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Excitation functions of neutrons induced reactions on terbium from threshold to 20 MeV

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Abstract

Cross-sections for (n,2n), (n,p), and (n,α) reactions have been measured on terbium isotopes at the neutron energies from 13.5 to 14.8 MeV using the activation technique in combination with high-resolution gamma-ray spectroscopy. Data are reported for the following reactions: 159Tb(n,2n)158m+gTb, 159Tb(n,p)159Gd, and 159Tb(n,α)156Eu. The cross sections were also estimated with the TALYS-1.4 nuclear model code, at neutron energies varying from the reaction threshold to 20 MeV. The results were discussed and compared with experimental data found in the literature, and with the comprehensive evaluation data in ENDF/B-VII.1 and JENDL-4.0 libraries.

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References

  1. CINDA-A (2000) The index to literature and computer files on microscopic neutron data. International Atomic Energy Agency, Vienna

    Google Scholar 

  2. Mclane V, Dunford CL, Rose PF (1988) Neutron cross sections, vol 2. Academic, New York

    Google Scholar 

  3. Prestwood RJ, Curtis DB, Rokop DJ, Nethaway DR, Smith NL (1984) Determination of the cross section for 159Tb(n,2n)158Tb and the half-life of 158Tb. Phys Rev C 30:823

    Article  CAS  Google Scholar 

  4. Qaim SM (1974) Total (n,2n) cross sections and isomeric cross-section ratios at 14.7 MeV in the region of rare earths. Nucl Phys A224:319

    Article  Google Scholar 

  5. Ikeda Y, Smith DL, Kumar A, Konno C (1991) Measurements of long-lived activation cross sections by 14 MeV neutrons at FNS. JAERI-M Rep 91(032):272

    Google Scholar 

  6. Meadows JW, Smith DL, Greenwood LR, Haight RC, Ikeda Y, Konno C (1996) Measurement of fast-neutron activation cross sections for copper, europium, hafnium, iron, nickel, silver, terbium and titanium at 10.0 and 14.7 MeV and for the Be(d,n) thick-target spectrum. Ann Nucl Energy 23:877

    Article  CAS  Google Scholar 

  7. Ikeda Y, Konno C, Kumar A, Kasugai Y (1996) Summary of activation cross sections measurements at fusion neutron source in JAERI. IAEA Nucl. Data Section report to the I.N.D.C. 342: 19.

  8. Qaim SM, Cserpak F, Csikai J (1992) Cross sections of 151Eu(n,2n)150mEu and 159Tb(n,2n)158Tb reactions near their thresholds. Appl Radat Isot 43:1065

    Article  CAS  Google Scholar 

  9. Yu W, Zhao W, Cheng J, Lu H (1995) Cross sections of 109Ag(n,2n)108mAg, 151Eu(n,2n)150mEu, 159Tb(n,2n)158Tb and 179Hf(n,2n)178m2Hf reactions. Chin J Nucl Phys (Beijing) 17:268

    CAS  Google Scholar 

  10. Dzysiuk N, Kadenko I, Koning AJ, Yermolenko R (2010) Cross sections for fast-neutron interaction with Lu, Tb, and Ta isotopes. Phys Rev C 81:014610

    Article  CAS  Google Scholar 

  11. Wang Y, Yuan J, Yang J, Kong X, Ren Z, Wang H (1992) Measurement of some (n,2n) reaction cross sections for producing long half-life residues. High Energy Phys Nucl. Phys 16:731 (in Chinese)

    CAS  Google Scholar 

  12. Qaim SM, Cserpak F, Csikai J (1996) Excitation functions of 109Ag(n,2n)108mAg, 151Eu(n,2n)150mEu and 159Tb(n,2n)158Tb reactions from threshold to 15 MeV. Appl Radiat Isot 47:569

    Google Scholar 

  13. Bramlitt ET, Fink RW (1963) Rare nuclear reactions induced by 14.7 MeV neutrons. Phys. Rev 131:2649

    Article  CAS  Google Scholar 

  14. Bari A (1982) 14.8 MeV neutron activation cross-sections for (n,p) and (n,α) reactions of some rare earth nuclides. J Radioanal Chem 75:189

    Article  CAS  Google Scholar 

  15. Havlik E (1971) Measurement of (n,p), (n,α) and (n,2n) cross-sections of heavy nuclei. Acta Phys Austriaca 34:209 (in German)

    CAS  Google Scholar 

  16. Qaim SM (1976) Measurement of (n,p) reaction cross sections at 14.7 MeV using high-pressure liquid chromatography in the region of rare earths. Radiochem Radioanal Lett 25:335

    CAS  Google Scholar 

  17. Konno C, Ikeda Y, Oishi K, Kawade K, Yamamoto H, Maekawa H (1993) Activation cross section measurements at neutron energy from 13.3 to 14.9 MeV, JAERI Reports, 1329

  18. Prasad PR, Rao JR, Kondaiah E (1969) Cross sections for (n,2n), (n,α) and (n,p) reactions in rare-earth isotopes at 14.2 MeV. Nucl Phys A125:57

    Article  Google Scholar 

  19. Qaim SM (1984) Activation cross sections of (n,α) reactions at 14.7 MeV in the region of rare earths. Radiochim Acta 35:9

    Google Scholar 

  20. Kulisic P, Cindro N, Strohal P, Lalovic B (1965) Direct processes in (n,α) reactions. Nucl Phys 73:548

    Article  CAS  Google Scholar 

  21. Kong X, Wang Y, Yang J (1998) Cross sections for (n,2n), (n,p) and (n,α) reactions on rare-earth isotopes at 14.7 MeV. Appl Radiat Isot 49:1529

    Article  CAS  Google Scholar 

  22. Wagner M, Vonach H, Pavlik A, Strohmaier B, Tagesen S, Martinez-Rico J (1990) Physik daten-physics data, evaluation of cross sections for 14 important neutron-dosimetry reactions, Fachinformationszentrum Karlsruhe, Gesellschaft für wissenschaftlich-technische Information mbH, in the Federal Republic of Germany. No. 13–15

  23. Luo J, Du L, Zhao J (2013) A method to determine fast neutron energies in large sample. Nucl Instrum Methods B 298:61–65

    Article  CAS  Google Scholar 

  24. Luo J, Li C, Liu Z, Wang X, Liu R, Jiang L (2010) Measurement of neutron-induced activation cross sections of lanthanum at 14.8 MeV. J Radioanal Nucl Chem 283(2):421–426

    Article  CAS  Google Scholar 

  25. Browne E, Firestone RB (1996) Table of isotopes. Wiley, New York

    Google Scholar 

  26. Luo J, Han J, Liu R, Jiang L, Ge S, Liu Z, Sun G (2013) Measurements of activation cross-sections for the 101Ru(n,p)101Tc reaction for neutrons with energies between 13 and 15 MeV. J Radioanal Nucl Chem 296(3):1225–1230

    Article  CAS  Google Scholar 

  27. Luo J, Tuo F, Kong X (2011) Cross-sections for formation of 178m2Hf and 179m2Hf through reactions on natural hafnium at neutron energy 14.8 ± 0.2 MeV. J Radioanal Nucl Chem 288(1):143–148

    Article  CAS  Google Scholar 

  28. Luo J, Han J, Liu R, Jiang L, Liu Z, Sun G, Ge S (2013) Activation measurements of fast neutron radiative capture for 139La. Radiat Phys Chem 86:79–83

    Article  CAS  Google Scholar 

  29. Koning A, Hilaire S, Duijvestijn M “TALYS-1.4 (2012) A nuclear reaction program,” NRG-1755 ZG Petten, The Netherlands, http://www.talys.eu/more-about-talys/talys-general-features/

  30. Koning J, Delaroche JP (2003) Local and global nucleon optical models from 1 keV to 200 MeV. Nucl Phys A 713:231

    Article  Google Scholar 

  31. Watanabe S (1958) High energy scattering of deuterons by complex nuclei. Nucl Phys 8:484

    Article  CAS  Google Scholar 

  32. Hauser W, Feshbach H (1952) The inelastic scattering of neutrons. Phys Rev 87:366

    Article  CAS  Google Scholar 

  33. Kalbach (1986) Two-component exciton model: basic formalism away from shell closures. Phys Rev C 33:818

    Article  CAS  Google Scholar 

  34. Evaluated Nuclear Data File (ENDF), ENDF/B-VII.1 (USA, 2011), http://www-nds.iaea.org/exfor/servlet/ E4sSearch2.

  35. Evaluated Nuclear Data File (ENDF), JENDL-4.0 (Japan, 2012), http://www-nds.iaea.org/exfor/servlet/ E4sSearch2.

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Acknowledgments

We would like to thank the Intense Neutron Generator group at Chinese Academy of Engineering Physics for performing the irradiations. This work is supported by the National Natural Science Foundation of China (Grant No. 11165007), by the Key Project of Chinese Ministry of Education (No. 211184).

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Correspondence to Junhua Luo.

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Luo, J., An, L., Jiang, L. et al. Excitation functions of neutrons induced reactions on terbium from threshold to 20 MeV. J Radioanal Nucl Chem 300, 819–823 (2014). https://doi.org/10.1007/s10967-014-3043-z

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