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A cospectral correction model for measurement of turbulent NO2 flux

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Abstract

A correction model for eddy correlation flux measurements is developed and applied to nitrogen dioxide flux measurements obtained from a SOLENT sonic anemometer and a Scintrex Luminox LMA-3 analyser for NO2. Four field campaigns were carried out near the village of Merenschwand in Central Switzerland from which two were selected for further analysis in this paper. The need for the correction of measured eddy covariance fluxes arises due to the damping loss of the NO2 analyser at high frequencies. This damping loss is described by an analogy to inductance in an electronical alternating current circuit. The independent variables in the correction model are:z (measuring height above zero-plane displacement),\(\bar u\) (mean horizontal wind speed), ζ (Monin-Obukhov stability parameter),f (natural frequency) and inductanceL. The value for inductanceL can be derived from spectral and cospectral analysis. The theoretical cospectrum of an ideal measurement is taken from Kaimalet al. (1972) and extended with a damping term in order to describe the real measurements of the cospectrum. The inductanceL of the LMA-3 with a 0.6 cm teflon aspiration tube of 5 m length lies in the order of 0.30 to 0.35 for the dataset from Merenschwand. With this inductance, a correction factor of 1.17 in August/September 1992 and of 1.18 in May 1993 was determined for the NO2 flux maxima during daytime. The range of the correction factor is 1.05 to 1.31 for the mean daily cycles of both datasets.

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References

  • Businger, J. A.: 1986, ‘Evaluation of the Accuracy with which Dry Deposition can be Measured with Current Micrometeorological Techniques’,J. Climate and Appl. Meteorol. 25, 1100–1124.

    Google Scholar 

  • Claussen, M.: 1985, ‘A Model of Turbulence Spectra in the Atmospheric Surface Layer’,Boundary-Layer Meteorol. 33, 151–172.

    Google Scholar 

  • Grant, A. L. M. and Watkins, R. D.: 1989, ‘Errors in Turbulence Measurements with a Sonic Anemometer’,Boundary-Layer Meteorol. 46, 181–194.

    Google Scholar 

  • Ellenberg, H.: 1990, ‘Ökologische Veränderungen in Biozönosen durch Stickstoffeintrag’, In:Ammoniak in der Umwelt — Kreisläufe, Wirkungen, Minderung, Darmstadt: Kuratorium für Technik und Bauwesen in der Landwirtschaft, 44.1–44.24.

    Google Scholar 

  • Hesterberg, R.: 1994,Die Stickoxide im schweizerischen Mittelland und der Stickstoffeintrag in ein Naturschutzgebiet, PhD-Thesis, University of Bern (unpublished).

  • Hesterberg, R., Blatter, A., Fahrni, M., Rosset, M., Neftel, A., Eugster W., and Wanner, H.: 1995, ‘Deposition of Nitrogen-Containing Compounds to a Non-Cultivated Area in Central Switzerland’,Environmental Pollution, accepted for publication.

  • Hicks, B. B. and McMillen, R. T.: 1988, ‘On the Measurement of Dry Deposition using Imperfect Sensors and in Non-Ideal Terrain’,Boundary-Layer Meteorol. 42, 79–94.

    Google Scholar 

  • Højstrup, J.: 1981, ‘A Simple Model for the Adjustment of Velocity Spectra in Unstable Conditions Downstream of an Abrupt Change in Roughness and Heat Flux’,Boundary-Layer Meteorol. 21, 341–356.

    Google Scholar 

  • Kaimal, J. C. and Gaynor, J. E.: 1991, ‘Another Look at Sonic Thermometry’,Boundary-Layer Meteorol. 56, 401–410.

    Google Scholar 

  • Kaimal, J. C. and Gaynor, J. E.: 1983, ‘The Boulder Atmospheric Observatory’,J. Climate and Appl. Meteorol. 22, 863–880.

    Google Scholar 

  • Kaimal, J. C., Wyngaard, J. C., and Haugen, D. A.: 1968, ‘Deriving Power Spectra from a Three-Component Sonic Anemometer’,J. Appl. Meteorol. 7, 827–837.

    Google Scholar 

  • Kaimal, J. C., Wyngaard, J. C., Izumi, Y., and Coté, O. R.: 1972, ‘Spectral Characteristics of Surface-Layer Turbulence’,Quart. J. Roy. Meteorol. Soc.,98, 563–589.

    Google Scholar 

  • Leuning, R. and Moncrieff, J.: 1990, ‘Eddy-Covariance CO2 Flux Measurements Using Open- and Closed-Path CO2 analysers: Corrections for Analyser Water Vapour Sensitivity and Damping of Fluctuations in Air Sampling Tubes’,Boundary-Layer Meteorol. 53, 63–76.

    Google Scholar 

  • Monin, A. S. and Obukhov, A. M.: 1954 ‘Osnovnye zakonomernosti turbulentnogo peremešivaniâ v prizemnom sloe atmosfery’,Trudy geofiz. inst. Akad. Nauk SSSR 24(151), 163–187.

    Google Scholar 

  • Moore, C. J.: 1986, ‘Frequency Response Corrections for Eddy Correlation Systems’,Boundary-Layer Meteorol. 37, 17–35.

    Google Scholar 

  • Panofsky, H. A.: 1978, ‘Matching in the Convective Planetary Boundary Layer’,J. Atmos. Sci. 35, 272–276.

    Google Scholar 

  • Panofsky, H. A. and Dutton, J. A.: 1984,Atmospheric Turbulence, John Wiley & Sons, New York.

    Google Scholar 

  • Panofsky, H. A., Larko, D., Lipschutz, R., Stone, G., Bradley, E. F., Bowen, A. J., and Højstrup, J.: 1982, ‘Spectra of Velocity Components over Complex Terrain’,Quart. J. Roy. Meteorol. Soc. 108, 215–230.

    Google Scholar 

  • Philip, J. R.: 1963a, ‘The Theory of Dispersal during Laminar Flow in Tubes. II’,Aust. J. Phys. 16, 300–310.

    Google Scholar 

  • Philip, J. R.: 1963b, ‘The Damping of a Fluctuating Concentration by Continuous Sampling through a Tube’,Aust. J. Phys. 16, 454–463.

    Google Scholar 

  • Pilegaard, K., Hummelshøj, P., and Jensen, N. O.:Deposition of Ozone and Nitrogen Dioxide to Open Land and Forests, Contribution to the BIATEX Workshop Aveiro, May 1993, 1–8.

  • Purcell, E. M.: 1965, ‘Electricity and Magnetism’,Berkeley Physics Course Vol. 2, McGraw-Hill Book, New York, 274–295.

    Google Scholar 

  • Skupniewicz, C. E., Kamada, R. F., and Schacher, G. E.: 1989, ‘Turbulence Measurements over Complex Terrain’,Boundary-Layer Meteorol. 48, 109–128.

    Google Scholar 

  • Vilá-Guerau de Arellano, J. and Duynkerke, P. G.: 1992, ‘Influence of Chemistry on the Flux-Gradient Relationship for the NO−O3−NO2 System’,Boundary-Layer Meteorol. 61, 375–387.

    Google Scholar 

  • Wyngaard, J. C. and Coté, O. R.: 1972, ‘Cospectral Similarity in the Atmospheric Surface Layer’,Quart. J. R. Met. Soc. 98, 590–603.

    Google Scholar 

  • Zeman, O. and Jensen, N. O.: 1987, ‘Modification of Turbulence Characteristics in Flow over Hills’,Quart. J. Roy. Meteorol. Soc. 113, 55–80.

    Google Scholar 

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Eugster, W., Senn, W. A cospectral correction model for measurement of turbulent NO2 flux. Boundary-Layer Meteorol 74, 321–340 (1995). https://doi.org/10.1007/BF00712375

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