific capacity of 1,153.5 C·g−1 at the current density of 1 A·g−1, and can remain at 774.5 C·g−1 even at 40 A·g−1 (the retention rate as high as 67.1%) and then the HMCS/NiSe2 electrode can keep 80.5% specific capacity after 5,000 cycles at a current density of 10 A·g−1. Moreover, the density functional theory (DFT) calculation confirmed that the introduction HMCS into NiSe2 made adsorption/desorption of OH− easier, which can achieve higher rate capability. The HMCS/NiSe2//6 M KOH//HMCS hybrid device has energy density of 47.15 Wh·kg−1 and power density of 801.8 W·kg−1. This work provides a feasible electrode material with a high rate and its preparation method for high energy density and power density energy storage devices.

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Acknowledgements

This work was supported by the National Natural Science Foundation of China (No. 52002122), the Science and Technology Department of Hubei Province (No. 2019AAA038) and the Wuhan Yellow Crane Talent Program (No. 2017-02). This project has received funding from the European Union’s Horizon 2020 research and innovation programme under grant agreement No. 823717-ESTEEM3.

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  1. Hubei Key Laboratory of Ferro & Piezoelectric Materials and Devices, School of Microelectronics and Faculty of Physics and Electronic Science, Hubei University, Wuhan, 430062, China

    Xiaojuan Zhao, Houzhao Wan, Nengze Wang, Cong Wang, Yi Gan, Xu Chen, Qiuyang Tan, Xiang Liu, Jun Zhang, Hanbin Wang & Hao Wang

  2. College of Optical and Electronic Technology, China Jiliang University, Hangzhou, 310018, China

    Pei Liang

  3. Max Planck Institute for Solid State Research, Heisenbergstr 1, 70569, Stuttgart, Germany

    Xu Chen & Yi Wang

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Favorable anion adsorption/desorption of high rate NiSe2 nanosheets/hollow mesoporous carbon for battery-supercapacitor hybrid devices

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Zhao, X., Wan, H., Liang, P. et al. Favorable anion adsorption/desorption of high rate NiSe2 nanosheets/hollow mesoporous carbon for battery-supercapacitor hybrid devices. Nano Res. 14, 2574–2583 (2021). https://doi.org/10.1007/s12274-020-3257-z

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