Abstract
The reactions of halogens and their compounds, in particular of chlorine and chlorinated hydrocarbons (CHCs), are of growing interest to the combustion community because of the increasing role that incineration plays in the treatment of hazardous chemical wastes, which frequently contain these compounds. Although a reasonably large body of knowledge appears to exist on the rates and mechanisms of reactions of chlorine-containing species, most of our present understanding is derived from experiments done at or near ambient temperatures. Studies at high temperatures are limited; more are urgently needed for the development of quantitative detailed chemical kinetic mechanisms describing the oxidation and pyrolysis of CHCs at combustion conditions. To cope with the scarcity of high-temperature data, techniques have been developed to extrapolate rate information obtained at lower temperatures to combustion conditions, and these permit the available thermochemical and kinetic data to be used to develop mechanisms suitable for odeling the combustion of CHCs. For such modeling studies, however, it is required that the rate parameters of a large number of reactions be estimated. Although estimation in itself is not undesirable, as there will always be more reactions in such complex systems than resources available to study them individually in isolated experiments, experimental rate measurements on reactions of chlorinated species at combustion temperatures serve as vital references to assess the validity of predictions and to calibrate theoretical methods. Only with reliable experimental rate data together with robust theoretical methods will we be in a position to develop mechanisms with broad ranges of applicability and to address issues related to the formation and destruction of pollutants in the combustion of CHCs.
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Senkan, S.M. (2000). Survey of Rate Coefficients in the C-H-Cl-O System. In: Gardiner, W.C. (eds) Gas-Phase Combustion Chemistry. Springer, New York, NY. https://doi.org/10.1007/978-1-4612-1310-9_4
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