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In situ visualization of water transport in cement mortar with an ultra-low w/b ratio under the coupling conditions of osmotic pressure, confining pressure, and temperature

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Abstract

The deep underground environment has complex geological conditions, which result in cement-based materials under the coupling conditions of high crustal stress, high pressure, and high temperature for the long-term. Thus, the mechanism of water transport is more complicated and often accelerates the deterioration of cement-based materials. In this study, the rules of water transport in mortar with an ultra-low w/b ratio under the coupling conditions of osmotic pressure, confining pressure, and temperature were systemically investigated based on a novel experimental device and low-field NMR technology. Experimental results showed that the saturation of the pore structure and penetration depth of mortar increased rapidly in the early stage (the first 10 min), and the water was mainly filled in nano-scale pores. Low-field NMR imaging technology could be applied to the visualization study of water transport in WPC mortar. With the increase of osmotic pressure and ambient temperature, the penetration rate of water in mortar was significantly increased, and the water was preferentially filled in nano-scale pores with pore sizes less than approximately 200 nm. The increase of confining pressure could improve the permeability of mortar to a certain extent due to the decrease in the penetration rate of water. For water transport in mortar with an ultra-low w/b ratio, the descending order of influence degree of different factors was osmotic pressure, confining pressure, and temperature.

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References

  1. Zhang ZY, Zou Y, Yang J, Zhou JT (2022) Capillary rise height of sulfate in Portland-limestone cement concrete under physical attack: experimental and modelling investigation. Cem Concr Comp 125:104299

    Article  Google Scholar 

  2. Lv LS, Wang JY, Xiao RC, Fang MS, Tan Y (2021) Chloride ion transport properties in microcracked ultra-high performance concrete in the marine environment. Constr Build Mater 291:123310

    Article  Google Scholar 

  3. Babaee M, Castel A (2018) Water vapor sorption isotherms, pore structure, and moisture transport characteristics of alkali-activated and Portland cement-based binders. Cem Concr Res 113:99–120

    Article  Google Scholar 

  4. Caneda-Martinez L, Medina C, de Rojas MIS, Frias M (2019) Water transport in binary eco-cements containing coal mining waste. Cem Concr Comp 104:103373

    Article  Google Scholar 

  5. Cantero B, Bravo M, de Brito J, del Bosque IFS, Medina C (2021) Water transport and shrinkage in concrete made with ground recycled concrete-additioned cement and mixed recycled aggregate. Cem Concr Comp 118:103957

    Article  Google Scholar 

  6. Wu HX, Yang DY, Xu JG, Liang CF, Ma ZM (2021) Water transport and resistance improvement for the cementitious composites with eco-friendly powder from various concrete wastes. Constr Build Mater 290:123247

    Article  Google Scholar 

  7. Zhang ZD, Angst U (2020) A dual-permeability approach to study anomalous moisture transport properties of cement-based materials. Transp Porous Med 135(1):59–78

    Article  Google Scholar 

  8. Yang L, Zhang YS, Liu ZY, Zhao P, Liu C (2015) In-situ tracking of water transport in cement paste using X-ray computed tomography combined with CsCl enhancing. Mater Lett 160:381–383

    Article  Google Scholar 

  9. Yang L, Gao DY, Zhang YS, She W (2018) Study on water and chloride transport in cracked mortar using X-ray CT, gravimetric method and natural immersion method. Constr Build Mater 176:652–664

    Article  Google Scholar 

  10. Oesch T, Weise F, Meinel D, Gollwitzer C (2019) Quantitative in-situ analysis of water transport in concrete completed using X-ray computed tomography. Transp Porous Med 127(2):371–389

    Article  Google Scholar 

  11. Brew DRM, de Beer FC, Radebe MJ, Nshimirimana R, McGlinn PJ, Aldridge LP, Payne TE (2009) Water transport through cement-based barriers-A preliminary study using neutron radiography and tomography. Nucl Instrum Meth A 605(1–2):163–166

    Article  Google Scholar 

  12. Wang Y, Liu ZN, He FQ, Zhuo WD, Yuan Q, Chen CP, Yang JM (2021) Study on water instability of magnesium potassium phosphate cement mortar based on low-field 1H nuclear magnetic resonance. Measurement 44:109523

    Article  Google Scholar 

  13. Bao JW, Li SG, Yu ZH, Xu J, Li YL, Zhang P, Si Z, Gao S (2021) Water transport in recycled aggregate concrete under sustained compressive loading: experimental investigation and mesoscale numerical modelling. J Build Eng 44:103373

    Article  Google Scholar 

  14. Drouet E, Poyet S, Torrenti JM (2015) Temperature influence on water transport in hardened cement pastes. Cem Concr Res 76:37–50

    Article  Google Scholar 

  15. Gerard B, Breysse D, Ammouche A, Houdusse O, Didry O (1996) Cracking and permeability of concrete under tension. Mater Struct 29(3):141–151

    Article  Google Scholar 

  16. Yang ZF, Weiss WJ, Olek J (2006) Water transport in concrete damaged by tensile loading and freeze-thaw cycling. J Mater Civ Eng 18(3):424–434

    Article  Google Scholar 

  17. Mengel L, Krauss HW, Lowke D (2020) Water transport through cracks in plain and reinforced concrete - Influencing factors and open questions. Constr Build Mater 254:118990

    Article  Google Scholar 

  18. Wang K, Jansen DC, Shah SP, Karr AF (1997) Permeability study of cracked concrete. Cem Concr Res 27(3):381–393

    Article  Google Scholar 

  19. Li SC, Wang Q, Jiang B, He MC, Sun HB, Shao X, Wang CH, Qin Q, Yu HC (2017) Modeling and experimental study of mechanical properties of confined concrete arch in complicated deep underground engineering. Int J Geomech 17(6):04016137

    Article  Google Scholar 

  20. Cho BH, Nam BH, Seo S, Kim J, An J, Youn H (2019) Waterproofing performance of waterstop with adhesive bonding used at joints of underground concrete structures. Constr Build Mater 221:491–500

    Article  Google Scholar 

  21. Zhan PM, Xu J, Wang J, Jiang CH (2021) Multi-scale study on synergistic effect of cement replacement by metakaolin and typical supplementary cementitious materials on properties of ultra-high performance concrete. Constr Build Mater 307:125082

    Article  Google Scholar 

  22. Tahwia AM, Elgendy GM, Amin M (2021) Durability and microstructure of eco-efficient ultra-high-performance concrete. Constr Build Mater 303:124491

    Article  Google Scholar 

  23. Simina M, Molnar L, Manea D, Ardelean I (2012) Monitoring the air influence on cement-lime mortar hydration using low-field nuclear magnetic resonance relaxometry. Appl Magn Reson 43(3):443–450

    Article  Google Scholar 

  24. Wang BM, Zhang Y, Ma HN (2014) Porosity and pore size distribution measurement of cement/carbon nanofiber composites by H-1 low field nuclear magnetic resonance. J Wuhan Univ Technol 29(1):82–88

    Article  Google Scholar 

  25. She AM, Ma K, Liao G, Yao W, Zuo JQ (2021) Investigation of hydration and setting process in nanosilica-cement blended pastes: In situ characterization using low field nuclear magnetic resonance. Constr Build Mater 304:124631

    Article  Google Scholar 

  26. Liu KQ, Yang XS, Zhang H, Yao S, Huang ZL, Zhang XN, Cao Q, Li B, Luo Z, Cheng XW, Yang ZL, Chi CR (2021) Pore connectivity of oil well cement in the early hydration stage by in situ electrical resistivity measurements and low-field nuclear magnetic resonance. Constr Build Mater 303:12448

    Article  Google Scholar 

  27. Zhou CS, Ren FZ, Zeng Q, Xiao LZ, Wang W (2018) Pore-size resolved water vapor adsorption kinetics of white cement mortars as viewed from proton NMR relaxation. Cem Concr Res 105:31–43

    Article  Google Scholar 

  28. Wang YZ, Yang WC, Ge Y, Liu PH, Zhang A (2022) Analysis of freeze-thaw damage and pore structure deterioration of mortar by low-field NMR. Constr Build Mater 319:126097

    Article  Google Scholar 

  29. Zhang A, Yang WC, Ge Y, Wang YZ, Liu PH (2020) Study on the hydration and moisture transport of white cement containing nanomaterials by using low field nuclear magnetic resonance. Constr Build Mater 249:118788

    Article  Google Scholar 

  30. Zhao HT, Wu X, Huang YY, Zhang P, Tian Q, Liu JP (2021) Investigation of moisture transport in cement-based materials using low-field nuclear magnetic resonance imaging. Mag Concr Res 73(5):252–270

    Article  Google Scholar 

  31. McDonald PJ, Istok O, Janota M, Gajewicz-Jarmin AM, Faux DA (2020) Sorption, anomalous water transport and dynamic porosity in cement paste: a spatially localised 1H NMR relaxation study and a proposed mechanism. Cem Concr Res 133:106045

  32. de Cano-Barrita PF, Balcom BJ, Castellanos F (2017) Carbonation front in cement paste detected by T2 NMR measurements using a low field unilateral magnet. Mater Struct 50:150

    Article  Google Scholar 

  33. Mitchell J, Fordham EJ (2018) Sodium-23 NMR in porous media. Microporous Mesoporous Mater 269:109–112

    Article  Google Scholar 

  34. Ji YL, Pel L, Sun ZP (2022) NMR study on the early-age hydration and ion binding of the cement paste prepared with NaCl solutions. Cem Concr Comp 129:104489

    Article  Google Scholar 

  35. Gussoni M, Greco F, Bonazzi F, Vezzoli A, Botta D, Dotelli G, Natali Sora I, Pelosato R, Zetta L (2004) 1H NMR spin-spin relaxation and imaging in porous systems: an application to the morphological study of white portland cement during hydration in the presence of organics. Magn Reson Imaging 22(6):877–889

    Article  Google Scholar 

  36. Wang J, Dong S, Zhou C, Ashour A, Han B (2021) Investigating pore structure of nano-engineered concrete with low-field nuclear magnetic resonance. J Mater Sci 56(1):243–259

    Article  Google Scholar 

  37. Weng L, Wu Z, Zhang S, Liu Q, Chu Z (2022) Real-time characterization of the grouting diffusion process in fractured sandstone based on the low-field nuclear magnetic resonance technique. Int J Rock Mech Min Sci 152:105060

    Article  Google Scholar 

Download references

Acknowledgements

The authors gratefully acknowledge the financial support from the National Key Research and Development Program of China (2021YFB2601200), the National Natural Science Foundation of China (52078125, U21A20150, 52293431, 52208228), the Science Foundation for Distinguished Young Scholars of Jiangsu Province (BK20220071).

Funding

National Natural Science Foundation of China, 52078125, Zhiyong liu.

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Authors and Affiliations

  1. Jiangsu Key Laboratory for Construction Materials, Southeast University, Nanjing, 211189, China

    Zhiyong Liu, Yuncheng Wang, Yunsheng Zhang & Jinyang Jiang

  2. School of Materials Science and Engineering, Southeast University, Nanjing, 211189, China

    Zhiyong Liu

  3. School of Civil Engineering and Architecture, Anhui University of Science and Technology, Huainan, 232001, China

    Meng Wu

  4. State Key Laboratory of Geomechanics and Deep Underground Engineering, China University of Mining and Technology, Xuzhou, 221116, China

    Xizhi Xia

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  1. Zhiyong Liu
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Liu, Z., Wang, Y., Wu, M. et al. In situ visualization of water transport in cement mortar with an ultra-low w/b ratio under the coupling conditions of osmotic pressure, confining pressure, and temperature. Mater Struct 56, 68 (2023). https://doi.org/10.1617/s11527-023-02145-5

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