Abstract
Remarkable progress in high-performance polymer solar cells demonstrates their great potential for practical applications in the near future. Indeed, the power conversion efficiencies over 10% have been reported by many research groups, which are achieved through rational optimization of light-harvesting materials, interfaces and device processing technologies. In this mini review, we summarized the recent progress of highly efficient polymer solar cells, with specifically concern on successful strategies of rational molecular design of electron-donating and electron-accepting materials, elaborative interfacial engineering, and reasonable device architectures.
Similar content being viewed by others
References
Li G, Zhu R, Yang Y. Nat Photon, 2012, 6: 153–161
Li Y. Acc Chem Res, 2012, 45: 723–733
Zhou H, Yang L, You W. Macromolecules, 2012, 45: 607–632
Liu C, Wang K, Gong X, Heeger AJ. Chem Soc Rev, 2016, 45: 4848–4849
Duan C, Zhang K, Zhong C, Huang F, Cao Y. Chem Soc Rev, 2013, 42: 9071–9104
Zhang S, Ye L, Hou J. Adv Energy Mater, 2016, 6: 1502529
Li Y. Sci China Chem, 2015, 58: 188–188
Huang F. Sci China Chem, 2015, 58: 190–190
Huang F, Cao Y. Acta Polym Sin, 2016, 4: 399–401
Li Y. Sci China Chem, 2016, 59: 1430–1431
Zuo L, Chang CY, Chueh CC, Zhang S, Li H, Jen AKY, Chen H. Energy Environ Sci, 2015, 8: 1712–1718
You J, Dou L, Yoshimura K, Kato T, Ohya K, Moriarty T, Emery K, Chen CC, Gao J, Li G, Yang Y. Nat Commun, 2013, 4: 1446–1456
Zheng Z, Zhang S, Zhang M, Zhao K, Ye L, Chen Y, Yang B, Hou J. Adv Mater, 2015, 27: 1189–1194
Zhang K, Gao K, Xia R, Wu Z, Sun C, Cao J, Qian L, Li W, Liu S, Huang F, Peng X, Ding L, Yip HL, Cao Y. Adv Mater, 2016, 28: 4817–4823
Zhang Q, Wan X, Liu F, Kan B, Li M, Feng H, Zhang H, Russell TP, Chen Y. Adv Mater, 2016, 28: 7008–7012
Chen CC, Chang WH, Yoshimura K, Ohya K, You J, Gao J, Hong Z, Yang Y. Adv Mater, 2014, 26: 5670–5677
Yusoff ARM, Kim D, Kim HP, Shneider FK, da Silva WJ, Jang J. Energy Environ Sci, 2015, 8: 303–316
Meng X, Zhao G, Xu Q, Tan Z, Zhang Z, Jiang L, Shu C, Wang C, Li Y. Adv Funct Mater, 2014, 24: 158–163
Liao SH, Li YL, Jen TH, Cheng YS, Chen SA. J Am Chem Soc, 2012, 134: 14271–14274
Wang E, Wang L, Lan L, Luo C, Zhuang W, Peng J, Cao Y. Appl Phys Lett, 2008, 92: 033307
Blouin N, Michaud A, Leclerc M. Adv Mater, 2007, 19: 2295–2300
Stuart AC, Tumbleston JR, Zhou H, Li W, Liu S, Ade H, You W. J Am Chem Soc, 2013, 135: 1806–1815
Zhang M, Gu Y, Guo X, Liu F, Zhang S, Huo L, Russell TP, Hou J. Adv Mater, 2013, 25: 4944–4949
Yue J, Liang J, Sun S, Zhong W, Lan L, Ying L, Yang W, Cao Y. Dyes Pigments, 2015, 123: 64–71
Nguyen TL, Choi H, Ko SJ, Uddin MA, Walker B, Yum S, Jeong JE, Yun MH, Shin TJ, Hwang S, Kim JY, Woo HY. Energy Environ Sci, 2014, 7: 3040–3051
Lan L, Chen Z, Hu Q, Ying L, Zhu R, Liu F, Russell TP, Huang F, Cao Y. Adv Sci, 2016, 3: 1600032
Zhang ZG, Li Y. Sci China Chem, 2015, 58: 192–209
Li W, Li Q, Liu S, Duan C, Ying L, Huang F, Cao Y. Sci China Chem, 2015, 58: 257–266
Liu Z, Sun J, Zhu Y, Liu P, Zhang L, Chen J, Huang F, Cao Y. Sci China Chem, 2015, 58: 267–275
Long X, Ding Z, Dou C, Zhang J, Liu J, Wang L. Adv Mater, 2016, 28: 6504–6508
Wang N, Chen W, Shen W, Duan L, Qiu M, Wang J, Yang C, Du Z, Yang R. J Mater Chem A, 2016, 4: 10212–10222
Shi SB, Liao QG, Tang YM, Guo H, Zhou X, WangYL, Yang TB, Liang YY, Cheng X, Liu F, Guo XG. Adv Mater, 2016, doi: 10.1002/adma.20160311
Hou J, Chen HY, Zhang S, Chen RI, Yang Y, Wu Y, Li G. J Am Chem Soc, 2009, 131: 15586–15587
Chen HY, Hou J, Zhang S, Liang Y, Yang G, Yang Y, Yu L, Wu Y, Li G. Nat Photon, 2009, 3: 649–653
Liang Y, Wu Y, Feng D, Tsai ST, Son HJ, Li G, Yu L. J Am Chem Soc, 2009, 131: 56–57
Liang Y, Yu L. Acc Chem Res, 2010, 43: 1227–1236
Liang Y, Xu Z, Xia J, Tsai ST, Wu Y, Li G, Ray C, Yu L. Adv Mater, 2010, 22: E135–E138
Liao SH, Jhuo HJ, Cheng YS, Chen SA. Adv Mater, 2013, 25: 4766–4771
Cui C, Wong WY, Li Y. Energy Environ Sci, 2014, 7: 2276–2284
Ye L, Zhang S, Zhao W, Yao H, Hou J. Chem Mater, 2014, 26: 3603–3605
Huo L, Zhang S, Guo X, Xu F, Li Y, Hou J. Angew Chem Int Ed, 2011, 50: 9697–9702
Liu P, Zhang K, Liu F, Jin Y, Liu S, Russell TP, Yip HL, Huang F, Cao Y. Chem Mater, 2014, 26: 3009–3017
Zhong H, Li CZ, Carpenter J, Ade H, Jen AKY. J Am Chem Soc, 2015, 137: 7616–7619
Zhang S, Ye L, Zhao W, Yang B, Wang Q, Hou J. Sci China Chem, 2015, 58: 248–256
Liu C, Yi C, Wang K, Yang Y, Bhatta RS, Tsige M, Xiao S, Gong X. ACS Appl Mater Interfaces, 2015, 7: 4928–4935
Liao SH, Jhuo HJ, Yeh PN, Cheng YS, Li YL, Lee YH, Sharma S, Chen SA. Sci Rep, 2014, 4: 6813–6819
Zhao F, Wang Z, Zhang J, Zhu X, Zhang Y, Fang J, Deng D, Wei Z, Li Y, Jiang L, Wang C. Adv Energy Mater, 2016, 6
Jagadamma LK, Al-Senani M, El-Labban A, Gereige I, Ngongang Ndjawa GO, Faria JCD, Kim T, Zhao K, Cruciani F, Anjum DH, McLachlan MA, Beaujuge PM, Amassian A. Adv Energy Mater, 2015, 5: 1500204
Nho S, Baek G, Park S, Lee BR, Cha MJ, Lim DC, Seo JH, Oh SH, Song MH, Cho S. Energy Environ Sci, 2016, 9: 240–246
Nian L, Zhang W, Zhu N, Liu L, Xie Z, Wu H, Würthner F, Ma Y. J Am Chem Soc, 2015, 137: 6995–6998
Nam S, Seo J, Woo S, Kim WH, Kim H, Bradley DDC, Kim Y. Nat Commun, 2015, 6: 8929–8938
Ouyang X, Peng R, Ai L, Zhang X, Ge Z. Nat Photon, 2015, 9: 520–524
Liu Y, Page ZA, Russell TP, Emrick T. Angew Chem Int Ed, 2015, 54: 11485–11489
He Z, Xiao B, Liu F, Wu H, Yang Y, Xiao S, Wang C, Russell TP, Cao Y. Nat Photon, 2015, 9: 174–179
Chen JD, Cui C, Li YQ, Zhou L, Ou QD, Li C, Li Y, Tang JX. Adv Mater, 2015, 27: 1035–1041
Baek SW, Hun Kim J, Kang J, Lee H, Young Park J, Lee JY. Adv Energy Mater, 2015, 5: 1501393
Huang J, Li CZ, Chueh CC, Liu SQ, Yu JS, Jen AKY. Adv Energy Mater, 2015, 5: 1500406
Liu Y, Zhao J, Li Z, Mu C, Ma W, Hu H, Jiang K, Lin H, Ade H, Yan H. Nat Commun, 2014, 5: 5293–5301
Chen Z, Cai P, Chen J, Liu X, Zhang L, Lan L, Peng J, Ma Y, Cao Y. Adv Mater, 2014, 26: 2586–2591
Hu H, Jiang K, Yang G, Liu J, Li Z, Lin H, Liu Y, Zhao J, Zhang J, Huang F, Qu Y, Ma W, Yan H. J Am Chem Soc, 2015, 137: 14149–14157
Zhao J, Li Y, Yang G, Jiang K, Lin H, Ade H, Ma W, Yan H. Nat Energy, 2016, 1: 15027–15034
Jin Y, Chen Z, Dong S, Zheng N, Ying L, Jiang XF, Liu F, Huang F, Cao Y. Adv Mater, 2016, 28: 9811–9818
Kawashima K, Fukuhara T, Suda Y, Suzuki Y, Koganezawa T, Yoshida H, Ohkita H, Osaka I, Takimiya K. J Am Chem Soc, 2016, 138: 10265–10275
Zhou C, Zhang G, Zhong C, Jia X, Luo P, Xu R, Gao K, Jiang X, Liu F, Russell TP, Huang F, Cao Y. Adv Energy Mater, 2016, 1601081
Vohra V, Kawashima K, Kakara T, Koganezawa T, Osaka I, Takimiya K, Murata H. Nat Photon, 2015, 9: 403–408
Lin Y, Wang J, Zhang ZG, Bai H, Li Y, Zhu D, Zhan X. Adv Mater, 2015, 27: 1170–1174
Meng D, Sun D, Zhong C, Liu T, Fan B, Huo L, Li Y, Jiang W, Choi H, Kim T, Kim JY, Sun Y, Wang Z, Heeger AJ. J Am Chem Soc, 2016, 138: 375–380
Lin Y, He Q, Zhao F, Huo L, Mai J, Lu X, Su CJ, Li T, Wang J, Zhu J, Sun Y, Wang C, Zhan X. J Am Chem Soc, 2016, 138: 2973–2976
Gao L, Zhang ZG, Xue L, Min J, Zhang J, Wei Z, Li Y. Adv Mater, 2016, 28: 1884–1890
Hwang YJ, Li H, Courtright BAE, Subramaniyan S, Jenekhe SA. Adv Mater, 2016, 28: 124–131
Zhong Y, Trinh MT, Chen R, Purdum GE, Khlyabich PP, Sezen M, Oh S, Zhu H, Fowler B, Zhang B, Wang W, Nam CY, Sfeir MY, Black CT, Steigerwald ML, Loo YL, Ng F, Zhu XY, Nuckolls C. Nat Commun, 2015, 6: 8242
Li S, Liu W, Shi M, Mai J, Lau TK, Wan J, Lu X, Li CZ, Chen H. Energy Environ Sci, 2016, 9: 604–610
Zhao W, Qian D, Zhang S, Li S, Inganäs O, Gao F, Hou J. Adv Mater, 2016, 28: 4734–4739
Li S, Ye L, Zhao W, Zhang S, Mukherjee S, Ade H, Hou J. Adv Mater, 2016, 28: 9423–9429
Qin YP, Uddin MA, Chen Y, Jang B, Zhao K, Zheng Z, Yu RN, Shin TJ, Woo HY, Hou JH. Adv Mater, 2016, doi: 10.1002/adma.20160180
Zhang Q, Kan B, Liu F, Long G, Wan X, Chen X, Zuo Y, Ni W, Zhang H, Li M, Hu Z, Huang F, Cao Y, Liang Z, Zhang M, Russell TP, Chen Y. Nat Photon, 2014, 9: 35–41
Zhou J, Zuo Y, Wan X, Long G, Zhang Q, Ni W, Liu Y, Li Z, He G, Li C, Kan B, Li M, Chen Y. J Am Chem Soc, 2013, 135: 8484–8487
Kan B, Li M, Zhang Q, Liu F, Wan X, Wang Y, Ni W, Long G, Yang X, Feng H, Zuo Y, Zhang M, Huang F, Cao Y, Russell TP, Chen Y. J Am Chem Soc, 2015, 137: 3886–3893
Zhang Y, Deng D, Lu K, Zhang J, Xia B, Zhao Y, Fang J, Wei Z. Adv Mater, 2015, 27: 1071–1076
Wang Z, Zhang Y, Zhang J, Wei Z, Ma W. Adv Energy Mater, 2016, 6: 1502456
Zhang J, Zhang Y, Fang J, Lu K, Wang Z, Ma W, Wei Z. J Am Chem Soc, 2015, 137: 8176–8183
Liu T, Huo L, Sun X, Fan B, Cai Y, Kim T, Kim JY, Choi H, Sun Y. Adv Energy Mater, 2016, 6: 1502109
Nian L, Gao K, Liu F, Kan Y, Jiang X, Liu L, Xie Z, Peng X, Russell TP, Ma Y. Adv Mater, 2016, 28: 8184–8190
Lu H, Zhang JC, Chen JY, Liu Q, Gong X, Feng SY, Xu XJ, Ma W, Bo ZS. Adv Mater, 2016, doi: 10.1002/adma.20160358
Liu T, Guo Y, Yi YP, Huo LJ, Xue XN, Sun XB, Fu HT, Xiong WT, Meng D, Wang ZH, Liu F, Russell TP, Sun YM. Adv Mater, 2016, doi: 10.1002/adma.20160257
Cheng P, Yan C, Wu Y, Wang J, Qin M, An Q, Cao J, Huo L, Zhang F, Ding L, Sun Y, Ma W, Zhan X. Adv Mater, 2016, 28: 8021–8028
Xu X, Li Z, Wang Z, Li K, Feng K, Peng Q. Nano Energy, 2016, 25: 170–183
Liu S, You P, Li J, Li J, Lee CS, Ong BS, Surya C, Yan F. Energy Environ Sci, 2015, 8: 1463–1470
Goh T, Huang JS, Yager KG, Sfeir MY, Nam CY, Tong X, Guard LM, Melvin PR, Antonio F, Bartolome BG, Lee ML, Hazari N, Taylor AD. Adv Energy Mater, 2016, 6: 1600660
An Q, Zhang F, Sun Q, Zhang M, Zhang J, Tang W, Yin X, Deng Z. Nano Energy, 2016, 26: 180–191
Zhang M, Zhang F, An Q, Sun Q, Wang W, Zhang J, Tang W. Nano Energy, 2016, 22: 241–254
Liang Z, Zhang Q, Jiang L, Cao G. Energy Environ Sci, 2015, 8: 3442–3476
Lu J, Cai W, Zhang G, Liu S, Ying L, Huang F. Acta Chim Sin, 2015, 73: 1153–1160
Hu Z, Zhang K, Huang F, Cao Y. Chem Commun, 2015, 51: 5572–5585
Wang J, Lin K, Zhang K, Jiang XF, Mahmood K, Ying L, Huang F, Cao Y. Adv Energy Mater, 2016, 6: 1502563
Nian L, Zhang W, Wu S, Qin L, Liu L, Xie Z, Wu H, Ma Y. ACS Appl Mater Interfaces, 2015, 7: 25821–25827
Nian L, Chen Z, Herbst S, Li Q, Yu C, Jiang X, Dong H, Li F, Liu L, Würthner F, Chen J, Xie Z, Ma Y. Adv Mater, 2016, 28: 7521–7526
Yu W, Huang L, Yang D, Fu P, Zhou L, Zhang J, Li C. J Mater Chem A, 2015, 3: 10660–10665
Lin X, Yang Y, Nian L, Su H, Ou J, Yuan Z, Xie F, Hong W, Yu D, Zhang M, Ma Y, Chen X. Nano Energy, 2016, 26: 216–223
Wang Z, Li Z, Xu X, Li Y, Li K, Peng Q. Adv Funct Mater, 2016, 26: 4643–4652
Wu Z, Sun C, Dong S, Jiang XF, Wu S, Wu H, Yip HL, Huang F, Cao Y. J Am Chem Soc, 2016, 138: 2004–2013
Liu J, Li X, Zhang S, Ren X, Cheng J, Zhu L, Zhang D, Huo L, Hou J, Choy WCH. Adv Mater Interfaces, 2015, 2: 1500324
Wan Q. Guo X, Wang ZY, Li WB, Guo B, Ma W, Zhang MJ, Li YF. Adv Funct Mater, 2016, doi: 10.1002/adfm.20160218
Huang J, Carpenter JH, Li CZ, Yu JS, Ade H, Jen AKY. Adv Mater, 2016, 28: 967–974
Duan C, Huang F, Cao Y. Polym Chem, 2015, 6: 8081–8098
Li W, Hendriks KH, Roelofs WSC, Kim Y, Wienk MM, Janssen RAJ. Adv Mater, 2013, 25: 3182–3186
Hu X, Yi C, Wang M, Hsu CH, Liu S, Zhang K, Zhong C, Huang F, Gong X, Cao Y. Adv Energy Mater, 2014, 4: 1400378
Li W, Albrecht S, Yang L, Roland S, Tumbleston JR, McAfee T, Yan L, Kelly MA, Ade H, Neher D, You W. J Am Chem Soc, 2014, 136: 15566–15576
Lucera L, Machui F, Kubis P, Schmidt HD, Adams J, Strohm S, Ahmad T, Forberich K, Egelhaaf HJ, Brabec CJ. Energy Environ Sci, 2016, 9: 89–94
Zhang K, Hu Z, Xu R, Jiang XF, Yip HL, Huang F, Cao Y. Adv Mater, 2015, 27: 3607–3613
Li N, Brabec CJ. Energy Environ Sci, 2015, 8: 2902–2909
Cai W, Liu P, Jin Y, Xue Q, Liu F, Russell TP, Huang F, Yip HL, Cao Y. Adv Sci, 2015, 2: 1500095
Zhang H, Yao H, Zhao W, Ye L, Hou J. Adv Energy Mater, 2016, 6: 1502177
Deng Y, Li W, Liu L, Tian H, Xie Z, Geng Y, Wang F. Energy Environ Sci, 2015, 8: 585–591
Chueh CC, Yao K, Yip HL, Chang CY, Xu YX, Chen KS, Li CZ, Liu P, Huang F, Chen Y, Chen WC, Jen AKY. Energy Environ Sci, 2013, 6: 3241–3248
Jung JW, Jo JW, Chueh CC, Liu F, Jo WH, Russell TP, Jen AKY. Adv Mater, 2015, 27: 3310–3317
Acknowledgments
This work was supported by the Ministry of Science and Technology (2014CB643501), the National Natural Science Foundation of China (21520102006, 21634004, 51673069, 21490573), and the Guangdong Natural Science Foundation (S2012030006232).
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Hu, Z., Ying, L., Huang, F. et al. Towards a bright future: polymer solar cells with power conversion efficiencies over 10%. Sci. China Chem. 60, 571–582 (2017). https://doi.org/10.1007/s11426-016-0424-9
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s11426-016-0424-9