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Two-Photon Excited Luminescence of NV-Centers and Stimulated Raman Scattering in Nanodiamonds

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Abstract

In this study, zero-phonon line (ZPL) at 638 nm associated with multiphoton excited negatively-charged single nitrogen-vacancy (NV)-center luminescence is registered in ethanol suspension of submicrometer diamond particles obtained at high pressures and high temperatures (HPHT). Simultaneously Stokes and anti-Stokes components of the stimulated Raman scattering (SRS) in the same sample is registered with a frequency shift of 1332 cm1 corresponding to the fundamental optical mode of the diamond crystal. We observe anti-Stokes component intensity enhancement caused by its wavelength coincidence with the wavelength of luminescence caused by negatively-charged single nitrogen-vacancy (NV) centers.

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Correspondence to A. D. Kudryavtseva.

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We dedicate this paper to Professor Vladimir S. Gorelik, our friend and collaborator during many years; this study is a continuation of our fruitful collaboration.

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Kudryavtseva, A.D., Shevchenko, M.A., Tcherniega, N.V. et al. Two-Photon Excited Luminescence of NV-Centers and Stimulated Raman Scattering in Nanodiamonds. J Russ Laser Res 42, 682–687 (2021). https://doi.org/10.1007/s10946-021-10010-5

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  • DOI: https://doi.org/10.1007/s10946-021-10010-5

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