Abstract
Air quality monitoring could potentially improve exposure estimates for use in epidemiological studies. We investigated air quality by monitoring concentrations of 222Rn near the ground and particulate matter (PM) with an aerodynamic diameter less than or equal to 10 μm (PM10) and 2.5 μm (PM2.5) for Bucharest-Magurele periurban area. Atmospheric radon concentrations have been continuously monitored near the ground at 1 m height as well as at 10 m height. This paper presents time-series of radon concentrations monitoring in air near the ground measured during 1 January 2011–1 January 2012 by use of solid state nuclear track detectors SSNTD CR-39, exposed for 10 days periods. The daily average atmospheric radon concentration near the ground registered at 1 m height was found to be in range of 40.25 ± 7.53 Bq/m3, which was comparable with the daily average radon concentration of 44.92 ± 9.94 Bq/m3 recorded for period 1 August 2011–20 December 2011 at 10 m height by AlphaGUARD Radon monitor. Also, was done a comparative analysis of spatio-temporal variations in time series of outdoor radon concentration and PM in two size fractions (PM10 and PM2.5) in Bucharest Magurele area for 2011 year. The predominant recorded component in PM10 was PM2.5. Observational results show that recorded yearly average PM2.5 and PM10 concentrations were 35.96 μg/m3 and 40.91 μg/m3, respectively. The average ratio of PM2.5/PM10 was 87.9 % at this sampling site. However, in densely populated Bucharest urban and suburban areas the mean daily EC limit values for PM10, PM2.5 and attached 222Rn are frequently exceeded leading to serious public concern during the last years. The ambient air pollution measurements like as PM10 and PM2.5 levels are used as a proxy for personal exposure levels. Have been investigated also meteorological effects on the temporal patterns of atmospheric radon and particle matter.
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References
European Environment Agency (EEA) (2003) Europe’s environment: the third assessment. Environmental Assessment Report 10, Copenhagen, pp 1–343
Araujo J, Nel A (2009) Particulate matter and atherosclerosis: role of particle size, composition and oxidative stress. Part Fibre Toxicol 6:1–24
Marcazzan GM, Vaccaro S, Valli G, Vecchi R (2001) Characterisation of PM10 and PM2.5 particulate matter in the ambient air of Milan (Italy). Atmos Environ 35:4639–4650
Marcazzan GM, Caprioli E, Valli G, Vecchi R (2003) Temporal variation of 212Pb concentration in outdoor air of Milan and a comparison with 214Bi. J Environ Radioact 65:77–90
Dulaiova H, Peterson R, Burnett WC, Lane-Smith D (2005) A multi-detector continuous monitor for assessment of 222Rn in the coastal ocean. J Radioanal Nucl Chem 263:361–365
Smetanova I, Holy K, Muellerova M, Polaskova A (2009) The effect of meteorological parameters on radon concentration in borehole air and water. J Radioanal Nucl Chem 283:101–109
Porstendorfer J, Zock Ch, Reineking A (2000) Aerosol size distribution of radon progeny in outdoor Air. J Environ Radioact 51:37–48
Porstendorfer J, Grundel M (2004) Differences between the activity size distributions of the different natural radionuclide aerosols in outdoor air. Atmos Environ 38:3723–3728
Graustein WC, Turekian KK (1990) Radon fluxes from soils to the atmosphere measured by 210Pb–226Ra disequilibrium in soils. Geophys Res Lett 17:841–844
Hussain N, Church TM, Veron AJ, Larson RE (1998) Radon daughter disequilibria and lead systematics in the western North Atlantic. J Geophys Res 103:16059–16071
Nazaroff WW (1992) Radon transport from soil to air. Rev Geophys 30:137–160
Turekian KK, Nozaki Y, Benninger LK (1977) Geochemistry of atmospheric radon and radon products. Annu Rev Earth Planet Sci 5:227–255
Whittlestone S, Zahorowski W, Schery SD (1998) Radon flux variability with season and location in Tasmania, Australia. J Radioanal Nucl Chem 236:213–217
Alastuey A, Querol X, Rodriguez S, Plana F, Lopez-Soler A, Ruiz C, Mantilla E (2004) Monitoring of atmospheric particulate matter around sources of secondary inorganic aerosol. Atmos Environ 38:4979–4992
Fang GC, Chang CN, Wu YS, Yang DG, Chu CC (1999) Characterization of chemical species in universal sampler (PM2.5 and PM2.5–10) aerosols in suburban area of central Taiwan. Toxicol Environ Chem 71:341–355
Ostro B, Chestnut L (1998) Assessing the health benefits of reducing particulate matter air pollution in the United States. Environ Res 76:94–106
Fang GC, Chang CN, Chu CC, Wu YS, Yang IL, Chen MH (2003) Characterization of particulate, metallic elements of TSP, PM2.5 and PM2.5–10 aerosols at a farm sampling site in Taiwan, Taichung. Sci Total Environ 308:157–166
Chen LY, Kwok WS (2000) Vertical dispersion of suspended particulates in urban area of Hong Kong. Atmos Environ 34:4403–4412
Ohlstrom MO, Lehitinen KEJ, Moisio M, Jokiniemi JK (2000) Fine-particle emissions of energy production in Finland. Atmos Environ 34:3701–3711
Harrison RM, Shi JP, Jones MR (1999) Continuous measurements of aerosol physical properties in the urban atmosphere. Atmos Environ 33:1037–1047
Dockery D, Pope C, Xu X, Sprengler J, Ware J, Fay M et al (1993) An association between air pollution and mortality in six US cities. N Engl J Med 329:1753–1759
Pope CA III, Burnett RT, Thun MJ, Calle EE, Krewski D, Ito K et al (2002) Lung cancer, cardiopulmonary mortality, and long-term exposure to fine particulate air pollution. J Am Med Assoc 8488
Ramanathan V (2007) Warming trends in Asia amplified by brown cloud solar absorption. Nature 448:575–578
Li N, Hao M, Phaden RF, Hinds WC, Nel AE (2003) Particulate air pollutants and asthma a paradigm for the role of oxidative stress in PM-induced adverse health effects. Clin Immunol 109:250–265
Directive 2008/50/EC of the European Parliament and of the Council of 21 May 2008 on ambient air quality and cleaner air for Europe (2008) Off J Eur Union L 152:1–43
Ashikawa N, Syojo N, Imamura H, Fujisaki M, Matsuoka N, Takashima Y (1998) The size distribution of 210Po in the atmosphere around Mt Sakurajima in Kagoshima prefecture, Japan. J Radioanal Nucl Chem 230(1–2):9–104
Zhuo W, Guo Q, Chen B, Cheng G (2008) Estimating the amount and distribution of radon flux density from the soil surface in China. J Environ Radioact 99:1143–1148
Yamamoto H, Abe T, Kuwabara J, Komura K, Ueno K, Takizawa Y (1994) Polonium210 and lead-210 in marine organisms: Intake levels for Japanese. J Radioanal Nucl Chem 178(1):81
UNSCEAR Report 2010, Report of the United Nations Scientific Committee on the Effects of Atomic Radiations 2010 (2011) N.Y., pp 1–51
Espinosa G, Golzarri JI, Ponciano-Rodriguez G, Gaso MI, Mena M, Segovia N, Vazquez-Lopez C, Sajo-Bohus L (2009) Population vulnerability due to the exposure to radon and airborne particulate matter (PM10), in Mexico City. Radiat Meas 44:1028–1031
Kim KH, Mishra VK, Kang CH, Choi KC, Kim YJ, Kim DS (2006) The ionic compositions of fine and coarse particle fractions in the two urban areas of Korea. J Environ Manage 78:170–182
Hueglin C, Gehrig R, Baltensperger U, Gysel M, Monnd C, Vonmonta H (2005) Chemical characterisation of PM2.5, PM10 and coarse particles at urban, near-city and rural sites in Switzerland. Atmos Environ 39:637–651
EU Regular economic report, January 2007 (2007) Washington, DC, World Bank
Dockery D, Pope A (1996) Epidemiology of acute health effects: summary of time-series studies. In: Wilson R, Spengler JD (eds) Particles in air: concentration and health effects. Harvard University Press, Cambridge, pp 123–147
Lippmann M (1998) The 1997 US EPA standards for particulate matter and ozone. In: Hester RE, Harrison RM (eds) Issues in environmental science and technology, vol 10. Royal Society of Chemistry, pp 75–99
Zahorowski W, Chambers SD, Henderson-Sellers A (2004) Ground based radon-222 observations and their application to atmospheric studies. J Environ Radioact 76:3–33
Cuculeanu V, Simion F, Simion E, Geicu A et al (2011) Dynamics, deterministic nature and correlations of outdoor 222Rn and 220Rn progeny concentrations measured at Bacau, Romania. J Environ Radioact 102:703–712
Baciu AC (2005) Radon and thoron progeny concentration variability in relation to meteorological conditions at Bucharest (Romania). J Environ Radioact 83:171–189
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This work was supported by the NUCLEU Program and PN II-PCCA Program of Romanian Ministry of Education, Research, Youth and Sport.
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Zoran, M.A., Dida, M.R., Zoran, A. et al. Outdoor 222Radon concentrations monitoring in relation with particulate matter levels and possible health effects. J Radioanal Nucl Chem 296, 1179–1192 (2013). https://doi.org/10.1007/s10967-012-2259-z
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DOI: https://doi.org/10.1007/s10967-012-2259-z