Abstract
MgTiO3-based microwave dielectric ceramics were prepared successfully by reaction sintering method. The X-ray diffraction patterns of the sintered samples revealed a major phase of MgTiO3-based and CaTiO3 phases, accompanied with Mg2TiO4 or MgTi2O5 determined by the sintering temperature and time. The microwave dielectric properties had a strong dependence of sintering condition due to the different phase compositions and the microstructure characteristics. The ceramics sintered at 1360 °C for 4 h exhibited good microwave dielectric properties: a dielectric constant of 20.3, a high quality factor of 48,723 GHz (at 9GHz), and a temperature coefficient of resonant frequency of −1.8 ppm/oC. The obtained results demonstrated that the reaction-sintering process is a simple and effective method to prepare the MgTiO3-based ceramics for microwave applications.
Similar content being viewed by others
References
E.S. Kim, C.J. Jeon, J. Eur. Ceram. Soc. 30(2), 341–346 (2010)
H.K. Shin, H. Shin, S.Y. Cho, K.S. Hong, P.J. Am, Ceram. Soc. 88(9), 2461–2465 (2005)
W.C. Won, K. Kenichi, O. Hitoshi, Jpn. J. Appl. Phys. 43(9A), 6221–6224 (2004)
B. Tang, H. Li, P. Fan, S.Q. Yu, S.R. Zhang, J. Mater. Sci. Mater. Electron. 25, 2482 (2014)
I.N. Lin, C.B. Chang, K.C. Leou, H.F. Cheng, J. Eur. Ceram. Soc. 30(2), 159 (2010)
M. Bari, E. Taheri-Nassaj, H. Taghipour-Armaki, J. Electron. Mater. 44(10), 3670–3676 (2015)
Y.G. Zhao, P. Zhang, J. Alloys Compd. 672, 630–635 (2016)
X.M. Xue, H.T. Yu, G.L. Xu, J. Mater. Sci.: Mater. Electron. 24(4), 1287 (2013)
Y.H. Park, J.M. Ryu, M.Y. Shin, K.H. Ko, D.W. Kim, K.S. Hong, J. Am. Ceram. Soc. 84(11), 2542 (2001)
S.Q. Yu, B. Tang, S.R. Zhang, X.H. Zhou, Mater. Lett. 80, 124–126 (2012)
C.F. Shih, W.M. Li, K.S. Tung, J. Am. Ceram. Soc. 93(9), 2448 (2010)
R.D. Shannon, Acta Cryst A32, 751 (1976)
A. Templeton, X. Wang, S.J. Penn, S.J. Webb, L.F. Cohen, N.M. Alford, J. Am. Ceram. Soc. 83(1), 95 (2008)
H. Shin, H.K. Shin, H.S. Jung, S.Y. Cho, K.S. Hong, Mater. Res. Bull. 40, 2012 (2005)
H.K. Shin, H. Shin, S.Y. Cho, K.S. Hong, J. Am. Ceram. Soc. 88, 3461 (2005)
A. Belous, Q. Ovchar, D. Durilin, J. Am. Ceram. Soc. 89(11), 3441–3445 (2006)
R. Freer, F. Azough, J. Eur. Ceram. Soc. 28(7), 1433–1441 (2008)
Acknowledgements
We appreciate the assistance from Suzhou Boom High Purtiy Materials Technology Co., Ltd. This research did not receive any specific grant from funding agencies in the public, commercial, or not-for-profit sectors.
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
He, L., Yu, H., Zeng, M. et al. Phase compositions and microwave dielectric properties of MgTiO3-based ceramics obtained by reaction-sintering method. J Electroceram 40, 360–364 (2018). https://doi.org/10.1007/s10832-018-0138-x
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s10832-018-0138-x