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Membrane-based treatment of shale oil and gas wastewater: The current state of knowledge

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Abstract

Shale oil and gas exploitation not only consumes substantial amounts of freshwater but also generates large quantities of hazardous wastewater. Tremendous research efforts have been invested in developing membrane-based technologies for the treatment of shale oil and gas wastewater. Despite their success at the laboratory scale, membrane processes have not been implemented at full scale in the oil and gas fields. In this article, we analyze the growing demands of wastewater treatment in shale oil and gas production, and then critically review the current stage of membrane technologies applied to the treatment of shale oil and gas wastewater. We focus on the unique niche of those technologies due to their advantages and limitations, and use mechanical vapor compression as the benchmark for comparison. We also highlight the importance of pretreatment as a key component of integrated treatment trains, in order to improve the performance of downstream membrane processes and water product quality. We emphasize the lack of sufficient efforts to scale up existing membrane technologies, and suggest that a stronger collaboration between academia and industry is of paramount importance to translate membrane technologies developed in the laboratory to the practical applications by the shale oil and gas industry.

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References

  • Ahmadun F R, Pendashteh A, Abdullah L C, Biak D R A, Madaeni S S, Abidin Z Z (2009). Review of technologies for oil and gas produced water treatment. Journal of Hazardous Materials, 170(2-3): 530–551

    Article  CAS  Google Scholar 

  • Alessi D S, Zolfaghari A, Kletke S, Gehman J, Allen D M, Goss G G (2017). Comparative analysis of hydraulic fracturing wastewater practices in unconventional shale development: Water sourcing, treatment and disposal practices. Canadian Water Resources Journal, 42(2): 105–121

    Article  Google Scholar 

  • Alzahrani S, Mohammad A W, Hilal N, Abdullah P, Jaafar O (2013). Identification of foulants, fouling mechanisms and cleaning efficiency for NF and RO treatment of produced water. Separation and Purification Technology, 118: 324–341

    Article  CAS  Google Scholar 

  • Arkansas Department of Environmental Quality (2016). Fact Sheet and Supplementary Information for General Permit Discharges from Groundwater and SurfaceWater Clean Up Located within the State of Arkansas

    Google Scholar 

  • Aybar H S (2002). Analysis of a mechanical vapor compression desalination system. Desalination, 142(2): 181–186

    Article  CAS  Google Scholar 

  • Bahar R, Hawlader M N A, Woei L S (2004). Performance evaluation of a mechanical vapor compression desalination system. Desalination, 166(1–3): 123–127

    Article  CAS  Google Scholar 

  • Bai B, Carlson K, Prior A, Douglas C (2015). Sources of variability in flowback and produced water volumes from shale oil and gas wells. Journal of Unconventional Oil and Gas Resources, 12: 1–5

    Article  Google Scholar 

  • Bai B, Goodwin S, Carlson K (2013). Modeling of frac flowback and produced water volume from Wattenberg oil and gas field. Journal of Petroleum Science Engineering, 108: 383–392

    Article  CAS  Google Scholar 

  • Bell E A, Poynor T E, Newhart K B, Regnery J, Coday B D, Cath T Y (2017). Produced water treatment using forward osmosis membranes: Evaluation of extended-time performance and fouling. Journal of Membrane Science, 525: 77–88

    Article  CAS  Google Scholar 

  • Bond R, Veerapaneni S (2007). Zero liquid discharge for inland desalination. No. 500–01–040. Denver, CO: AWWA Research Foundation

    Google Scholar 

  • Boo C, Lee J, Elimelech M (2016a). Engineering surface energy and nanostructure of microporous films for expanded membrane distillation applications. Environmental Science & Technology, 50(15): 8112–8119

    Article  CAS  Google Scholar 

  • Boo C, Lee J, Elimelech M (2016b). Omniphobic polyvinylidene fluoride (PVDF) membrane for desalination of shale gas produced water by membrane distillation. Environmental Science & Technology, 50(22): 12275–12282

    Article  CAS  Google Scholar 

  • Brantley S L, Yoxtheimer D, Arjmand S, Grieve P, Vidic R, Pollak J, Llewellyn G T, Abad J, Simon C (2014). Water resource impacts during unconventional shale gas development: The Pennsylvania experience. International Journal of Coal Geology, 126: 140–156

    Article  CAS  Google Scholar 

  • Burbano A, Brankhuber P (2012). Demonstration of membrane zero liquid discharge for drinking water systems: A literature review. Alexandria, VA: Water Environment Research Foundation

    Google Scholar 

  • Butkovskyi A, Bruning H, Kools S A E, Rijnaarts H H M, Van Wezel A P (2017). Organic pollutants in shale gas flowback and produced waters: Identification, potential ecological impact, and implications for treatment strategies. Environmental Science & Technology, 51(9): 4740–4754

    Article  CAS  Google Scholar 

  • Cath T Y, Childress A E, Elimelech M (2006). Forward osmosis: Principles, applications, and recent developments. Journal of Membrane Science, 281(1–2): 70–87

    Article  CAS  Google Scholar 

  • Chang H, Li T, Liu B, Vidic R, Elimelech M, Crittenden J C (2019a). Potential and implemented membrane-based technologies for the treatment and reuse of flowback and produced water from shale gas and oil plays: A review. Desalination, 455: 34–57

    Article  CAS  Google Scholar 

  • Chang H Q, Liu B C, Yang B X, Yang X, Guo C, He Q P, Liang S M, Chen S, Yang P (2019b). An integrated coagulation-ultrafiltration-nanofiltration process for internal reuse of shale gas flowback and produced water. Separation and Purification Technology, 211: 310–321

    Article  CAS  Google Scholar 

  • Chen G, Wang Z W, Nghiem L D, Li X M, Xie M, Zhao B L, Zhang M X, Song J F, He T (2015). Treatment of shale gas drilling flowback fluids (SGDFs) by forward osmosis: Membrane fouling and mitigation. Desalination, 366: 113–120

    Article  CAS  Google Scholar 

  • Chermak J A, Schreiber M E (2014). Mineralogy and trace element geochemistry of gas shales in the United States: Environmental implications. International Journal of Coal Geology, 126: 32–44

    Article  CAS  Google Scholar 

  • Chevron Corporation (2018). Chevron tech challenge: Produced water-Unlocking a valuable natural resource

    Google Scholar 

  • Chew N G P, Zhao S S, Loh C H, Permogorov N, Wang R (2017). Surfactant effects on water recovery from produced water via direct-contact membrane distillation. Journal of Membrane Science, 528: 126–134

    Article  CAS  Google Scholar 

  • Cho Y H, Kim H W, Nam S Y, Park H B (2011). Fouling-tolerant polysulfone-poly(ethylene oxide) random copolymer ultrafiltration membranes. Journal of Membrane Science, 379(1–2): 296–306

    Article  CAS  Google Scholar 

  • Coday B D, Almaraz N, Cath T Y (2015). Forward osmosis desalination of oil and gas wastewater: Impacts of membrane selection and operating conditions on process performance. Journal of Membrane Science, 488: 40–55

    Article  CAS  Google Scholar 

  • Coday B D, Cath T Y (2014). Forward osmosis: Novel desalination of produced water and fracturing flowback. Journal-American Water Works Association, 106(2): E55–E66

    Article  CAS  Google Scholar 

  • Coday B D, Xu P, Beaudry E G, Herron J, Lampi K, Hancock N T, Cath T Y (2014). The sweet spot of forward osmosis: Treatment of produced water, drilling wastewater, and other complex and difficult liquid streams. Desalination, 333(1): 23–35

    Article  CAS  Google Scholar 

  • Davenport D M, Deshmukh A, Werber J R, Elimelech M (2018). High-pressure reverse osmosis for energy-efficient hypersaline brine desalination: Current status, design considerations, and research needs. Environmental Science & Technology Letters, 5(8): 467–475

    Article  CAS  Google Scholar 

  • Deshmukh A, Boo C, Karanikola V, Lin S H, Straub A P, Tong T Z, Warsinger D M, Elimelech M (2018). Membrane distillation at the water-energy nexus: limits, opportunities, and challenges. Energy & Environmental Science, 11(5): 1177–1196

    Article  CAS  Google Scholar 

  • Du X W, Zhang Z Y, Carlson K H, Lee J, Tong T Z (2018). Membrane fouling and reusability in membrane distillation of shale oil and gas produced water: Effects of membrane surface wettability. Journal of Membrane Science, 567: 199–208

    Article  CAS  Google Scholar 

  • Duong H C, Chivas A R, Nelemans B, Duke M, Gray S, Cath T Y, Nghiem L D (2015). Treatment of RO brine from CSG produced water by spiral-wound air gap membrane distillation: A pilot study. Desalination, 366: 121–129

    Article  CAS  Google Scholar 

  • Eastern Municipal Water District and Carollo Engineers (2008). Evaluation and selection of available processes for a zero-liquid discharge system for the Perris, California ground water basin. Denver, CO: U.S. Department of the Interior, Bureau of Reclamation

    Google Scholar 

  • Elimelech M, Phillip W A (2011). The future of seawater desalination: Energy, technology, and the environment. Science, 333(6043): 712–717

    Article  CAS  Google Scholar 

  • Esmaeilirad N, Carlson K, Omur Ozbek P (2015). Influence of softening sequencing on electrocoagulation treatment of produced water. Journal of Hazardous Materials, 283: 721–729

    Article  CAS  Google Scholar 

  • Ferrer I, Thurman E M (2015). Chemical constituents and analytical approaches for hydraulic fracturing waters. Trends in Environmental Analytical Chemistry, 5: 18–25

    Article  CAS  Google Scholar 

  • Forrestal C, Stoll Z, Xu P, Ren Z J (2015). Microbial capacitive desalination for integrated organic matter and salt removal and energy production from unconventional natural gas produced water. Environmental Science. Water Research & Technology, 1(1): 47–55

    Article  CAS  Google Scholar 

  • Freedman D E, Riley S M, Jones Z L, Rosenblum J S, Sharp J O, Spear J R, Cath T Y (2017). Biologically active filtration for fracturing flowback and produced water treatment. Journal of Water Process Engineering, 18: 29–40

    Article  Google Scholar 

  • Gallegos T J, Varela B A, Haines S S, Engle M A (2015). Hydraulic fracturing water use variability in the United States and potential environmental implications. Water Resources Research, 51(7): 5839–5845

    Article  CAS  Google Scholar 

  • Gregory K B, Vidic R D, Dzombak D A (2011). Water management challenges associated with the production of shale gas by hydraulic fracturing. Elements, 7(3): 181–186

    Article  Google Scholar 

  • Guo C, Chang H Q, Liu B C, He Q P, Xiong B Y, Kumar M, Zydney A L (2018). A combined ultrafiltration-reverse osmosis process for external reuse of Weiyuan shale gas flowback and produced water. Environmental Science. Water Research & Technology, 4(7): 942–955

    Article  CAS  Google Scholar 

  • Hanson A J, Luek J L, Tummings S S, McLaughlin M C, Blotevogel J, Mouser P J (2019). High total dissolved solids in shale gas wastewater inhibit biodegradation of alkyl and nonylphenol ethoxylate surfactants. Science of the Total Environment, 668: 1094–1103

    Article  CAS  Google Scholar 

  • Hayes T D, Halldorson B, Horner P, Ewing J, Werline J R, Severin B F (2014). Mechanical vapor recompression for the treatment of shale-gas flowback water. Oil and Gas Facilities, 3(4): 54–62

    Article  Google Scholar 

  • He C, Wang X H, Liu W S, Barbot E, Vidic R D (2014). Microfiltration in recycling of Marcellus Shale flowback water: Solids removal and potential fouling of polymeric microfiltration membranes. Journal of Membrane Science, 462: 88–95

    Article  CAS  Google Scholar 

  • He F, Sirkar K K, Gilron J (2009). Effects of antiscalants to mitigate membrane scaling by direct contact membrane distillation. Journal of Membrane Science, 345(1–2): 53–58

    Article  CAS  Google Scholar 

  • He Y, Sun C, Zhang Y, Folkerts E J, Martin J W, Goss G G (2018). Developmental toxicity of the organic fraction from hydraulic fracturing flowback and produced waters to early life stages of zebrafish (Danio rerio). Environmental Science & Technology, 52 (6): 3820–3830

    Article  CAS  Google Scholar 

  • Huang Y X, Wang Z, Jin J, Lin S (2017). Novel janus membrane for membrane distillation with simultaneous fouling and wetting resistance. Environmental Science & Technology, 51(22): 13304–13310

    Article  CAS  Google Scholar 

  • Jain P, Sharma M, Dureja P, Sarma P M, Lal B (2017). Bioelectrochemical approaches for removal of sulfate, hydrocarbon and salinity from produced water. Chemosphere, 166: 96–108

    Article  CAS  Google Scholar 

  • Jiang Q Y, Rentschler J, Perrone R, Liu K L (2013). Application of ceramic membrane and ion-exchange for the treatment of the flowback water from Marcellus shale gas production. Journal of Membrane Science, 431: 55–61

    Article  CAS  Google Scholar 

  • Kim J, Kim J, Hong S (2018). Recovery of water and minerals from shale gas produced water by membrane distillation crystallization. Water Research, 129: 447–459

    Article  CAS  Google Scholar 

  • Kim J, Kwon H, Lee S, Lee S, Hong S (2017). Membrane distillation (MD) integrated with crystallization (MDC) for shale gas produced water (SGPW) treatment. Desalination, 403: 172–178

    Article  CAS  Google Scholar 

  • Kim S Y, Omur-Ozbek P, Dhanasekar A, Prior A, Carlson K (2016). Temporal analysis of flowback and produced water composition from shale oil and gas operations: Impact of frac fluid characteristics. Journal of Petroleum Science Engineering, 147: 202–210

    Article  CAS  Google Scholar 

  • Kondash A, Vengosh A (2015). Water footprint of hydraulic fracturing. Environmental Science & Technology Letters, 2(10): 276–280

    Article  CAS  Google Scholar 

  • Kondash A J, Albright E, Vengosh A (2017). Quantity of flowback and produced waters from unconventional oil and gas exploration. Science of the Total Environment, 574: 314–321

    Article  CAS  Google Scholar 

  • Kondash A J, Lauer N E, Vengosh A (2018). The intensification of the water footprint of hydraulic fracturing. Sci Adv, 4(8): eaar5982

    Article  CAS  Google Scholar 

  • Kong F X, Chen J F, Wang H M, Liu X N, Wang X M, Wen X, Chen C M, Xie Y F F (2017). Application of coagulation-UF hybrid process for shale gas fracturing flowback water recycling: Performance and fouling analysis. Journal of Membrane Science, 524: 460–469

    Article  CAS  Google Scholar 

  • Kong F X, Sun G D, Chen J F, Han J D, Guo C M, Zhang T, Lin X F, Xie Y F F (2018). Desalination and fouling of NF/low pressure RO membrane for shale gas fracturing flowback water treatment. Separation and Purification Technology, 195: 216–223

    Article  CAS  Google Scholar 

  • Koren A, Nadav N (1994). Mechanical vapor compression to treat oil-field produced water. Desalination, 98(1–3): 41–48

    Article  CAS  Google Scholar 

  • Krupnick A, Wang Z M, Wang Y S (2014). Environmental risks of shale gas development in China. Energy Policy, 75: 117–125

    Article  Google Scholar 

  • Lawson K W, Lloyd D R (1997). Membrane distillation. Journal of Membrane Science, 124(1): 1–25

    Article  CAS  Google Scholar 

  • Lester Y, Ferrer I, Thurman E M, Sitterley K A, Korak J A, Aiken G, Linden K G (2015). Characterization of hydraulic fracturing flowback water in Colorado: Implications for water treatment. Science of the Total Environment, 512-513: 637–644

    Article  CAS  Google Scholar 

  • Lin S H, Nejati S, Boo C, Hu Y X, Osuji C O, Elimelech M (2014). Omniphobic membrane for robust membrane distillation. Environmental Science & Technology Letters, 1(11): 443–447

    Article  CAS  Google Scholar 

  • Lobo F L, Wang H, Huggins T, Rosenblum J, Linden K G, Ren Z J (2016). Low-energy hydraulic fracturing wastewater treatment via AC powered electrocoagulation with biochar. Journal of Hazardous Materials, 309: 180–184

    Article  CAS  Google Scholar 

  • Lokare O R, Tavakkoli S, Rodriguez G, Khanna V, Vidic R D (2017a). Integrating membrane distillation with waste heat from natural gas compressor stations for produced water treatment in Pennsylvania. Desalination, 413: 144–153

    Article  CAS  Google Scholar 

  • Lokare O R, Tavakkoli S, Wadekar S, Khanna V, Vidic R D (2017b). Fouling in direct contact membrane distillation of produced water from unconventional gas extraction. Journal of Membrane Science, 524: 493–501

    Article  CAS  Google Scholar 

  • Lutz B D, Lewis A N, Doyle M W (2013). Generation, transport, and disposal of wastewater associated with Marcellus Shale gas development. Water Resources Research, 49(2): 647–656

    Article  CAS  Google Scholar 

  • McCutcheon J R, Mcginnis R L, Elimelech M (2005). A novel ammonia-carbon dioxide forward (direct) osmosis desalination process. Desalination, 174(1): 1–11

    Article  CAS  Google Scholar 

  • McGinnis R L, Hancock N T, Nowosielski-Slepowron M S, Mcgurgan G D (2013). Pilot demonstration of the NH3/CO2 forward osmosis desalination process on high salinity brines. Desalination, 312: 67–74

    Article  CAS  Google Scholar 

  • Miller D J, Huang X F, Li H, Kasemset S, Lee A, Agnihotri D, Hayes T, Paul D R, Freeman B D (2013). Fouling-resistant membranes for the treatment of flowback water from hydraulic shale fracturing: A pilot study. Journal of Membrane Science, 437: 265–275

    Article  CAS  Google Scholar 

  • Mondal S, Wickramasinghe S R (2008). Produced water treatment by nanofiltration and reverse osmosis membranes. Journal of Membrane Science, 322(1): 162–170

    Article  CAS  Google Scholar 

  • Monge M, Gil-Alana L A, De Gracia F P (2017). US shale oil production and WTI prices behaviour. Energy, 141: 12–19

  • Notte C, Allen D M, Gehman J, Alessi D S, Goss G G (2017). Comparative analysis of hydraulic fracturing wastewater practices in unconventional shale developments: Regulatory regimes. Canadian Water Resources Journal, 42(2): 122–137

    Article  Google Scholar 

  • Oasys Water Inc (2014). Oasys applies FO to treat wastewater from China’s growing power market. Membrane Technology, 2014(11): 2–3

    Article  Google Scholar 

  • Oetjen K, Chan K E, Gulmark K, Christensen J H, Blotevogel J, Borch T, Spear J R, Cath T Y, Higgins C P (2018). Temporal characterization and statistical analysis of flowback and produced waters and their potential for reuse. Science of the Total Environment, 619-620: 654–664

    Article  CAS  Google Scholar 

  • Riley S M, Ahoor D C, Cath T Y (2018a). Enhanced biofiltration of O&G produced water comparing granular activated carbon and nutrients. Science of the Total Environment, 640-641: 419–428

    Article  CAS  Google Scholar 

  • Riley S M, Ahoor D C, Regnery J, Cath T Y (2018b). Tracking oil and gas wastewater-derived organic matter in a hybrid biofilter membrane treatment system: A multi-analytical approach. Science of the Total Environment, 613-614: 208–217

    Article  CAS  Google Scholar 

  • Riley S M, Oliveira J M S, Regnery J, Cath T Y (2016). Hybrid membrane bio-systems for sustainable treatment of oil and gas produced water and fracturing flowback water. Separation and Purification Technology, 171: 297–311

    Article  CAS  Google Scholar 

  • Rosenblum J, Thurman E M, Ferrer I, Aiken G, Linden K G (2017). Organic chemical characterization and mass balance of a hydraulically fractured well: From fracturing fluid to produced water over 405 days. Environmental Science & Technology, 51(23): 14006–14015

    Article  CAS  Google Scholar 

  • Sardari K, Fyfe P, Lincicome D, Wickramasinghe S R (2018a). Aluminum electrocoagulation followed by forward osmosis for treating hydraulic fracturing produced waters. Desalination, 428: 172–181

    Article  CAS  Google Scholar 

  • Sardari K, Fyfe P, Lincicome D, Wickramasinghe S R (2018b). Combined electrocoagulation and membrane distillation for treating high salinity produced waters. Journal of Membrane Science, 564: 82–96

    Article  CAS  Google Scholar 

  • Schantz A B, Xiong B Y, Dees E, Moore D R, Yang X J, Kumar M (2018). Emerging investigators series: Prospects and challenges for high-pressure reverse osmosis in minimizing concentrated waste streams. Environmental Science. Water Research & Technology, 4 (7): 894–908

    Article  CAS  Google Scholar 

  • Shaffer D L, Arias Chavez L H, Ben-Sasson M, Romero-Vargas Castrillón S, Yip N Y, Elimelech M (2013). Desalination and reuse of high-salinity shale gas produced water: drivers, technologies, and future directions. Environmental Science & Technology, 47(17): 9569–9583

    Article  CAS  Google Scholar 

  • Shaffer D L, Werber J R, Jaramillo H, Lin S H, Elimelech M (2015). Forward osmosis: Where are we now? Desalination, 356: 271–284

    Article  CAS  Google Scholar 

  • Shih J S, Saiers J E, Anisfeld S C, Chu Z, Muehlenbachs L A, Olmstead S M M (2015). Characterization and analysis of liquid waste from Marcellus Shale gas development. Environmental Science & Technology, 49(16): 9557–9565

    Article  CAS  Google Scholar 

  • Singh D, Sirkar K K (2012). Desalination of brine and produced water by direct contact membrane distillation at high temperatures and pressures. Journal of Membrane Science, 389: 380–388

    Article  CAS  Google Scholar 

  • Stephenson M H (2016). Shale gas in North America and Europe. Energy Science & Engineering, 4(1): 4–13

    Article  Google Scholar 

  • Stoll Z A, Forrestal C, Ren Z J, Xu P (2015). Shale gas produced water treatment using innovative microbial capacitive desalination cell. Journal of Hazardous Materials, 283: 847–855

    Article  CAS  Google Scholar 

  • Sun Y, Wang D, Tsang D C W, Wang L, Ok Y S, Feng Y (2019). A critical review of risks, characteristics, and treatment strategies for potentially toxic elements in wastewater from shale gas extraction. Environment International, 125: 452–469

    Article  CAS  Google Scholar 

  • Tavakkoli S, Lokare O R, Vidic R D, Khanna V (2017). A techno-economic assessment of membrane distillation for treatment of Marcellus shale produced water. Desalination, 416: 24–34

    Article  CAS  Google Scholar 

  • Thiel G P, Tow E W, Banchik L D, Chung H W, Lienhard J H (2015). Energy consumption in desalinating produced water from shale oil and gas extraction. Desalination, 366: 94–112

    Article  CAS  Google Scholar 

  • Tong T, Elimelech M (2016). The global rise of zero liquid discharge for wastewater management: Drivers, technologies, and future directions. Environmental Science & Technology, 50(13): 6846–6855

    Article  CAS  Google Scholar 

  • U.S. Energy Information Administration (2018a). How much shale (tight) oil is produced in the United States? Available online at: https://www.eia.gov/tools/faqs/faq.php?id=847&t=6. (accessed February 26, 2019)

    Google Scholar 

  • U.S. Energy Information Administration (2018b). How much shale gas is produced in the United States? Available online at: https:www.eia.gov/tools/faqs/faq.php?id=907&t=8. (accessed February 26, 2019).

    Google Scholar 

  • U.S. EPA (1995). Technically-based Local Limits Development Strategy

    Google Scholar 

  • U.S. EPA (2005). 2005 Remediation General Permit Fact Sheet Excerpts

    Google Scholar 

  • Van de Graaf T, Haesebrouck T, Debaere P (2018). Fractured politics? The comparative regulation of shale gas in Europe. Journal of European Public Policy, 25(9): 1276–1293

    Article  Google Scholar 

  • Vengosh A, Jackson R B, Warner N, Darrah T H, Kondash A (2014). A critical review of the risks to water resources from unconventional shale gas development and hydraulic fracturing in the United States. Environmental Science & Technology, 48(15): 8334–8348

    Article  CAS  Google Scholar 

  • Vidic R D, Brantley S L, Vandenbossche J M, Yoxtheimer D, Abad J D (2013). Impact of shale gas development on regional water quality. Science, 340(6134): 1235009

    Article  CAS  Google Scholar 

  • Wang Z, Elimelech M, Lin S (2016). Environmental applications of interfacial materials with special wettability. Environmental Science & Technology, 50(5): 2132–2150

    Article  CAS  Google Scholar 

  • Winglee J M, Bossa N, Rosen D, Vardner J T, Wiesner M R (2017). Modeling the concentration of volatile and semivolatile contaminants in direct contact membrane distillation (DCMD) product water. Environmental Science & Technology, 51(22): 13113–13121

    Article  CAS  Google Scholar 

  • Wu Q, Chen G E, Sun W G, Xu Z L, Kong Y F, Zheng X P, Xu S J (2017). Bio-inspired GO-Ag/PVDF/F127 membrane with improved anti-fouling for natural organic matter (NOM) resistance. Chemical Engineering Journal, 313: 450–460

    Article  CAS  Google Scholar 

  • Xiong B, Zydney A L, Kumar M (2016). Fouling of microfiltration membranes by flowback and produced waters from the Marcellus shale gas play. Water Research, 99: 162–170

    Article  CAS  Google Scholar 

  • Xiong B Y, Roman-White S, Piechowicz B, Miller Z, Farina B, Tasker T, Burgos W, Zydney A L, Kumar M (2018). Polyacrylamide in hydraulic fracturing fluid causes severe membrane fouling during flowback water treatment. Journal of Membrane Science, 560: 125–131

    Article  CAS  Google Scholar 

  • Yang H, Huang X J, Yang Q Y, Tu J J, Li S F, Yang D M, Xia H, Flower R J, Thompson J R (2015). Water requirements for shale gas fracking in Fuling, Chongqing, Southwest China. Energy Procedia, 76: 106–112

    Article  Google Scholar 

  • Yao M W, Woo Y C, Tijing L D, Choi J S, Shon H K (2018). Effects of volatile organic compounds on water recovery from produced water via vacuum membrane distillation. Desalination, 440: 146–155

    Article  CAS  Google Scholar 

  • Yu M, Weinthal E, Patiño-Echeverri D, Deshusses M A, Zou C, Ni Y, Vengosh A (2016). Water availability for shale gas development in Sichuan Basin, China. Environmental Science & Technology, 50(6): 2837–2845

    Article  CAS  Google Scholar 

  • Zhai J, Huang Z, Rahaman M H, Li Y, Mei L, Ma H, Hu X, Xiao H, Luo Z, Wang K (2017). Comparison of coagulation pretreatment of produced water from natural gas well by polyaluminium chloride and polyferric sulphate coagulants. Environmental Technology, 38(10): 1200–1210

    Article  CAS  Google Scholar 

  • Zhang R, Liu Y, He M, Su Y, Zhao X, Elimelech M, Jiang Z (2016). Antifouling membranes for sustainable water purification: strategies and mechanisms. Chemical Society Reviews, 45(21): 5888–5924

    Article  CAS  Google Scholar 

  • Zhang Z Y, Du X W, Carlson K H, Robbins C A, Tong T Z (2019). Effective treatment of shale oil and gas produced water by membrane distillation coupled with precipitative softening and walnut shell filtration. Desalination, 454: 82–90

    Article  CAS  Google Scholar 

  • Zhou X S, Gingerich D B, Mauter M S (2015). Water treatment capacity of forward-osmosis systems utilizing power-plant waste heat. Industrial & Engineering Chemistry Research, 54(24): 6378–6389

    Article  CAS  Google Scholar 

  • Zou C, Ni Y, Li J, Kondash A, Coyte R, Lauer N, Cui H, Liao F, Vengosh A (2018). The water footprint of hydraulic fracturing in Sichuan Basin, China. Science of the Total Environment, 630: 349–356

    Article  CAS  Google Scholar 

  • Zou Y Q, Yang C B, Wu D S, Yan C, Zeng M S, Lan Y Y, Dai Z X (2016). Probabilistic assessment of shale gas production and water demand at Xiuwu Basin in China. Applied Energy, 180: 185–195

    Article  CAS  Google Scholar 

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Acknowledgements

This work was supported by the start-up funds that T. T. received from the Department of Civil and Environmental Engineering, College of Engineering, at Colorado State University, as well as the Advanced Industries Accelerator Grant that T.T. and K.H.C. received from Colorado Office of Economic Development and International Trade and CSU Ventures.

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Correspondence to Tiezheng Tong.

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Highlights

• Shale oil and gas production generates wastewater with complex composition.

• Membrane technologies emerged for the treatment of shale oil and gas wastewater.

• Membrane technologies should tolerate high TDS and consume low primary energy.

• Pretreatment is a key component of integrated wastewater treatment systems.

• Full-scale implementation of membrane technologies is highly desirable.

Author Biography

Dr. Tiezheng Tong is currently an assistant professor in the Department of Civil and Environmental Engineering at Colorado State University (CSU). Before joining CSU, he was a postdoctoral research associate at Yale University. He received his B.S. (2004) and M.S. (2010) degrees in Environmental Engineering from Beijing Normal University and Tsinghua University, and a second M.S. degree (2011) and a Ph.D. degree (2015) in Civil and Environmental Engineering from Northwestern University, Evanston. Dr. Tong’s research group utilizes interdisciplinary approaches to promote environmental sustainability at the water-energy-health nexus. His current research areas focus on developing novel membrane materials and processes for wastewater treatment and water purification, as well as understanding and mitigating mineral scaling in membrane desalination processes. He has published more than 30 peer-reviewed articles and given more than 20 conference presentations internationally. He is the recipient of several professional awards including the Environmental Chemistry Graduate Student Award of American Chemistry Society, the Illinois Section of the ASCE Environmental & Water Resources Institute (EWRI) Student Scholarship Award, and the Student Award from Sustainable Nanotechnology Organization. He also serves as an independent reviewer for more than 20 journals.

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Tong, T., Carlson, K.H., Robbins, C.A. et al. Membrane-based treatment of shale oil and gas wastewater: The current state of knowledge. Front. Environ. Sci. Eng. 13, 63 (2019). https://doi.org/10.1007/s11783-019-1147-y

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  • DOI: https://doi.org/10.1007/s11783-019-1147-y

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