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Preparation and sodium-ion storage performance of bimetallic oxygen sulfide composite hollow carbon fibers

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Abstract

In sodium-ion storage technologies, the high radius of Na+ causes slow diffusion kinetics, and the repeated sodiation/desodiation will damage the electrode structure. Herein, the iron-tin oxysulfide (FSOS) is confined in the N-doped hollow carbon nanofibers through a coaxial electrospinning. FSOS with multiple cationic valences can promote the adsorption and redox reaction of Na+, which facilitate electrolyte penetration. For anode material in sodium-ion batteries (SIBs), FSOS@NSC offers competitive cycling performance (246 mA h g−1 after 1500 cycles with capacity retention of 80.3%) as well as high-rate capability (242 mA h g−1), and a sodium-ion capacitor device (SICs) with a large operating voltage window by using FSOS@NSC as the anode (0.01–4.0 V). FSOS@NSC//AC hybrid system delivers capacity retention of 74.6% at 20 A g−1 after 2000 cycles and high energy density (100.5 W h kg−1). This research offers a method for creating a new generation by anion regulation with partial sulfuration.

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Acknowledgments

The authors are thankful for funds from Natural Science Foundation of Shandong Province under Grant No. ZR2022ME131.

Funding

This study was funded by Natural Science Foundation of Shandong Province under Grant No. ZR2022ME131.

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  1. School of Materials Science and Engineering, Ocean University of China, Qingdao, 266100, People’s Republic of China

    Yilin Li, Zeyin He, Dong Han, Jing Shi & Huanlei Wang

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  1. Yilin Li
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YL contributed toward conceptualization, investigation, methodology, formal analysis, and writing –original draft. ZH contributed toward methodology, formal analysis, visualization, and data curation. DH contributed toward investigation, data curation, and visualization. JS contributed toward supervision, validation, resources, funding acquisition, and writing—review & editing. HW contributed toward visualization, supervision, and resources.

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Li, Y., He, Z., Han, D. et al. Preparation and sodium-ion storage performance of bimetallic oxygen sulfide composite hollow carbon fibers. Journal of Materials Research 39, 702–715 (2024). https://doi.org/10.1557/s43578-023-01261-w

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